亜硝酸ガスの測定，異相化学および健康影響の研究
大気環境学会賞ではこれまでに行ってきた研究である、大気汚染物質の新規な測定法の開発や測定、大気中で起こっているであろう反応の研究、さらに水滴の凍結や乾燥過程での反応、亜硝酸の人体影響、バイオディーゼル燃料の製造と燃焼排ガスの測定や大気環境への影響など、大気環境にかかわる多岐に渡る研究が対象であった。これらをすべてを紹介するのは紙面の関係で無理であるので、ここでは、受賞の元となった業績の中でも大きな比率を占める大気中の亜硝酸ガス (HONO) が関わる研究で1) 大気中の異相の化学、2) ガス状HONOの測定、3) HONOの人体影響について述べる。...
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| Published in | 大気環境学会誌 Vol. 54; no. 1; pp. 1 - 8 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | Japanese |
| Published |
公益社団法人 大気環境学会
10.01.2019
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 1341-4178 2185-4335 |
| DOI | 10.11298/taiki.54.1 |
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| Abstract | 大気環境学会賞ではこれまでに行ってきた研究である、大気汚染物質の新規な測定法の開発や測定、大気中で起こっているであろう反応の研究、さらに水滴の凍結や乾燥過程での反応、亜硝酸の人体影響、バイオディーゼル燃料の製造と燃焼排ガスの測定や大気環境への影響など、大気環境にかかわる多岐に渡る研究が対象であった。これらをすべてを紹介するのは紙面の関係で無理であるので、ここでは、受賞の元となった業績の中でも大きな比率を占める大気中の亜硝酸ガス (HONO) が関わる研究で1) 大気中の異相の化学、2) ガス状HONOの測定、3) HONOの人体影響について述べる。 |
|---|---|
| AbstractList | 大気環境学会賞ではこれまでに行ってきた研究である、大気汚染物質の新規な測定法の開発や測定、大気中で起こっているであろう反応の研究、さらに水滴の凍結や乾燥過程での反応、亜硝酸の人体影響、バイオディーゼル燃料の製造と燃焼排ガスの測定や大気環境への影響など、大気環境にかかわる多岐に渡る研究が対象であった。これらをすべてを紹介するのは紙面の関係で無理であるので、ここでは、受賞の元となった業績の中でも大きな比率を占める大気中の亜硝酸ガス (HONO) が関わる研究で1) 大気中の異相の化学、2) ガス状HONOの測定、3) HONOの人体影響について述べる。 |
| Author | 竹中, 規訓 |
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| Copyright | 2019 大気環境学会 |
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| DOI | 10.11298/taiki.54.1 |
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| References | Perrino, C., De Santis, F., Febo, A.: Criteria for the choice of a denuder sampling technique devoted to the measurement of atmospheric nitrous and nitric acids. Atmos. Environ., 24A, 617–626 (1990). O'Driscoll, P., Lang, K., Minogue, N., Sodeau, J.: Freezing halide ion solutions and the release of interhalogens to the atmosphere, J. Phys. Chem., 110, 4615–4618 (2006). Ohyama, M., Horie, I., Isohama, Y., Azuma, K., Adachi, S., Minejima, C., Takenaka, N.: Effects of nitrous acid exposure on baseline pulmonary resistance and Muc5ac in rats, Inhal. Toxicol. Jun. 4 on line published, 1–10 (2018). Gross, G. W., Wu, C., Bryant, L., McKee, C.: Concentration dependent solute redistribution at the ice/water phase boundary. II. Experimental investigation, J. Chem. Phys., 62, 3085–3092 (1975). Heland, J., Kleffmann, J., Kurtenbach R., Wiesen, P.: A New Instrument To Measure Gaseous Nitrous Acid (HONO) in the Atmosphere, Environ. Sci. Technol., 35, 3207–3212 (2001). 国立天文台：理科年表オフィシャルサイト，https://www.rikanenpyo.jp/kaisetsu/kisyo/kisyo_009.html （2018.11.2アクセス） Lund, D. B., Fennema, O., Powrie, W. D.: Enzymic and acid hydrolysis of sucrose as influenced by freezing, J. Food Sci., 34, 378–382 (1969). Ohyama, M., Nakajima, T., Minejima, C., Azuma, K., Oka, K., Itano, Y., Shouitiro, S., Takenaka, N.: Association between indoor nitrous acid, outdoor nitrogen dioxide, and asthma attacks: Results of a pilot study. Int. J. Environ. Health Res., Accepted for pubnlication. Doi. Org/10.1080/09603123.2018.1559924 Hatley, R. H. M., Frank, F., Day, H., Byth, B.: Subzero-temperature preservation of reactive fluids in the undercooled state. 