Synergy between surfactants’ stiffness and concentration on their self-assembly into reverse micelles as water droplet carriers in nonpolar solvents
A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration ( c s ) and the persistence length ( L p ) of the surfactants is presented here. The influence of c s and L p on the structur...
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| Published in | PloS one Vol. 19; no. 2; p. e0294913 |
|---|---|
| Main Authors | , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Public Library of Science
02.02.2024
Public Library of Science (PLoS) |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1932-6203 1932-6203 |
| DOI | 10.1371/journal.pone.0294913 |
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| Abstract | A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration (
c
s
) and the persistence length (
L
p
) of the surfactants is presented here. The influence of
c
s
and
L
p
on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from
c
= 6
wt
% up to
c
= 12
wt
%, for increasing surfactants’ rigidity from
L
p
= 0.73 nm up to
L
p
= 44.99 nm. It is found that there exists a collaborative interplay between
c
s
and
L
p
that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents. |
|---|---|
| AbstractList | A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration (cs) and the persistence length (Lp) of the surfactants is presented here. The influence of cs and Lp on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from c = 6 wt% up to c = 12 wt%, for increasing surfactants' rigidity from Lp = 0.73 nm up to Lp = 44.99 nm. It is found that there exists a collaborative interplay between cs and Lp that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents. A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration ( c s ) and the persistence length ( L p ) of the surfactants is presented here. The influence of c s and L p on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from c = 6 wt % up to c = 12 wt %, for increasing surfactants’ rigidity from L p = 0.73 nm up to L p = 44.99 nm. It is found that there exists a collaborative interplay between c s and L p that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents. A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration (cs) and the persistence length (Lp) of the surfactants is presented here. The influence of cs and Lp on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from c = 6 wt% up to c = 12 wt%, for increasing surfactants' rigidity from Lp = 0.73 nm up to Lp = 44.99 nm. It is found that there exists a collaborative interplay between cs and Lp that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents.A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration (cs) and the persistence length (Lp) of the surfactants is presented here. The influence of cs and Lp on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from c = 6 wt% up to c = 12 wt%, for increasing surfactants' rigidity from Lp = 0.73 nm up to Lp = 44.99 nm. It is found that there exists a collaborative interplay between cs and Lp that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents. A study of the self-assembly process into reverse micelles (RMs) of linear surfactants and monomeric aqueous solutes dissolved in nonpolar solvents, varying the concentration (c.sub.s) and the persistence length (L.sub.p) of the surfactants is presented here. The influence of c.sub.s and L.sub.p on the structural and dynamic properties of the aggregates is investigated through mesoscopic simulations carried out with the dissipative particle dynamics method. All simulations are performed at a fixed water/surfactant molecular ratio of 2:1, varying the surfactant concentration from c = 6 wt% up to c = 12 wt%, for increasing surfactants' rigidity from L.sub.p = 0.73 nm up to L.sub.p = 44.99 nm. It is found that there exists a collaborative interplay between c.sub.s and L.sub.p that enhances the number of RMs assembled and their diffusion as carriers of water droplets. These results should be useful as guidelines to understand and improve processes where the RMs are implemented to carry aqueous solutes in nonpolar solvents. |
| Audience | Academic |
| Author | Gama Goicochea, A. Hernández Velázquez, J.D. |
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| Cites_doi | 10.1021/la303245e 10.1038/46509 10.1021/la9904556 10.1016/j.polymer.2017.09.046 10.1021/la902128g 10.1021/la060386c 10.1126/science.266.5183.254 10.1016/S0006-3495(01)75737-2 10.1007/BF02797115 10.1016/j.colsurfb.2017.12.012 10.3390/polym8070254 10.1021/la001182d |
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| SubjectTerms | Analysis Evaluation Micelles Numerical analysis Properties Surface active agents |
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| Title | Synergy between surfactants’ stiffness and concentration on their self-assembly into reverse micelles as water droplet carriers in nonpolar solvents |
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