京都市に流通する食品中の放射性物質の実態調査(1991~2011年) 福島第一原子力発電所事故前後の比較

チェルノブイリ原子力発電所事故以後,京都市内に流通する食品中の放射性ヨウ素(131I)および放射性セシウム(137Csおよび134Cs)のモニタリングを実施してきたが,2011年3月の福島原子力発電所の事故は,調査の重要性を改めて認識させることとなった.福島原子力発電所事故前後において検出した核種と検出率,および濃度について検討した.検査にはゲルマニウム半導体検出器を用いた.福島原発事故以前は,輸入品,国産品をモニタリングの対象とした.核種としては137Csのみが検出された.魚介類からの検出頻度は約70%であり,濃度は最高でも1.7 Bq/kgであった.乾燥キノコを除くキノコ類からの検出頻度は...

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Published in食品衛生学雑誌 Vol. 54; no. 3; pp. 178 - 187
Main Authors 伴, 創一郎, 石川, 和弘, 土井, 直也, 川上, 雅弘, 瀬村, 俊亮, 三宅, 司郎, 並河, 幹夫, 折戸, 太一, 伴埜, 行則, 三輪, 真理子
Format Journal Article
LanguageJapanese
Published 公益社団法人 日本食品衛生学会 25.06.2013
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ISSN0015-6426
1882-1006
DOI10.3358/shokueishi.54.178

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Abstract チェルノブイリ原子力発電所事故以後,京都市内に流通する食品中の放射性ヨウ素(131I)および放射性セシウム(137Csおよび134Cs)のモニタリングを実施してきたが,2011年3月の福島原子力発電所の事故は,調査の重要性を改めて認識させることとなった.福島原子力発電所事故前後において検出した核種と検出率,および濃度について検討した.検査にはゲルマニウム半導体検出器を用いた.福島原発事故以前は,輸入品,国産品をモニタリングの対象とした.核種としては137Csのみが検出された.魚介類からの検出頻度は約70%であり,濃度は最高でも1.7 Bq/kgであった.乾燥キノコを除くキノコ類からの検出頻度は,83%と高く,濃度の最高値は7.5 Bq/kgであった.野菜類は,207検体のうち2件のみ(根菜を除く)で検出したが濃度も明らかに低かった.福島原発事故以降は,東北・関東地方産の流通食品を検査した.3月23日に中央卸売市場から採取したミズ菜から3,400 Bq/kgの131I,280 Bq/kgの134Cs,および280 Bq/kgの137Csを検出したのをはじめ,3月と4月に検査したすべての葉菜類でこれらの放射性物質を検出した.しかし,11月以降はすべてが不検出となった.魚介類から検出された137Csは,平均で7.9 Bq/kgだった.肉類では,トレーサビリティーによって汚染稲わらを与えられたことが判明したウシの肉からのみ暫定規制値を超える137Csが検出された.また,甲状腺に対するリスクが懸念される131Iは,5月以降すべての試料で不検出となった.基準値を超える食品が京都市内を流通する恐れは,すでにほとんどないと考えられた.
AbstractList チェルノブイリ原子力発電所事故以後,京都市内に流通する食品中の放射性ヨウ素(131I)および放射性セシウム(137Csおよび134Cs)のモニタリングを実施してきたが,2011年3月の福島原子力発電所の事故は,調査の重要性を改めて認識させることとなった.福島原子力発電所事故前後において検出した核種と検出率,および濃度について検討した.検査にはゲルマニウム半導体検出器を用いた.福島原発事故以前は,輸入品,国産品をモニタリングの対象とした.核種としては137Csのみが検出された.魚介類からの検出頻度は約70%であり,濃度は最高でも1.7 Bq/kgであった.乾燥キノコを除くキノコ類からの検出頻度は,83%と高く,濃度の最高値は7.5 Bq/kgであった.野菜類は,207検体のうち2件のみ(根菜を除く)で検出したが濃度も明らかに低かった.福島原発事故以降は,東北・関東地方産の流通食品を検査した.3月23日に中央卸売市場から採取したミズ菜から3,400 Bq/kgの131I,280 Bq/kgの134Cs,および280 Bq/kgの137Csを検出したのをはじめ,3月と4月に検査したすべての葉菜類でこれらの放射性物質を検出した.しかし,11月以降はすべてが不検出となった.魚介類から検出された137Csは,平均で7.9 Bq/kgだった.肉類では,トレーサビリティーによって汚染稲わらを与えられたことが判明したウシの肉からのみ暫定規制値を超える137Csが検出された.また,甲状腺に対するリスクが懸念される131Iは,5月以降すべての試料で不検出となった.基準値を超える食品が京都市内を流通する恐れは,すでにほとんどないと考えられた.
