Covalent Selenium Embedded in Hierarchical Carbon Nanofibers for Ultra-High Areal Capacity Li-Se Batteries
Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we...
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| Published in | iScience Vol. 23; no. 3; p. 100919 |
|---|---|
| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
27.03.2020
Elsevier |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2589-0042 2589-0042 |
| DOI | 10.1016/j.isci.2020.100919 |
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| Abstract | Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm−2 displays a specific capacity of 762 mAh g−1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm−2, ultra-high areal capacities of 7.30 mAh cm−2 is achieved, which greatly exceeds those reported previously for Li-Se batteries.
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•The CSe@HNCNFs were used as flexible and free-standing cathode for Li-Se battery•The CSe@HNCNFs effectively retard polyselenides diffusion during cycling•The CSe@HNCNFs delivered high areal capacity of 7.30 mAh cm−2•The CSe@HNCNFs displayed excellent cyclic stability and rate performance
Energy Storage; Materials Characterization Techniques; Nanostructure |
|---|---|
| AbstractList | Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm−2 displays a specific capacity of 762 mAh g−1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm−2, ultra-high areal capacities of 7.30 mAh cm−2 is achieved, which greatly exceeds those reported previously for Li-Se batteries.
[Display omitted]
•The CSe@HNCNFs were used as flexible and free-standing cathode for Li-Se battery•The CSe@HNCNFs effectively retard polyselenides diffusion during cycling•The CSe@HNCNFs delivered high areal capacity of 7.30 mAh cm−2•The CSe@HNCNFs displayed excellent cyclic stability and rate performance
Energy Storage; Materials Characterization Techniques; Nanostructure Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm−2 displays a specific capacity of 762 mAh g−1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm−2, ultra-high areal capacities of 7.30 mAh cm−2 is achieved, which greatly exceeds those reported previously for Li-Se batteries. • The CSe@HNCNFs were used as flexible and free-standing cathode for Li-Se battery • The CSe@HNCNFs effectively retard polyselenides diffusion during cycling • The CSe@HNCNFs delivered high areal capacity of 7.30 mAh cm−2 • The CSe@HNCNFs displayed excellent cyclic stability and rate performance Energy Storage; Materials Characterization Techniques; Nanostructure Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L . However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm displays a specific capacity of 762 mAh g after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm , ultra-high areal capacities of 7.30 mAh cm is achieved, which greatly exceeds those reported previously for Li-Se batteries. Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm−2 displays a specific capacity of 762 mAh g−1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm−2, ultra-high areal capacities of 7.30 mAh cm−2 is achieved, which greatly exceeds those reported previously for Li-Se batteries. : Energy Storage; Materials Characterization Techniques; Nanostructure Subject Areas: Energy Storage, Materials Characterization Techniques, Nanostructure Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L-1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm-2 displays a specific capacity of 762 mAh g-1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm-2, ultra-high areal capacities of 7.30 mAh cm-2 is achieved, which greatly exceeds those reported previously for Li-Se batteries.Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L-1. However, current studies are largely limited to electrodes with rather low mass loading and low areal capacity, resulting in low volumetric performance. Herein, we report a design of covalent selenium embedded in hierarchical nitrogen-doped carbon nanofibers (CSe@HNCNFs) for ultra-high areal capacity Li-Se batteries. The CSe@HNCNFs provide excellent ion and electron transport performance, whereas effectively retard polyselenides diffusion during cycling. We show that the Li-Se battery with mass loading of 1.87 mg cm-2 displays a specific capacity of 762 mAh g-1 after 2,500 cycles, with almost no capacity fading. Furthermore, by increasing the mass loading to 37.31 mg cm-2, ultra-high areal capacities of 7.30 mAh cm-2 is achieved, which greatly exceeds those reported previously for Li-Se batteries. |
| ArticleNumber | 100919 |
| Author | Zhou, Jian Li, Shengyang Duan, Xiangfeng Chen, Maoxin Zhu, Jian Wang, Tao Zhang, Meng Liu, Jialing Xu, Hanjiao Zhang, Qiusheng Liang, Junfei |
| AuthorAffiliation | 1 State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China 2 Department of Chemistry and Biochemistry, University of California, Los Angeles, CA 90095, USA 3 School of Energy and Power Engineering, North University of China, Taiyuan, Shanxi 030051, P. R. China |
| AuthorAffiliation_xml | – name: 3 School of Energy and Power Engineering, North University of China, Taiyuan, Shanxi 030051, P. R. China – name: 1 State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – name: 2 Department of Chemistry and Biochemistry, University of California, Los Angeles, CA 90095, USA |
| Author_xml | – sequence: 1 givenname: Jian surname: Zhou fullname: Zhou, Jian organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 2 givenname: Maoxin surname: Chen fullname: Chen, Maoxin organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 3 givenname: Tao surname: Wang fullname: Wang, Tao organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 4 givenname: Shengyang surname: Li fullname: Li, Shengyang organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 5 givenname: Qiusheng surname: Zhang fullname: Zhang, Qiusheng organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 6 givenname: Meng surname: Zhang fullname: Zhang, Meng organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 7 givenname: Hanjiao surname: Xu fullname: Xu, Hanjiao organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 8 givenname: Jialing surname: Liu fullname: Liu, Jialing organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 9 givenname: Junfei surname: Liang fullname: Liang, Junfei organization: Department of Chemistry and Biochemistry, University of California, Los Angeles, CA 90095, USA – sequence: 10 givenname: Jian orcidid: 0000-0001-9852-1645 surname: Zhu fullname: Zhu, Jian email: jzhu@hnu.edu.cn organization: State Key Laboratory for Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, and Hunan Key Laboratory of Two-Dimensional Materials, Hunan University, Changsha 410082, P. R. China – sequence: 11 givenname: Xiangfeng surname: Duan fullname: Duan, Xiangfeng organization: Department of Chemistry and Biochemistry, University of California, Los Angeles, CA 90095, USA |
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| Snippet | Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L−1. However, current... Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L . However, current... Lithium selenium (Li-Se) batteries have attracted increasing interest for its high theoretical volumetric capacities up to 3,253 Ah L-1. However, current... |
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| StartPage | 100919 |
| SubjectTerms | Energy Storage Materials Characterization Techniques Nanostructure |
| Title | Covalent Selenium Embedded in Hierarchical Carbon Nanofibers for Ultra-High Areal Capacity Li-Se Batteries |
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