Coupling and Reforming of Methane with Carbon Dioxide in a Pulsed Plasma

Coupling and reforming of methane with carbon dioxide were studied at room temperature and 773 K in a pulsed plasma. Methane and carbon dioxide could be converted mainly to ethylene, carbon monoxide, and hydrogen at room temperature. At 773K, the main product was ethane at a low pulse frequency and...

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Published inKAGAKU KOGAKU RONBUNSHU Vol. 26; no. 5; pp. 731 - 733
Main Authors OUYANG, FENG, YAO, SHUILIANG, SUZUKI, EIJI, NAKAYAMA, AKIRA, MIZUNO, AKIRA, OKUMOTO, MAMORU
Format Journal Article
LanguageJapanese
Published The Society of Chemical Engineers, Japan 10.09.2000
Subjects
carbon dioxide
ethylene production
methane coupling
methane reforming
Online AccessGet full text
ISSN0386-216X
1349-9203
DOI10.1252/kakoronbunshu.26.731

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Abstract Coupling and reforming of methane with carbon dioxide were studied at room temperature and 773 K in a pulsed plasma. Methane and carbon dioxide could be converted mainly to ethylene, carbon monoxide, and hydrogen at room temperature. At 773K, the main product was ethane at a low pulse frequency and ethylene at a high pulse frequency. The energy efficiency can be significantly improved by using a high pulse frequency and high temperature.
AbstractList Coupling and reforming of methane with carbon dioxide were studied at room temperature and 773 K in a pulsed plasma. Methane and carbon dioxide could be converted mainly to ethylene, carbon monoxide, and hydrogen at room temperature. At 773K, the main product was ethane at a low pulse frequency and ethylene at a high pulse frequency. The energy efficiency can be significantly improved by using a high pulse frequency and high temperature.
Author SUZUKI, EIJI
OKUMOTO, MAMORU
OUYANG, FENG
NAKAYAMA, AKIRA
YAO, SHUILIANG
MIZUNO, AKIRA
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  fullname: MIZUNO, AKIRA
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  fullname: OKUMOTO, MAMORU
  organization: Department of Ecological Engineering, Toyohashi University of Technology
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References Suib, S.L. and R.P. Zerger; “A Direct, Continuous, Low-Power Catalytic Conversion of Methane to Higher Hydrocarbons via Microwave Plasmas, ” J. Catal., 139, 383-391 (1993)
Yao, S.L., F. Ouyang, A. Nakayama, E. Suzuki, M. Okumoto and A. Mizuno; “Influences of Frequency on Methane Selective Oxidation in a Pulsed Plasma, ” J. Inst. Electrostat Jpn., 24, 163-64 (2000)
Liu, C., A. Marafee, R. Mallison and L. Lobban; “Methane Conversion to Higher Hydrocarbons in a Corona Discharge over Metal Oxide Catalysts with OH Groups, ” Appl. Catal. A, 164, 21-23 (1997)
Shepelev, S.S., H.D. Gesser, and N.R. Hunter; “Light Paraffin Oxidative Conversion in a Silent Electric Discharge, ” Plasma Chem. Plasma Proc., 13, 479-488 (1993)
Baulch, D.L., C.J. Cobos, R.A. Cox, P. Frank, G. Hayman, TH. Just, J.A. Kerr, T. Murrells, M.J. Pilling, J. Troe, R.W. Walker, and J. Warnatz; “Summary Table of Evaluated Kinetic Data for Combustion Modeling: Supplement 1, ” Combust. Flame, 98, 59-79 (1994)
Tominaga, H. and K. Yoshida; New Technology of Methanol Production, p.36, Science Forum, Tokyo, Japan (1987)
References_xml – reference: Tominaga, H. and K. Yoshida; New Technology of Methanol Production, p.36, Science Forum, Tokyo, Japan (1987)
– reference: Shepelev, S.S., H.D. Gesser, and N.R. Hunter; “Light Paraffin Oxidative Conversion in a Silent Electric Discharge, ” Plasma Chem. Plasma Proc., 13, 479-488 (1993)
– reference: Liu, C., A. Marafee, R. Mallison and L. Lobban; “Methane Conversion to Higher Hydrocarbons in a Corona Discharge over Metal Oxide Catalysts with OH Groups, ” Appl. Catal. A, 164, 21-23 (1997)
– reference: Suib, S.L. and R.P. Zerger; “A Direct, Continuous, Low-Power Catalytic Conversion of Methane to Higher Hydrocarbons via Microwave Plasmas, ” J. Catal., 139, 383-391 (1993)
– reference: Yao, S.L., F. Ouyang, A. Nakayama, E. Suzuki, M. Okumoto and A. Mizuno; “Influences of Frequency on Methane Selective Oxidation in a Pulsed Plasma, ” J. Inst. Electrostat Jpn., 24, 163-64 (2000)
– reference: Baulch, D.L., C.J. Cobos, R.A. Cox, P. Frank, G. Hayman, TH. Just, J.A. Kerr, T. Murrells, M.J. Pilling, J. Troe, R.W. Walker, and J. Warnatz; “Summary Table of Evaluated Kinetic Data for Combustion Modeling: Supplement 1, ” Combust. Flame, 98, 59-79 (1994)
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Snippet Coupling and reforming of methane with carbon dioxide were studied at room temperature and 773 K in a pulsed plasma. Methane and carbon dioxide could be...
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SubjectTerms carbon dioxide
ethylene production
methane coupling
methane reforming
Title Coupling and Reforming of Methane with Carbon Dioxide in a Pulsed Plasma
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