Advanced treatment of biologically pretreated coking wastewater by electrochemical oxidation using Ti/RuO2-IrO2 electrodes
Background Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This work investigated the feasibility of electrochemical treatment using a Ti/RuO2–IrO2 anode as an advanced treatment of coking wastewater. The...
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| Published in | Journal of chemical technology and biotechnology (1986) Vol. 88; no. 8; pp. 1568 - 1575 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Chichester, UK
John Wiley & Sons, Ltd
01.08.2013
Wiley Wiley Subscription Services, Inc |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0268-2575 1097-4660 |
| DOI | 10.1002/jctb.4006 |
Cover
| Abstract | Background
Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This work investigated the feasibility of electrochemical treatment using a Ti/RuO2–IrO2 anode as an advanced treatment of coking wastewater. The influential operating factors including current density (9.6–108.2 mA cm−2) and electrode gap (0.5–2.5 cm) were evaluated.
Results
The current density and electrodes gap had significant effects on COD and NH4+‐N removal and the energy consumption. The degradation of COD and NH4+‐N followed pseudo‐first‐order kinetics. In most experiments, high levels of NH4+‐N removal (NH4+‐N removal ratio > 95%) was achieved along with moderate mineralization (COD removal ratio: 60–80%). COD (178.0–285.0 mg L‐1) and NH4+‐N (55.0–76.0 mg L‐1) were degraded by 62% and 96%, respectively, at the optimum conditions (electrode gap: 0.5 cm, current density: 15.6 mA cm−2) after 60 min treatment. Under this optimal condition, the corresponding energy consumption was 8.60 kWh m‐3 for effluent meeting the discharge standards. Furthermore, gas chromatography–mass spectrometry (GC‐MS) analysis indicated that this technique could be employed to eliminate bio‐refractory and toxic compounds such as phenanthrene, indole, quinoline and pyrimidine in coking wastewater.
Conclusion
Ti/RuO2–IrO2 anode systems were confirmed to be effective in advanced treatment of biologically pretreated coking wastewater. © 2012 Society of Chemical Industry |
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| AbstractList | Background Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This work investigated the feasibility of electrochemical treatment using a Ti/RuO2-IrO2 anode as an advanced treatment of coking wastewater. The influential operating factors including current density (9.6-108.2mAcm-2) and electrode gap (0.5-2.5cm) were evaluated. Results The current density and electrodes gap had significant effects on COD and NH4+-N removal and the energy consumption. The degradation of COD and NH4+-N followed pseudo-first-order kinetics. In most experiments, high levels of NH4+-N removal (NH4+-N removal ratio>95%) was achieved along with moderate mineralization (COD removal ratio: 60-80%). COD (178.0-285.0mgL-1) and NH4+-N (55.0-76.0mgL-1) were degraded by 62% and 96%, respectively, at the optimum conditions (electrode gap: 0.5cm, current density: 15.6mAcm-2) after 60min treatment. Under this optimal condition, the corresponding energy consumption was 8.60 kWh m-3 for effluent meeting the discharge standards. Furthermore, gas chromatography-mass spectrometry (GC-MS) analysis indicated that this technique could be employed to eliminate bio-refractory and toxic compounds such as phenanthrene, indole, quinoline and pyrimidine in coking wastewater. Conclusion Ti/RuO2-IrO2 anode systems were confirmed to be effective in advanced treatment of biologically pretreated coking wastewater. © 2012 Society of Chemical Industry Background Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This work investigated the feasibility of electrochemical treatment using a Ti/RuO2–IrO2 anode as an advanced treatment of coking wastewater. The influential operating factors including current density (9.6–108.2 mA cm−2) and electrode gap (0.5–2.5 cm) were evaluated. Results The current density and electrodes gap had significant effects on COD and NH4+‐N removal and the energy consumption. The degradation of COD and NH4+‐N followed