High stretchable and self-healing nanocellulose-poly(acrylic acid) composite hydrogels for sustainable CO2 shutoff
The injection of CO2 into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical...
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| Published in | Carbohydrate polymers Vol. 311; p. 120759 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier Ltd
01.07.2023
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0144-8617 1879-1344 1879-1344 |
| DOI | 10.1016/j.carbpol.2023.120759 |
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| Abstract | The injection of CO2 into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical properties, fatigue resistance, elastic and self-healing properties for the CO2 shutoff purpose. This gel consisting of grafted nanocellulose and polymer network was synthesized via a free-radical polymerization, and reinforced by using Fe3+ to cross-link the two networks. The as-prepared PAA-TOCNF-Fe3+ gel has a stress of 1.03 MPa and a high strain of 1491 %, and self-heals to its original 98 % in stress and 96 % in strain after rupture, respectively. The introduce of TOCNF/Fe3+ improves the excellent energy dissipation and self-healing via the synergy effect of dynamical coordination bonds and hydrogen bonds. Further, the PAA-TOCNF-Fe3+ gel is both flexible and high-strength in plugging the multi-round CO2 injection, during which the CO2 breakthrough pressure is above 9.9 MPa/m, the plugging efficiency exceeds 96 %, and the self-healing rate is larger than 90 %. Given that above, this gel shows a great potential to plug the high-pressure CO2 flow, which could offer a new method for CO2-EOR and carbon storage.
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| AbstractList | The injection of CO2 into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical properties, fatigue resistance, elastic and self-healing properties for the CO2 shutoff purpose. This gel consisting of grafted nanocellulose and polymer network was synthesized via a free-radical polymerization, and reinforced by using Fe3+ to cross-link the two networks. The as-prepared PAA-TOCNF-Fe3+ gel has a stress of 1.03 MPa and a high strain of 1491 %, and self-heals to its original 98 % in stress and 96 % in strain after rupture, respectively. The introduce of TOCNF/Fe3+ improves the excellent energy dissipation and self-healing via the synergy effect of dynamical coordination bonds and hydrogen bonds. Further, the PAA-TOCNF-Fe3+ gel is both flexible and high-strength in plugging the multi-round CO2 injection, during which the CO2 breakthrough pressure is above 9.9 MPa/m, the plugging efficiency exceeds 96 %, and the self-healing rate is larger than 90 %. Given that above, this gel shows a great potential to plug the high-pressure CO2 flow, which could offer a new method for CO2-EOR and carbon storage.The injection of CO2 into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical properties, fatigue resistance, elastic and self-healing properties for the CO2 shutoff purpose. This gel consisting of grafted nanocellulose and polymer network was synthesized via a free-radical polymerization, and reinforced by using Fe3+ to cross-link the two networks. The as-prepared PAA-TOCNF-Fe3+ gel has a stress of 1.03 MPa and a high strain of 1491 %, and self-heals to its original 98 % in stress and 96 % in strain after rupture, respectively. The introduce of TOCNF/Fe3+ improves the excellent energy dissipation and self-healing via the synergy effect of dynamical coordination bonds and hydrogen bonds. Further, the PAA-TOCNF-Fe3+ gel is both flexible and high-strength in plugging the multi-round CO2 injection, during which the CO2 breakthrough pressure is above 9.9 MPa/m, the plugging efficiency exceeds 96 %, and the self-healing rate is larger than 90 %. Given that above, this gel shows a great potential to plug the high-pressure CO2 flow, which could offer a new method for CO2-EOR and carbon storage. The injection of CO₂ into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical properties, fatigue resistance, elastic and self-healing properties for the CO₂ shutoff purpose. This gel consisting of grafted nanocellulose and polymer network was synthesized via a free-radical polymerization, and reinforced by using Fe³⁺ to cross-link the two networks. The as-prepared PAA-TOCNF-Fe³⁺ gel has a stress of 1.03 MPa and a high strain of 1491 %, and self-heals to its original 98 % in stress and 96 % in strain after rupture, respectively. The introduce of TOCNF/Fe³⁺ improves the excellent energy dissipation and self-healing via the synergy effect of dynamical coordination bonds and hydrogen bonds. Further, the PAA-TOCNF-Fe³⁺ gel is both flexible and high-strength in plugging the multi-round CO₂ injection, during which the CO₂ breakthrough pressure is above 9.9 MPa/m, the plugging efficiency exceeds 96 %, and the self-healing rate is larger than 90 %. Given that above, this gel shows a great potential to plug the high-pressure CO₂ flow, which could offer a new method for CO₂-EOR and carbon storage. The injection of CO2 into oil reservoirs to enhance oil recovery (EOR) has become a widely accepted and effective technical method, which, however, remains subject to the gas channeling caused by the reservoir fractures. Herein, this work developed a novel plugging gel combining excellent mechanical properties, fatigue resistance, elastic and self-healing properties for the CO2 shutoff purpose. This gel consisting of grafted nanocellulose and polymer network was synthesized via a free-radical polymerization, and reinforced by using Fe3+ to cross-link the two networks. The as-prepared PAA-TOCNF-Fe3+ gel has a stress of 1.03 MPa and a high strain of 1491 %, and self-heals to its original 98 % in stress and 96 % in strain after rupture, respectively. The introduce of TOCNF/Fe3+ improves the excellent energy dissipation and self-healing via the synergy effect of dynamical coordination bonds and hydrogen bonds. Further, the PAA-TOCNF-Fe3+ gel is both flexible and high-strength in plugging the multi-round CO2 injection, during which the CO2 breakthrough pressure is above 9.9 MPa/m, the plugging efficiency exceeds 96 %, and the self-healing rate is larger than 90 %. Given that above, this gel shows a great potential to plug the high-pressure CO2 flow, which could offer a new method for CO2-EOR and carbon storage. [Display omitted] |
| ArticleNumber | 120759 |
| Author | Huang, Xueli Wei, Peng Qi, Ying Liu, Ziteng Xie, Yahong |
| Author_xml | – sequence: 1 givenname: Ziteng surname: Liu fullname: Liu, Ziteng – sequence: 2 givenname: Peng surname: Wei fullname: Wei, Peng email: weipeng369@xju.edu.cn – sequence: 3 givenname: Ying surname: Qi fullname: Qi, Ying – sequence: 4 givenname: Xueli surname: Huang fullname: Huang, Xueli – sequence: 5 givenname: Yahong surname: Xie fullname: Xie, Yahong email: xyh0707@163.com |
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| Keywords | Nanocellulose CO2 shutoff Self-healing Dual-crosslinked hydrogel |
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| SubjectTerms | carbon dioxide carbon sequestration cellulose CO2 shutoff Dual-crosslinked hydrogel energy hydrogels hydrogen Nanocellulose oils polymerization polymers Self-healing |
| Title | High stretchable and self-healing nanocellulose-poly(acrylic acid) composite hydrogels for sustainable CO2 shutoff |
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