Author 土井, 直也
伴埜, 行則
伴, 創一郎
石川, 和弘
川上, 雅弘
折戸, 太一
並河, 幹夫
三輪, 真理子
瀬村, 俊亮
三宅, 司郎
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References_xml – reference: 9) Hamada, T., et al. Kagakugijutsucho Houshanou Sokuteihou Shiri-zu 7, Japan Chemical Analysis Center, 1990, 315 p.
– reference: 13) Bannai, T., Yoshida, S., Muramatsu, Y. Cultivation experiments on uptake radionuclides by mushrooms. Radioisotopes, 43, 77–82 (1994).
– reference: 15) Brown, J., Sherwood, J. Modeling Approach for the transfer of Radionuclides to Fruit Species of Importance in the UK. HPA-CRCE (Health Protection Agency—The Centre for Radiation, Chemical and Environmental Hazards)-032, 1–74 (2012).
– reference: 5) Kato, K., Yamazaki, K., Kasahara, M., Kon, N. Tonouchi, S. Studies on the level and distribution of 90Sr and 137Cs concentrations in foodstuffs. Annual Report of Niigata Prefectural Institute of Environmental Radiation Monitoring, 2, 21–30 (2004).
– reference: 6) Bland, M., Loutit, J., Sansom, J. Histochemical phosphatases and metachromasia in murine tumours induced by bone seeking radionuclides. British J. Cancer, 29, 206–222 (1974).
– reference: 7) Iwashima, K., Okubo, T. On the interim radionuclide action level for monitoring imported foods. Shokuhin Eisei Kenkyu (Food Sanitation Research), 37(7), 7–21 (1987).
– reference: 19) Aoyama, M., Tsumune, D., Uematsu, M., Kondo, F., Hamajima Y. Temporal variation of 134Cs and 137Cs activities in surface water at stations along the coastline near the Fukushima Daiichi Nuclear Power Plant accident site, Geochemical Journal, 46, 321–325 (2012).
– reference: 22) Handbook of Parameter Values for the Prediction of Radionuclide Transfer in Terrestrial and Freshwater Environments, IAEA Vienna, 2010, 3. Agricultural Ecosystems: Foliar Uptake.
– reference: 8) Takatani, S. Radioactive Contamination of imported food due to the Chernobyl Nuclear Power Plant accident. Shokuhin Eisei Kenkyu (Food Sanitation Research), 39(10), 15–27 (1989).
– reference: 24) WHO/SDE/PHE/99.6. Guidelines for Iodine: Prophylaxis following Nuclear Accidents, Update 1999. p. 1–39 (1999).
– reference: 16) Sanches, N., Anjos, R. M., Mosquera, B. 40K/137Cs discrimination ratios to the aboveground organs of tropical plants. Journal of Environmental Radioactivity, 99, 1127–1135 (2008).
– reference: 18) Aarkrog, A., Dahlgaard, H., Hallstadius, L., Hansen, H., Holm, E. Radiocaesium from sellafield effluents in Greenland water. Nature 304(5921), 49–51 (1983).
– reference: 28) Tian, Y., Akamine, T., Suda, M. Long-term Variability in the Abundance of Pacific Saury in the Northwestern Pacific Ocean and Climate Changes during the Last Century. Bulletin of the Japanese Society of Fisheries Oceanography (ISSN: 0916–1562) 66(1), 16–25 (2002).
– reference: 2) Komamura, M., Tsumura, A., Yamaguchi, N., Fujiwara, H., Kihou, N., Kodaira, K. 1959 Long-term monitoring and analysis of 90Sr and 137Cs concentrations in rice, wheat and soils in Japan from to 2000. Bulletin of National Institute for Agro-Environmental Sciences (ISSN 0911–9450), 24, 1–21 (2006).
– reference: 1) Völkle, H. 50 years of radiation protection and nuclear power in Switzerland: A brief history. Atoms for peace. An International Journal, 1(2/3), 239–244 (2006).
– reference: 11) Kasamatu, F. Marine Organisms and Radionuclides Radioisotopes, 48, 266–282 (1999).