pseudo‐first‐order kinetics. In most experiments, high levels of NH4+‐N removal (NH4+‐N removal ratio > 95%) was achieved along with moderate mineralization (COD removal ratio: 60–80%). COD (178.0–285.0 mg L‐1) and NH4+‐N (55.0–76.0 mg L‐1) were degraded by 62% and 96%, respectively, at the optimum conditions (electrode gap: 0.5 cm, current density: 15.6 mA cm−2) after 60 min treatment. Under this optimal condition, the corresponding energy consumption was 8.60 kWh m‐3 for effluent meeting the discharge standards. Furthermore, gas chromatography–mass spectrometry (GC‐MS) analysis indicated that this technique could be employed to eliminate bio‐refractory and toxic compounds such as phenanthrene, indole, quinoline and pyrimidine in coking wastewater. Conclusion Ti/RuO2–IrO2 anode systems were confirmed to be effective in advanced treatment of biologically pretreated coking wastewater. © 2012 Society of Chemical Industry |
| Author | He, Xuwen Chai, Zhen Li, Fuping Zhang, Chunhui Li, Dong Li, Jing Hu, Jianlong |
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| Keywords | Energy consumption Phenanthrene coking wastewater Electrochemical treatment Ti/RuO IrO Density N Waste water Electrodes Refractory Gas chromatography electrochemical oxidation Chemical oxygen demand Mineralization First order Oxidation Kinetics COD and NH Waste water purification Electrochemical reaction Mass spectrometry |
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| References_xml | – reference: Abdelwahab O, Amin NK and El-Ashtoukhy E-SZ, Electrochemical removal of phenol from oil refinery wastewater. J Hazard Mater 163(2-3):711-716 (2009). – reference: Li XY, Cui YH, Feng YJ, Xie ZM and Gu JD, Reaction pathways and mechanisms of the electrochemical degradation of phenol on different electrodes. Water Res 39(10):1972-1981 (2005). – reference: Zeng Y, Chen KN, Wu W, Wang JR and Lee S, Effect of IrO2 loading on RuO2-IrO2-TiO2 anodes: a study of microstructure and working life for the chlorine evolution reaction. Ceram Int 33(6):1087-1091 (2007). – reference: Lei XH, Li M, Zhang ZY, Feng CP, Bai W and Sugiura N, Electrochemical regeneration of zeolites and the removal of ammonia. J Hazard Mater 169:746-750 (2009). – reference: Wang JL, Quan XC, Wu LB, Qian Y and Hegemann W, Bioaugmentation as a tool to enhance the removal of refractory compound in coke plant wastewater. Process Biochem 38(5):777-781 (2002). – reference: Zanta CLPS, Michaud PA, Comninellis C, De Andrade AR and Boodts JFC, Electrochemical oxidation of p-chlorophenol on SnO2-Sb2O5 based anodes for wastewater treatment. J Appl Electrochem 33:1211-1215 (2003). – reference: Chu LB, Wang JL, Dong J, Liu HY and Sun XL, Treatment of coking wastewater by an advanced Fenton oxidation process using iron powder and hydrogen peroxide. Chemosphere 86:409-414 (2012). – reference: Sutton PM, Hurvid J and Hoeksema M, Biological fluidized-bed treatment of wastewater from byproduct coking operations: full-scale case history. Water Environ Res 71:5-9 (1999). – reference: Zhou MH, Dai QZ, Lei LC, Ma C and Wang DH, Long life modified lead dioxide anode for organic wastewater treatment: electrochemical characteristics and degradation mechanism. 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Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This... Background Electrochemical oxidation has attracted wide attention in wastewater treatment because of its strong oxidation performance and ease of control. This... |
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| SubjectTerms | Applied sciences Chemical engineering Chemical treatment COD and NH4+-N Coke coking wastewater Effluent standards electrochemical oxidation Electrochemistry Electrodes Energy consumption Exact sciences and technology Gas chromatography General purification processes Mass spectrometry Mineralization Oxidation Phenanthrene Pollution Reactors Ti/RuO2-IrO2 electrodes Wastewater treatment Wastewaters Water treatment and pollution |
| Title | Advanced treatment of biologically pretreated coking wastewater by electrochemical oxidation using Ti/RuO2-IrO2 electrodes |
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