Monolayer MoS2 Films Supported by 3D Nanoporous Metals for High-Efficiency Electrocatalytic Hydrogen Production
The “edge‐free” monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out‐of‐plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bendin...
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| Published in | Advanced materials (Weinheim) Vol. 26; no. 47; pp. 8023 - 8028 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Blackwell Publishing Ltd
17.12.2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0935-9648 1521-4095 1521-4095 |
| DOI | 10.1002/adma.201403808 |
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| Abstract | The “edge‐free” monolayer MoS2
films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out‐of‐plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor‐to‐metal transition of 2H MoS2 and the formation of catalytically active sites for HER. |
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| AbstractList | The "edge-free" monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out-of-plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor-to-metal transition of 2H MoS2 and the formation of catalytically active sites for HER.The "edge-free" monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out-of-plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor-to-metal transition of 2H MoS2 and the formation of catalytically active sites for HER. The “edge‐free” monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out‐of‐plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor‐to‐metal transition of 2H MoS2 and the formation of catalytically active sites for HER. The "edge-free" monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from large out-of-plane strains that are geometrically required to manage the 3D curvature of bicontinuous nanoporosity. The large lattice bending leads to local semiconductor-to-metal transition of 2H MoS2 and the formation of catalytically active sites for HER. |
| Author | Tan, Yongwen Chen, Luyang Cong, Weitao Han, Jiuhui Fujita, Takeshi Hirata, Akihiko Tang, Zheng Liu, Pan Ito, Yoshikazu Chen, Mingwei W. Guo, Xianwei |
| Author_xml | – sequence: 1 givenname: Yongwen surname: Tan fullname: Tan, Yongwen organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 2 givenname: Pan surname: Liu fullname: Liu, Pan organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 3 givenname: Luyang surname: Chen fullname: Chen, Luyang organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 4 givenname: Weitao surname: Cong fullname: Cong, Weitao organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 5 givenname: Yoshikazu surname: Ito fullname: Ito, Yoshikazu organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 6 givenname: Jiuhui surname: Han fullname: Han, Jiuhui organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 7 givenname: Xianwei surname: Guo fullname: Guo, Xianwei organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 8 givenname: Zheng surname: Tang fullname: Tang, Zheng organization: Key Laboratory of Polar Materials and Devices, East China Normal University, 200062, Shanghai, P.R. China – sequence: 9 givenname: Takeshi surname: Fujita fullname: Fujita, Takeshi organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 10 givenname: Akihiko surname: Hirata fullname: Hirata, Akihiko organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan – sequence: 11 givenname: Mingwei W. surname: Chen fullname: Chen, Mingwei W. email: mwchen@wpi-aimr.tohoku.ac.jp organization: WPI Advanced Institute for Materials Research, Tohoku University, 980-8577, Sendai, Japan |
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| Keywords | nanoporous metal monolayer dichalcogenide molybdenum disulphide 2D materials hydrogen evolution reaction |
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| Snippet | The “edge‐free” monolayer MoS2
films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from... The "edge-free" monolayer MoS2 films supported by 3D nanoporous gold show high catalytic activities towards hydrogen evolution reaction (HER), originating from... |
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| SubjectTerms | 2D materials hydrogen evolution reaction molybdenum disulphide monolayer dichalcogenide nanoporous metal |
| Title | Monolayer MoS2 Films Supported by 3D Nanoporous Metals for High-Efficiency Electrocatalytic Hydrogen Production |
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