Bio-inspired vertebral design for scalable and flexible perovskite solar cells
The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrate...
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| Published in | Nature communications Vol. 11; no. 1; pp. 3016 - 10 |
|---|---|
| Main Authors | , , , , , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
15.06.2020
Nature Publishing Group Nature Portfolio |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2041-1723 2041-1723 |
| DOI | 10.1038/s41467-020-16831-3 |
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| Abstract | The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm
2
and 31.20 cm
2
respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics.
Flexible perovskite solar cells suffer huge efficiency loss upon area scale-up due to brittleness of ITO and poor perovskite film quality. Here Meng et al. solve this by inserting a conductive and glued polymer layer between ITO and perovskite layers and obtain efficiency of 17% for 30 cm
2
devices. |
|---|---|
| AbstractList | The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm
and 31.20 cm
respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics. Flexible perovskite solar cells suffer huge efficiency loss upon area scale-up due to brittleness of ITO and poor perovskite film quality. Here Meng et al. solve this by inserting a conductive and glued polymer layer between ITO and perovskite layers and obtain efficiency of 17% for 30 cm2 devices. The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm 2 and 31.20 cm 2 respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics. Flexible perovskite solar cells suffer huge efficiency loss upon area scale-up due to brittleness of ITO and poor perovskite film quality. Here Meng et al. solve this by inserting a conductive and glued polymer layer between ITO and perovskite layers and obtain efficiency of 17% for 30 cm 2 devices. The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm2 and 31.20 cm2 respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics.Flexible perovskite solar cells suffer huge efficiency loss upon area scale-up due to brittleness of ITO and poor perovskite film quality. Here Meng et al. solve this by inserting a conductive and glued polymer layer between ITO and perovskite layers and obtain efficiency of 17% for 30 cm2 devices. The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm2 and 31.20 cm2 respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics.The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm2 and 31.20 cm2 respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics. The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible perovskite solar cells (PSCs). The degradation is attributed to the brittleness and discrepancy of perovskite crystal growth upon different substrates. Inspired by robust crystallization and flexible structure of vertebrae, herein, we employ a conductive and glued polymer between indium tin oxide and perovskite layers, which simultaneously facilitates oriented crystallization of perovskite and sticks the devices. With the results of experimental characterizations and theoretical simulations, this bionic interface layer accurately controls the crystallization and acts as an adhesive. The flexible PSCs achieve the power conversion efficiencies of 19.87% and 17.55% at effective areas of 1.01 cm 2 and 31.20 cm 2 respectively, retaining over 85% of original efficiency after 7000 narrow bending cycles with negligible angular dependence. Finally, the modules are assembled into a wearable solar-power source, enabling the upscaling of flexible electronics. |
| ArticleNumber | 3016 |
| Author | Hu, Ting Huang, Zengqi Song, Yanlin Zhang, Lin Su, Meng Meng, Xiangchuan Xing, Zhi Huang, Zhandong Cui, Yongjie Chen, Yiwang Hu, Xiaotian Liao, Xunfan Wang, Fuyi Cai, Zheren Zhang, Yanyan |
| Author_xml | – sequence: 1 givenname: Xiangchuan orcidid: 0000-0002-9540-5240 surname: Meng fullname: Meng, Xiangchuan organization: College of Chemistry, Nanchang University, Institute of Polymers and Energy Chemistry, Nanchang University – sequence: 2 givenname: Zheren orcidid: 0000-0003-0232-8213 surname: Cai fullname: Cai, Zheren organization: Key Laboratory of Green Printing, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 3 givenname: Yanyan orcidid: 0000-0002-2048-145X surname: Zhang fullname: Zhang, Yanyan organization: CAS Key Laboratory of Analytical Chemistry for Living Biosystems, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 4 givenname: Xiaotian orcidid: 0000-0001-5483-8800 surname: Hu fullname: Hu, Xiaotian email: xiaotian@iccas.ac.cn organization: College of Chemistry, Nanchang University, Institute of Polymers and Energy Chemistry, Nanchang University – sequence: 5 givenname: Zhi orcidid: 0000-0003-0197-2664 surname: Xing fullname: Xing, Zhi organization: College of Chemistry, Nanchang University – sequence: 6 givenname: Zengqi orcidid: 0000-0001-5435-1744 surname: Huang fullname: Huang, Zengqi organization: College of Chemistry, Nanchang University – sequence: 7 givenname: Zhandong surname: Huang fullname: Huang, Zhandong organization: Key Laboratory of Green Printing, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 8 givenname: Yongjie orcidid: 0000-0003-2202-0697 surname: Cui fullname: Cui, Yongjie organization: College of Materials Science and Engineering, Donghua University – sequence: 9 givenname: Ting orcidid: 0000-0001-5261-9858 surname: Hu fullname: Hu, Ting organization: College of Chemistry, Nanchang University, Institute of Polymers and Energy Chemistry, Nanchang University – sequence: 10 givenname: Meng orcidid: 0000-0001-8485-2590 surname: Su fullname: Su, Meng organization: Key Laboratory of Green Printing, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 11 givenname: Xunfan orcidid: 0000-0002-6649-5865 surname: Liao fullname: Liao, Xunfan organization: College of Materials Science and Engineering, Donghua University, Institute of Advanced Scientific Research (iASR), Jiangxi Normal University – sequence: 12 givenname: Lin orcidid: 0000-0002-8251-2987 surname: Zhang fullname: Zhang, Lin organization: Hunan Key Laboratory of Super Microstructure and Ultrafast Process, School of Physics and Electronics, Central South University – sequence: 13 givenname: Fuyi orcidid: 0000-0003-0962-1260 surname: Wang fullname: Wang, Fuyi organization: CAS Key Laboratory of Analytical Chemistry for Living Biosystems, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 14 givenname: Yanlin surname: Song fullname: Song, Yanlin email: ylsong@iccas.ac.cn organization: Key Laboratory of Green Printing, Institute of Chemistry, Chinese Academy of Sciences (ICCAS) – sequence: 15 givenname: Yiwang orcidid: 0000-0003-4709-7623 surname: Chen fullname: Chen, Yiwang email: ywchen@ncu.edu.cn organization: College of Chemistry, Nanchang University, Institute of Polymers and Energy Chemistry, Nanchang University, Institute of Advanced Scientific Research (iASR), Jiangxi Normal University |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/32541859$$D View this record in MEDLINE/PubMed |
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| ContentType | Journal Article |
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| Copyright_xml | – notice: The Author(s) 2020 – notice: The Author(s) 2020. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License. |
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| DOI | 10.1038/s41467-020-16831-3 |
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| Snippet | The translation of unparalleled efficiency from the lab-scale devices to practical-scale flexible modules affords a huge performance loss for flexible... Flexible perovskite solar cells suffer huge efficiency loss upon area scale-up due to brittleness of ITO and poor perovskite film quality. Here Meng et al.... |
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| Title | Bio-inspired vertebral design for scalable and flexible perovskite solar cells |
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