1. The reduction of potassium ferricyanide by potassium cyanide, Biophys. Chem., 24, 41–46 (1986). Takenaka, N., Bandow, H.: Chemical kinetics of reactions in the unfrozen solution of ice, J. Phys. Chem. A, 111, 8780–8786 (2007). Ferm, M., Sjödin, Å.: A sodium carbonate coated denuder for determination of nitrous acid in the atmosphere, Atmos. Environ., 19, 979–983 (1985). 中島泰知，楠本繁子：NO2短期連続暴露のマウス肺・還元型グルタチオン量におよぼす影響，大阪府立公衆衛生研究所所報，労働衛生編6号 (1968). Arakaki, T., Shibata, M., Miyake, T., Hirakawa, T., Sakugawa, H.: Enhanced formation of formate by freezing in solutions of hydrated formaldehyde-metal-hydrogen peroxide, Geochem. J., 38, 383–388 (2004). Abel, E. H., Schmid, H., Schafranik, J.: Kinetik der Stickstoffentwicklung ans Ammoniumnitrit, Z. Phys. Chem., 1931A, 510–522 (1931). Trinh, H. T., Imanishi, K., Morikawa, T., Hagino, H., Takenaka, N.: Gaseous Nitrous Acid (HONO) and Nitrogen Oxides (NOx) Emission from gasoline and diesel vehicles under real-world driving test cycles, Air Waste Manag. Assoc., 67, 412–420 (2017). Takenaka, N., Takayama, K., Ojiro, N., Shimazaki, W., Ohira, K., Soda, H., Suzue, T., Sadanaga, Y., Bandow, H., Maeda, Y.: The chemistry of drying an aqueous solution of salts, J. Phys. Chem. A, 113, 12233–12242 (2009). Platt, U., Perner, D., Harris, G. W., Winer A. M., Pitts, Jr. J. N.: Observations of nitrous acid in an urban atmosphere by differential optical absorption, Nature, 285, 312–314 (1980). Takenaka, N., Tanaka, M., Okitsu, K., Bandow, H.: Rise in the pH of an unfrozen solution in ice due to the presence of NaCl and promotion of decomposition of gallic acids owing to a change in the pH, J. Phys. Chem. A, 110, 10628–10632 (2006). Sato, K., Furuya, S., Takenaka, N., Bandow, H., Maeda, Y., Furukawa, Y.: Oxidative reaction of thiosulfate with hydrogen peroxide by freezing, Bull. Chem. Soc. Jpn., 76, 1139–1144 (2003). Grant, N. H., Clark, D. E., Alburn, H. E.: Imidazole- and base-catalyzed hydrolysis of penicillin in frozen systems, J. Am. Chem. Soc., 83, 4476–4477 (1961). Takenaka, N., Ueda, A., Maeda, Y.: Acceleration of oxidation-reduction reactions in freezing solution, Proc. NIPR Symp. Polar Meterol. Glacial., 7, 24–32 (1993). Takenaka, N., Ueda, A., Maeda, Y.: Acceleration of the rate of nitrite oxidation by freezing in aqueous-solution, Nature, 358, 736–738 (1992). Wentworth, G. R., Murphy, J. G., Benedict, K. B., Bangs, E. J., Collett Jr., J. L.: The role of dew as a night-time reservoir and morning source for atmospheric ammonia, Atmos. Chem. Phys., 16, 7435–7449 (2016). 林 健太郎，野口 泉：濃度勾配が示す草地からの亜硝酸ガスの間接発生，大気環境学会誌，41, 279–287 (2006). 