Identifying and manipulating single atoms with scanning transmission electron microscopy

The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including therm...

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Published inChemical communications (Cambridge, England) Vol. 58; no. 88; pp. 12274 - 12285
Main Author Susi, Toma
Format Journal Article
LanguageEnglish
Published England Royal Society of Chemistry 03.11.2022
The Royal Society of Chemistry
Subjects
Carbon nanotubes
Chemistry
Crystal structure
Electron beams
Electron irradiation
Graphene
Graphite - chemistry
Microscopy, Electron, Scanning Transmission
Nanotubes, Carbon - chemistry
Radiation damage
Scanning probe microscopes
Scanning transmission electron microscopy
Silicon - chemistry
Thermal stability
Online AccessGet full text
ISSN1359-7345
1364-548X
1364-548X
DOI10.1039/d2cc04807h

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Abstract The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including thermal stability of the manipulated structures, the ability to reach into bulk crystals, and the chemical identification of single atoms. However, energetic electron irradiation also presents unique challenges, with an inevitable possibility of irradiation damage. Understanding the underlying mechanisms will undoubtedly continue to play an important role to guide experiments. Great progress has been made in several materials including graphene, carbon nanotubes, and crystalline silicon in the eight years since the discovery of electron-beam manipulation, but the important challenges that remain will determine how far we can expect to progress in the near future. A focused electron beam can be used to manipulate covalently bound impurities within crystal lattices with atomic precision.
AbstractList The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including thermal stability of the manipulated structures, the ability to reach into bulk crystals, and the chemical identification of single atoms. However, energetic electron irradiation also presents unique challenges, with an inevitable possibility of irradiation damage. Understanding the underlying mechanisms will undoubtedly continue to play an important role to guide experiments. Great progress has been made in several materials including graphene, carbon nanotubes, and crystalline silicon in the eight years since the discovery of electron-beam manipulation, but the important challenges that remain will determine how far we can expect to progress in the near future.The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including thermal stability of the manipulated structures, the ability to reach into bulk crystals, and the chemical identification of single atoms. However, energetic electron irradiation also presents unique challenges, with an inevitable possibility of irradiation damage. Understanding the underlying mechanisms will undoubtedly continue to play an important role to guide experiments. Great progress has been made in several materials including graphene, carbon nanotubes, and crystalline silicon in the eight years since the discovery of electron-beam manipulation, but the important challenges that remain will determine how far we can expect to progress in the near future.
The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including thermal stability of the manipulated structures, the ability to reach into bulk crystals, and the chemical identification of single atoms. However, energetic electron irradiation also presents unique challenges, with an inevitable possibility of irradiation damage. Understanding the underlying mechanisms will undoubtedly continue to play an important role to guide experiments. Great progress has been made in several materials including graphene, carbon nanotubes, and crystalline silicon in the eight years since the discovery of electron-beam manipulation, but the important challenges that remain will determine how far we can expect to progress in the near future.
The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a scanning transmission electron microscope instead of a physical tip in a scanning probe microscope confers several benefits, including thermal stability of the manipulated structures, the ability to reach into bulk crystals, and the chemical identification of single atoms. However, energetic electron irradiation also presents unique challenges, with an inevitable possibility of irradiation damage. Understanding the underlying mechanisms will undoubtedly continue to play an important role to guide experiments. Great progress has been made in several materials including graphene, carbon nanotubes, and crystalline silicon in the eight years since the discovery of electron-beam manipulation, but the important challenges that remain will determine how far we can expect to progress in the near future. A focused electron beam can be used to manipulate covalently bound impurities within crystal lattices with atomic precision.
Author Susi, Toma
AuthorAffiliation Faculty of Physics
University of Vienna
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/36260089$$D View this record in MEDLINE/PubMed
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Notes Toma Susi received his MSc in Engineering Physics from Helsinki University of Technology and his doctorate in Engineering Physics and Physics from Aalto University, Finland. He is currently an Associate Professor at the Faculty of Physics of the University of Vienna, Austria. He has worked on materials synthesis, spectroscopy, electron microscopy and modeling, primarily on heteroatom-doped graphene and carbon nanotubes. His research interests increasingly center on understanding and making use of focused electron irradiation to characterize and manipulate materials, and on simulating transmission electron microscopy from first principles.
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Snippet The manipulation of individual atoms has developed from visionary speculation into an established experimental science. Using focused electron irradiation in a...
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SubjectTerms Carbon nanotubes
Chemistry
Crystal structure
Electron beams
Electron irradiation
Graphene
Graphite - chemistry
Microscopy, Electron, Scanning Transmission
Nanotubes, Carbon - chemistry
Radiation damage
Scanning probe microscopes
Scanning transmission electron microscopy
Silicon - chemistry
Thermal stability
Title Identifying and manipulating single atoms with scanning transmission electron microscopy
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