– reference: 14) Itou, N. Kunugiyama. I., Kiguchi S., Kubo M., Kameta M., Furukawa Y. Transfer coefficients of 137Cs via the forage-cow-milk pathway in Aomori prefecture of Japan. Radioisotopes, 43, 695–699 (1994).
– reference: 10) J. A. Cooper. Factors determining the ultimate detection sensitivity of Ge (Li) gamma-ray spectrometers. Nuclear Instruments and Methods, 82, 273–277 (1970).
– reference: 25) United Nations Scientific Committee on the Effects of Atomic Radiation. UNSCEAR 2000 Reptor Vol. II. Sources and Effects of Ionizing Radiation, Annex D, Health effects due to radiation from the Chernobyl accident. and Annex J, Exposures and effects of the Chernobyl accident. (United Nations, New York, 2011).
– reference: 29) Nashida, K., et al. Migration of spotted mackerel Scomber australasicus estimated from a tagging experiment off Ashizuri Cape and around the Izu Islands, central and southern Pacific coast of Japan. Bulletin of Fisheries Research Agency, 17, 1–15 (2006).
– reference: 12) Sugiyama, H., Terada, H., Isomura, K., Tsukada, H., Shibata, H. Radiocesium uptake mechanisms in wild and culture mushrooms. Radioisotopes, 42, 683–690 (1993).
– reference: 23) Cardis, E., Kesminiene, A., Ivanov, V., Malakhova, I., Shibata, Y., Khrouch, V., Drozdovitch, V., Maceika, E., Zvonova, I., Vlassov, O., Bouville,A., Goulko, G., Hoshi, M., Abrosimov, A., Anoshko, J., Astakhova, L., Chekin, S., Demidchik, E., Galanti, R., Ito, M., Korobova, E., Lushnikov, E., Maksioutov, M., Masyakin, V., Nerovnia, A., Parshin, A., Parshkov, E., Piliptsevich, N., Pinchera, A., Polyakov, S., Shabeka, N., Suonio, E., Tenet, V., Tsyb, A., Yamashita, S., Williams, D. Risk of thyroid cancer After Exposure to 131 I in Childhood. Journal of National Cancer Institute, 97, 724–732 (2005).
– reference: 3) Fukuda, K. Fifty years annual review of environmental radioactivity survey in the Hokkaido Institute of Public Health for Years. Report of the Hokkaido Institute of Public Health, 57, 1–14 (2007).
– reference: 17) Povinec, P., Fowler, S., Baxter, M. Chernobyl and the marine environment: The radiological impact in context. International Atomic Energy Agency (IAEA) Bulletin, 1, 18–22 (1996).
– reference: 27) Kasamatsu, F. Marine organisms and radionuclides –with special reference to the factors affecting concentration of 137cs in marine fish—. Radioisotopes, 48, 266–282 (1999).
– reference: 20) Ken Buesseler, Aoyama M., Fukasawa M. Impacts of the Fukushima Nuclear Power Plants on Marine Radioactivity. Environmental Science and Technology, 45, 9931–9935 (2011).
– reference: 21) Geoff Brumfiel. Ocean still suffering from Fukushima fallout. Nature, doi: 10. 1038/nature.2012.11823
– reference: 4) Shimizu, M., Michihiro, K., Miyazaki, K., Nobumori, T. Investigation of environmental radioactivity affected by radioactive fallout in Okayama for the past 30 years. Annual Report of Okayama Prefectural Institute for Environmental Science and Public Health, 30, 75–83 (2006).
– reference: 26) Yamaguchi, N., et al. Behavior of radiocaesium in soil-plant systems and its controlling factor. Bulletin of National Institute of Agro-Environmental Science, 31, 75–129, (2012).
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Snippet チェルノブイリ原子力発電所事故以後,京都市内に流通する食品中の放射性ヨウ素(131I)および放射性セシウム(137Csおよび134Cs)のモニタリングを実施してきたが,2011...
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SubjectTerms チェルノブイリ原子力発電所事故
放射性セシウム
放射性ヨウ素
福島第一原子力発電所事故
食品中の放射性物質
Subtitle 福島第一原子力発電所事故前後の比較
Title 京都市に流通する食品中の放射性物質の実態調査(1991~2011年)
URI https://www.jstage.jst.go.jp/article/shokueishi/54/3/54_178/_article/-char/ja
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