Photoelectron diffraction, multi-atom resonant photoemission, pioneered by Fadley

We discuss two important subjects pioneered by Fadley. As the first topic, we discuss the energy dependence of the intensity ratio observed in Mn 3s multiplet splitting excited from antiferromagnetic MnO, MnF2 and KMnF3. We apply the many-body scattering theory developed by Hedin in order to incorpo...

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Bibliographic Details
Published inJournal of electron spectroscopy and related phenomena Vol. 257; p. 147202
Main Authors Fujikawa, T., Niki, K., Kogo, J.
Format Journal Article
LanguageEnglish
Published Elsevier B.V 01.05.2022
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ISSN0368-2048
1873-2526
DOI10.1016/j.elspec.2022.147202

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Summary:We discuss two important subjects pioneered by Fadley. As the first topic, we discuss the energy dependence of the intensity ratio observed in Mn 3s multiplet splitting excited from antiferromagnetic MnO, MnF2 and KMnF3. We apply the many-body scattering theory developed by Hedin in order to incorporate the extrinsic effects. We find that the extrinsic effects play an important role to explain the energy dependence of the branching ratio. Preliminary calculations show the smaller energy dependence than that observed. As the second topic we briefly discuss some features in multi-atom resonant photoemission (MARPE) based on the first principle quantum theory. Importance of the local symmetry around an emitter is stressed. •We discuss two important subjects pioneered by Fadley.•As the first topic, we discuss the energy dependence ofthe intensity ratio observed in Mn 3s multiplet splitting excited from antiferromagnetic MnO, MnF2 and KMnF3.•We apply the many-body scattering theory developed by Hedin in order to incorporate the extrinsic effects.
ISSN:0368-2048
1873-2526
DOI:10.1016/j.elspec.2022.147202