Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules
Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas−solid...
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| Published in | Nature communications Vol. 9; no. 1; pp. 3880 - 11 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
24.09.2018
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-018-06317-8 |
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| Abstract | Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas−solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T
80
lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment.
Perovskite solar cells often suffer from poor uniformity and reproducibility especially in case of large area devices. Here Liu et al. developed a gas−solid reaction method that enables facile fabrication of over 1 µm thick perovskite films for solar modules with high efficiency, stability and reproducibility. |
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| AbstractList | Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T
lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. Perovskite solar cells often suffer from poor uniformity and reproducibility especially in case of large area devices. Here Liu et al. developed a gas−solid reaction method that enables facile fabrication of over 1 µm thick perovskite films for solar modules with high efficiency, stability and reproducibility. Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment.Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas−solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T 80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. Perovskite solar cells often suffer from poor uniformity and reproducibility especially in case of large area devices. Here Liu et al. developed a gas−solid reaction method that enables facile fabrication of over 1 µm thick perovskite films for solar modules with high efficiency, stability and reproducibility. Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas−solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T 80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 mu m in ambient condition on the basis of the fast gas-solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 +/- 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cmx 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T-80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a simple perovskite formation method to fabricate perovskite films with thickness over 1 μm in ambient condition on the basis of the fast gas−solid reaction of chlorine-incorporated hydrogen lead triiodide and methylamine gas. The resultant thick and smooth chlorine-incorporated perovskite films exhibit full coverage, improved crystallinity, low surface roughness and low thickness variation. The resultant PSCs achieve an average power conversion efficiency of 19.1 ± 0.4% with good reproducibility. Meanwhile, this method enables an active area efficiency of 15.3% for 5 cm × 5 cm solar modules. The un-encapsulated PSCs exhibit an excellent T80 lifetime exceeding 1600 h under continuous operation conditions in dry nitrogen environment. |
| ArticleNumber | 3880 |
| Author | Liu, Zonghao Raga, Sonia R. Hawash, Zafer Kim, Taehoon Juarez-Perez, Emilio J. Liu, Shengzhong (Frank) Qiu, Longbin Ono, Luis K. Qi, Yabing Jiang, Yan Wu, Zhifang |
| Author_xml | – sequence: 1 givenname: Zonghao surname: Liu fullname: Liu, Zonghao organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 2 givenname: Longbin surname: Qiu fullname: Qiu, Longbin organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 3 givenname: Emilio J. orcidid: 0000-0001-6040-1920 surname: Juarez-Perez fullname: Juarez-Perez, Emilio J. organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 4 givenname: Zafer orcidid: 0000-0001-9606-3521 surname: Hawash fullname: Hawash, Zafer organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 5 givenname: Taehoon orcidid: 0000-0003-2145-5293 surname: Kim fullname: Kim, Taehoon organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 6 givenname: Yan orcidid: 0000-0001-7665-1174 surname: Jiang fullname: Jiang, Yan organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 7 givenname: Zhifang surname: Wu fullname: Wu, Zhifang organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 8 givenname: Sonia R. surname: Raga fullname: Raga, Sonia R. organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 9 givenname: Luis K. surname: Ono fullname: Ono, Luis K. organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) – sequence: 10 givenname: Shengzhong (Frank) surname: Liu fullname: Liu, Shengzhong (Frank) organization: Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology, School of Materials Science and Engineering, Shaanxi Normal University, Dalian National Laboratory for Clean Energy, iChEM, Dalian Institute of Chemical Physics, Chinese Academy of Sciences – sequence: 11 givenname: Yabing orcidid: 0000-0002-4876-8049 surname: Qi fullname: Qi, Yabing email: Yabing.Qi@OIST.jp organization: Energy Materials and Surface Sciences Unit (EMSSU), Okinawa Institute of Science and Technology Graduate University (OIST) |
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| Snippet | Besides high efficiency, the stability and reproducibility of perovskite solar cells (PSCs) are also key for their commercialization. Herein, we report a... Perovskite solar cells often suffer from poor uniformity and reproducibility especially in case of large area devices. Here Liu et al. developed a gas−solid... |
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| SubjectTerms | 147/135 147/3 639/301/299/946 639/4077/4072/4062 Chlorine Commercialization Efficiency Energy conversion efficiency Gas-solid reactions Humanities and Social Sciences Lead Materials Engineering Materialteknik Methylamine Modules multidisciplinary Perovskites Photovoltaic cells Reproducibility Science Science (multidisciplinary) Solar cells Surface roughness Thick films Thickness |
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| Title | Gas-solid reaction based over one-micrometer thick stable perovskite films for efficient solar cells and modules |
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