栗田恵子，青木一幸：連続濃縮器の開発と大気中の硝酸ガスおよび塩化水素の測定，第35回大気汚染学会講演要旨集，p. 552 (1994). Takenaka, N., Terada, H., Oro, Y., Hiroi, M., Yoshikawa, H., Okitsu, K., Bandow, H.: A new method for the measurement of trace amounts of HONO in the atmosphere using an air-dragged aqua-membrane-type denuder and fluorescence detection, Analyst, 129, 1130–1136 (2004). Takenaka, N., Furuya, S., Sato, K., Bandow, H., Maeda, Y., Furukawa, Y.: Rapid reaction of sulfide with hydrogen peroxide and formation of different final products by freezing compared to those in solution, Int. J. Chem. Kinet., 35, 198–205 (2003). Brown, W. D., Dolov, A.: Effect of freezing on autoxidation of oxymyoglobin solutions, J. Food Sci., 28, 211 (1963). Grant N. H., Alburn, H. E.: Transfer reactions in ice. Inhibition of nonenzymatic hydroxylaminolysis of amino acid esters by structural analogs, Biochemistry, 4, 1913–1916 (1965). |
| References_xml | – reference: 林 健太郎，野口 泉：濃度勾配が示す草地からの亜硝酸ガスの間接発生，大気環境学会誌，41, 279–287 (2006). – reference: Grant N. H., Alburn, H. E.: Transfer reactions in ice. Inhibition of nonenzymatic hydroxylaminolysis of amino acid esters by structural analogs, Biochemistry, 4, 1913–1916 (1965). – reference: Platt, U., Perner, D., Harris, G. W., Winer A. M., Pitts, Jr. J. N.: Observations of nitrous acid in an urban atmosphere by differential optical absorption, Nature, 285, 312–314 (1980). – reference: Arakaki, T., Shibata, M., Miyake, T., Hirakawa, T., Sakugawa, H.: Enhanced formation of formate by freezing in solutions of hydrated formaldehyde-metal-hydrogen peroxide, Geochem. J., 38, 383–388 (2004). – reference: Brown, W. D., Dolov, A.: Effect of freezing on autoxidation of oxymyoglobin solutions, J. Food Sci., 28, 211 (1963). – reference: Hatley, R. H. M., Frank, F., Day, H., Byth, B.: Subzero-temperature preservation of reactive fluids in the undercooled state. 1. The reduction of potassium ferricyanide by potassium cyanide, Biophys. Chem., 24, 41–46 (1986). – reference: Grant, N. H., Clark, D. E., Alburn, H. E.: Imidazole- and base-catalyzed hydrolysis of penicillin in frozen systems, J. Am. Chem. Soc., 83, 4476–4477 (1961). – reference: Takenaka, N., Ueda, A., Maeda, Y.: Acceleration of the rate of nitrite oxidation by freezing in aqueous-solution, Nature, 358, 736–738 (1992). – reference: O'Driscoll, P., Lang, K., Minogue, N., Sodeau, J.: Freezing halide ion solutions and the release of interhalogens to the atmosphere, J. Phys. Chem., 110, 4615–4618 (2006). – reference: Takenaka, N., Takayama, K., Ojiro, N., Shimazaki, W., Ohira, K., Soda, H., Suzue, T., Sadanaga, Y., Bandow, H., Maeda, Y.: The chemistry of drying an aqueous solution of salts, J. Phys. Chem. A, 113, 12233–12242 (2009). – reference: Ohyama, M., Horie, I., Isohama, Y., Azuma, K., Adachi, S., Minejima, C., Takenaka, N.: Effects of nitrous acid exposure on baseline pulmonary resistance and Muc5ac in rats, Inhal. Toxicol. Jun. 4 on line published, 1–10 (2018). – reference: Takenaka, N., Tanaka, M., Okitsu, K., Bandow, H.: Rise in the pH of an unfrozen solution in ice due to the presence of NaCl and promotion of decomposition of gallic acids owing to a change in the pH, J. Phys. Chem. A, 110, 10628–10632 (2006). – reference: Wentworth, G. R., Murphy, J. G., Benedict, K. B., Bangs, E. J., Collett Jr., J. L.: The role of dew as a night-time reservoir and morning source for atmospheric ammonia, Atmos. Chem. Phys., 16, 