A low-cost attempt to improve electrochemical performances of pitch-based hard carbon anodes in lithium-ion batteries by oxidative stabilization
The electrochemical performance of low-cost, pitch-based hard carbon anodes in lithium-ion batteries is reported. Pitch-based hard carbon anodes were prepared, stabilized in air at 290 °C for 1 h after different temperature programming, and then carbonized in N 2 at 1000 °C. The optimal anode with t...
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| Published in | Journal of solid state electrochemistry Vol. 21; no. 2; pp. 555 - 562 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer Berlin Heidelberg
01.02.2017
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1432-8488 1433-0768 |
| DOI | 10.1007/s10008-016-3406-1 |
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| Abstract | The electrochemical performance of low-cost, pitch-based hard carbon anodes in lithium-ion batteries is reported. Pitch-based hard carbon anodes were prepared, stabilized in air at 290 °C for 1 h after different temperature programming, and then carbonized in N
2
at 1000 °C. The optimal anode with temperature programming of 24 h had abundant oxygenic functional groups, a large interlayer space, and a stable morphology. When used as anodes in lithium-ion batteries after 100 cycles at a current density of 100 mA g
−1
, the capacity was 258.6 mAh g
−1
with a capacity retention ratio of 90.6 %. This large capacity combined with the superior cycling performance indicates that prolonged oxidative stabilization is an effective strategy in improving electrochemical performances of lithium-ion batteries. |
|---|---|
| AbstractList | The electrochemical performance of low-cost, pitch-based hard carbon anodes in lithium-ion batteries is reported. Pitch-based hard carbon anodes were prepared, stabilized in air at 290 °C for 1 h after different temperature programming, and then carbonized in N
2
at 1000 °C. The optimal anode with temperature programming of 24 h had abundant oxygenic functional groups, a large interlayer space, and a stable morphology. When used as anodes in lithium-ion batteries after 100 cycles at a current density of 100 mA g
−1
, the capacity was 258.6 mAh g
−1
with a capacity retention ratio of 90.6 %. This large capacity combined with the superior cycling performance indicates that prolonged oxidative stabilization is an effective strategy in improving electrochemical performances of lithium-ion batteries. The electrochemical performance of low-cost, pitch-based hard carbon anodes in lithium-ion batteries is reported. Pitch-based hard carbon anodes were prepared, stabilized in air at 290 °C for 1 h after different temperature programming, and then carbonized in N2 at 1000 °C. The optimal anode with temperature programming of 24 h had abundant oxygenic functional groups, a large interlayer space, and a stable morphology. When used as anodes in lithium-ion batteries after 100 cycles at a current density of 100 mA g−1, the capacity was 258.6 mAh g−1 with a capacity retention ratio of 90.6 %. This large capacity combined with the superior cycling performance indicates that prolonged oxidative stabilization is an effective strategy in improving electrochemical performances of lithium-ion batteries. |
| Author | Wang, Cheng-Yang Zhao, Pin-Yi Tang, Jia-Ji |
| Author_xml | – sequence: 1 givenname: Pin-Yi surname: Zhao fullname: Zhao, Pin-Yi organization: Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 2 givenname: Jia-Ji surname: Tang fullname: Tang, Jia-Ji organization: Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) – sequence: 3 givenname: Cheng-Yang surname: Wang fullname: Wang, Cheng-Yang email: cywang@tju.edu.cn organization: Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering and Technology, Tianjin University, Collaborative Innovation Center of Chemical Science and Engineering (Tianjin) |
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| Snippet | The electrochemical performance of low-cost, pitch-based hard carbon anodes in lithium-ion batteries is reported. Pitch-based hard carbon anodes were prepared,... |
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| SubjectTerms | Analytical Chemistry Anodes Anodizing Carbon Characterization and Evaluation of Materials Chemistry Chemistry and Materials Science Condensed Matter Physics Electrochemical analysis Electrochemistry Energy Storage Functional groups Interlayers Lithium-ion batteries Low cost Original Paper Physical Chemistry Stabilization |
| Title | A low-cost attempt to improve electrochemical performances of pitch-based hard carbon anodes in lithium-ion batteries by oxidative stabilization |
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