Nitrogenated holey two-dimensional structures
Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we...
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| Published in | Nature communications Vol. 6; no. 1; p. 6486 |
|---|---|
| Main Authors | , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
06.03.2015
Nature Publishing Group Nature Pub. Group |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/ncomms7486 |
Cover
| Abstract | Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C
2
N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10
7
, with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C
2
N-
h
2D crystal has potential for use in practical applications.
There is currently interest in two-dimensional graphene-like materials incorporating heteroatoms. Here, the authors synthesize a solution-processable, holey two-dimensional network with C
2
N stoichiometry containing evenly distributed holes and nitrogen atoms, and use it to fabricate a field effect transistor. |
|---|---|
| AbstractList | Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C
2
N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10
7
, with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C
2
N-
h
2D crystal has potential for use in practical applications.
There is currently interest in two-dimensional graphene-like materials incorporating heteroatoms. Here, the authors synthesize a solution-processable, holey two-dimensional network with C
2
N stoichiometry containing evenly distributed holes and nitrogen atoms, and use it to fabricate a field effect transistor. Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C2 N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 107 , with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C2 N-h2D crystal has potential for use in practical applications. Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C2N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10(7), with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C2N-h2D crystal has potential for use in practical applications. Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C2N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10(7), with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C2N-h2D crystal has potential for use in practical applications.Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C2N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10(7), with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C2N-h2D crystal has potential for use in practical applications. Recent graphene research has triggered enormous interest in new two-dimensional ordered crystals constructed by the inclusion of elements other than carbon for bandgap opening. The design of new multifunctional two-dimensional materials with proper bandgap has become an important challenge. Here we report a layered two-dimensional network structure that possesses evenly distributed holes and nitrogen atoms and a C 2 N stoichiometry in its basal plane. The two-dimensional structure can be efficiently synthesized via a simple wet-chemical reaction and confirmed with various characterization techniques, including scanning tunnelling microscopy. Furthermore, a field-effect transistor device fabricated using the material exhibits an on/off ratio of 10 7 , with calculated and experimental bandgaps of approximately 1.70 and 1.96 eV, respectively. In view of the simplicity of the production method and the advantages of the solution processability, the C 2 N- h 2D crystal has potential for use in practical applications. |
| ArticleNumber | 6486 |
| Author | Jung, Sun-Min Seo, Jeong-Min Baek, Jong-Beom Shin, Hyung-Joon Shin, Dongbin Park, Noejung Lee, Eun Kwang Jung, Minbok Mahmood, Javeed Oh, Joon Hak Bae, Seo-Yoon Sohn, So-Dam Choi, Hyun-Jung Jeon, In-Yup |
| Author_xml | – sequence: 1 givenname: Javeed surname: Mahmood fullname: Mahmood, Javeed organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 2 givenname: Eun Kwang surname: Lee fullname: Lee, Eun Kwang organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon, Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), 77 Cheongam – sequence: 3 givenname: Minbok surname: Jung fullname: Jung, Minbok organization: School of Materials Science and Engineering/Low-Dimensional Carbon Materials Center/KIST-UNIST Ulsan Center for Convergent Materials, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 4 givenname: Dongbin surname: Shin fullname: Shin, Dongbin organization: Department of Physics, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 5 givenname: In-Yup surname: Jeon fullname: Jeon, In-Yup organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 6 givenname: Sun-Min surname: Jung fullname: Jung, Sun-Min organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 7 givenname: Hyun-Jung surname: Choi fullname: Choi, Hyun-Jung organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 8 givenname: Jeong-Min surname: Seo fullname: Seo, Jeong-Min organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 9 givenname: Seo-Yoon surname: Bae fullname: Bae, Seo-Yoon organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 10 givenname: So-Dam surname: Sohn fullname: Sohn, So-Dam organization: School of Materials Science and Engineering/Low-Dimensional Carbon Materials Center/KIST-UNIST Ulsan Center for Convergent Materials, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 11 givenname: Noejung surname: Park fullname: Park, Noejung organization: Department of Physics, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 12 givenname: Joon Hak surname: Oh fullname: Oh, Joon Hak email: joonhoh@postech.ac.kr organization: Department of Chemical Engineering, Pohang University of Science and Technology (POSTECH), 77 Cheongam – sequence: 13 givenname: Hyung-Joon surname: Shin fullname: Shin, Hyung-Joon email: shinhj@unist.ac.kr organization: School of Materials Science and Engineering/Low-Dimensional Carbon Materials Center/KIST-UNIST Ulsan Center for Convergent Materials, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon – sequence: 14 givenname: Jong-Beom surname: Baek fullname: Baek, Jong-Beom email: jbbaek@unist.ac.kr organization: School of Energy and Chemical Engineering/Low-Dimensional Carbon Materials Center, Ulsan National Institute of Science and Technology (UNIST), 100 Banyeon |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/25744355$$D View this record in MEDLINE/PubMed |
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| Title | Nitrogenated holey two-dimensional structures |
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