Regeneration of Acid Orange 7 Exhausted Granular Activated Carbon Using Pulsed Discharge Plasmas

In this paper, a pulsed discharge plasma （PDP） system with a multi-needle-to-plate electrodes geometry was set up to investigate the regeneration of acid orange 7 （AO7） exhausted granular activated carbon （GAC）. Regeneration of GAC was studied under different conditions of peak pulse discharge volta...

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Published inPlasma science & technology Vol. 17; no. 10; pp. 881 - 886
Main Author 王慧娟 郭贺 刘永杰 依成武
Format Journal Article
LanguageEnglish
Published 01.10.2015
Subjects
Discharge
Electric potential
Plasmas
Regeneration
Scanning electron microscopy
Voltage
X-ray diffraction
XRD分析
初始pH值
扫描电子显微镜
放电电压
活性炭再生
脉冲放电等离子体
酸性橙7
颗粒活性炭
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ISSN1009-0630
DOI10.1088/1009-0630/17/10/12

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Summary:In this paper, a pulsed discharge plasma （PDP） system with a multi-needle-to-plate electrodes geometry was set up to investigate the regeneration of acid orange 7 （AO7） exhausted granular activated carbon （GAC）. Regeneration of GAC was studied under different conditions of peak pulse discharge voltage and water pH, as well as the modification effect of GAC by the pulse discharge process, to figure out the regeneration efficiency and the change of the GAC structure by the PDP treatment. The obtained results showed that there was an appropriate peak pulse voltage and an optimal initial pH value of the solution for GAC regeneration. Analyses of scanning electron microscope （SEM）, Boehm titration, Brunauer-Emmett-Teller （BET）, Horvath-Kawazoe （HK）, and X-ray Diffraction （XRD） showed that there were more mesopore and macropore in the regenerated GAC and the structure turned smoother with the increase of discharge voltage; the amount of acidic functional groups on the GAC surface increased while the amount of basic functional groups decreased after the regeneration process. From the result of the XRD analysis, there were no new substances produced on the GAC after PDP treatment.
Bibliography:In this paper, a pulsed discharge plasma （PDP） system with a multi-needle-to-plate electrodes geometry was set up to investigate the regeneration of acid orange 7 （AO7） exhausted granular activated carbon （GAC）. Regeneration of GAC was studied under different conditions of peak pulse discharge voltage and water pH, as well as the modification effect of GAC by the pulse discharge process, to figure out the regeneration efficiency and the change of the GAC structure by the PDP treatment. The obtained results showed that there was an appropriate peak pulse voltage and an optimal initial pH value of the solution for GAC regeneration. Analyses of scanning electron microscope （SEM）, Boehm titration, Brunauer-Emmett-Teller （BET）, Horvath-Kawazoe （HK）, and X-ray Diffraction （XRD） showed that there were more mesopore and macropore in the regenerated GAC and the structure turned smoother with the increase of discharge voltage; the amount of acidic functional groups on the GAC surface increased while the amount of basic functional groups decreased after the regeneration process. From the result of the XRD analysis, there were no new substances produced on the GAC after PDP treatment.
WANG Huijuan, GUO He, LIU Yongjie, YI Chengwu （ School of the Environment and Safety Engineering, Jiangsu University, Zhenjiang 212013, China）
pulsed discharge plasma, acid orange 7, granular activated carbon, regeneration, pore structure, functional groups
34-1187/TL
ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:1009-0630
DOI:10.1088/1009-0630/17/10/12