7435–7449 (2016). – reference: Heland, J., Kleffmann, J., Kurtenbach R., Wiesen, P.: A New Instrument To Measure Gaseous Nitrous Acid (HONO) in the Atmosphere, Environ. Sci. Technol., 35, 3207–3212 (2001). – reference: 国立天文台：理科年表オフィシャルサイト，https://www.rikanenpyo.jp/kaisetsu/kisyo/kisyo_009.html （2018.11.2アクセス） – reference: 栗田恵子，青木一幸：連続濃縮器の開発と大気中の硝酸ガスおよび塩化水素の測定，第35回大気汚染学会講演要旨集，p. 552 (1994). – reference: Takenaka, N., Terada, H., Oro, Y., Hiroi, M., Yoshikawa, H., Okitsu, K., Bandow, H.: A new method for the measurement of trace amounts of HONO in the atmosphere using an air-dragged aqua-membrane-type denuder and fluorescence detection, Analyst, 129, 1130–1136 (2004). – reference: Ferm, M., Sjödin, Å.: A sodium carbonate coated denuder for determination of nitrous acid in the atmosphere, Atmos. Environ., 19, 979–983 (1985). – reference: Takenaka, N., Ueda, A., Maeda, Y.: Acceleration of oxidation-reduction reactions in freezing solution, Proc. NIPR Symp. Polar Meterol. Glacial., 7, 24–32 (1993). – reference: Ohyama, M., Nakajima, T., Minejima, C., Azuma, K., Oka, K., Itano, Y., Shouitiro, S., Takenaka, N.: Association between indoor nitrous acid, outdoor nitrogen dioxide, and asthma attacks: Results of a pilot study. Int. J. Environ. Health Res., Accepted for pubnlication. Doi. Org/10.1080/09603123.2018.1559924 – reference: Takenaka, N., Furuya, S., Sato, K., Bandow, H., Maeda, Y., Furukawa, Y.: Rapid reaction of sulfide with hydrogen peroxide and formation of different final products by freezing compared to those in solution, Int. J. Chem. Kinet., 35, 198–205 (2003). – reference: Abel, E. H., Schmid, H., Schafranik, J.: Kinetik der Stickstoffentwicklung ans Ammoniumnitrit, Z. Phys. Chem., 1931A, 510–522 (1931). – reference: Lund, D. B., Fennema, O., Powrie, W. D.: Enzymic and acid hydrolysis of sucrose as influenced by freezing, J. Food Sci., 34, 378–382 (1969). – reference: Takenaka, N., Bandow, H.: Chemical kinetics of reactions in the unfrozen solution of ice, J. Phys. Chem. A, 111, 8780–8786 (2007). – reference: 中島泰知，楠本繁子：NO2短期連続暴露のマウス肺・還元型グルタチオン量におよぼす影響，大阪府立公衆衛生研究所所報，労働衛生編6号 (1968). – reference: Sato, K., Furuya, S., Takenaka, N., Bandow, H., Maeda, Y., Furukawa, Y.: Oxidative reaction of thiosulfate with hydrogen peroxide by freezing, Bull. Chem. Soc. Jpn., 76, 1139–1144 (2003). – reference: Perrino, C., De Santis, F., Febo, A.: Criteria for the choice of a denuder sampling technique devoted to the measurement of atmospheric nitrous and nitric acids. Atmos. Environ., 24A, 617–626 (1990). – reference: Trinh, H. T., Imanishi, K., Morikawa, T., Hagino, H., Takenaka, N.: Gaseous Nitrous Acid (HONO) and Nitrogen Oxides (NOx) Emission from gasoline and diesel vehicles under real-world driving test cycles, Air Waste Manag. Assoc., 67, 412–420 (2017). – reference: Gross, G. W., Wu, C., Bryant, L., McKee, C.: Concentration dependent solute redistribution at the ice/water phase boundary. II. Experimental investigation, J. Chem. Phys., 62, 3085–3092 (1975). |
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