表面改性炭材料在微生物燃料电池中的应用
研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱（FTIR）、Boehm滴定法和X射线光电子能谱（谱（XPS）等手段对催化剂进行了表征。 FTIR测试证明硝酸处理可引入含氧基团氨水处理可引入含氮基团。另外，还测试了含有不同表面官能团的XC-72R对氧还原的活性，并将其作为阴极催化剂用在MFC中，测试了电池性能。实验表明，经酸碱修饰的XC-72R作为空气阴极MFC的催化剂具有很好的应用前景。...
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| Published in | 催化学报 Vol. 35; no. 5; pp. 770 - 775 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | Chinese |
| Published |
中国科学院广州能源研究所，中国科学院可再生能源重点实验室，广东广州510640%中国科学院广州能源研究所，中国科学院可再生能源重点实验室，广东广州510640%天津大学环境科学与工程学院，内燃机燃烧学国家重点实验室，天津300072%南京师范大学化学与材料科学学院，江苏省生物功能材料重点实验室，江苏南京210097
2014
天津大学环境科学与工程学院，内燃机燃烧学国家重点实验室，天津300072 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0253-9837 1872-2067 |
| DOI | 10.1016/S1872-2067(14)60023-1 |
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| Abstract | 研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱（FTIR）、Boehm滴定法和X射线光电子能谱（谱（XPS）等手段对催化剂进行了表征。 FTIR测试证明硝酸处理可引入含氧基团氨水处理可引入含氮基团。另外，还测试了含有不同表面官能团的XC-72R对氧还原的活性，并将其作为阴极催化剂用在MFC中，测试了电池性能。实验表明，经酸碱修饰的XC-72R作为空气阴极MFC的催化剂具有很好的应用前景。 |
|---|---|
| AbstractList | 研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱（FTIR）、Boehm滴定法和X射线光电子能谱（谱（XPS）等手段对催化剂进行了表征。 FTIR测试证明硝酸处理可引入含氧基团氨水处理可引入含氮基团。另外，还测试了含有不同表面官能团的XC-72R对氧还原的活性，并将其作为阴极催化剂用在MFC中，测试了电池性能。实验表明，经酸碱修饰的XC-72R作为空气阴极MFC的催化剂具有很好的应用前景。 研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱(FTIR)、Boehm滴定法和X射线光电子能谱(谱(XPS)等手段对催化剂进行了表征。 FTIR测试证明硝酸处理可引入含氧基团氨水处理可引入含氮基团。另外，还测试了含有不同表面官能团的XC-72R对氧还原的活性，并将其作为阴极催化剂用在MFC中，测试了电池性能。实验表明，经酸碱修饰的XC-72R作为空气阴极MFC的催化剂具有很好的应用前景。 |
| Abstract_FL | The catalytic activity of surface-modified carbon powder, Vulcan XC-72R (XC), for the oxygen reduc-tion reaction (ORR) at an air cathode in a microbial fuel cell (MFC) has been investigated. The effects of treatment with different chemicals such as nitric acid and ammonia on the chemical characteris-tics of XC were studied. The catalysts were characterized by Fourier transform infrared spectrosco-py (FTIR), Boehm titration, and X-ray photoelectron spectroscopy. FTIR analysis showed that the functional groups of the materials were changed by chemical treatment, with nitric acid causing the introduction of oxygen-containing groups, and ammonia leading to the introduction of nitro-gen-containing groups. Electrochemical measurements of MFCs containing various modified carbon materials as ORR catalysts were performed, and the results showed that chemically modified car-bon materials are promising catalysts in MFCs. |
| Author | 杨改秀 孙永明 袁振宏 吕鹏梅 孔晓英 李连华 陈冠益 陆天虹 |
| AuthorAffiliation | 天津大学环境科学与工程学院,内燃机燃烧学国家重点实验室,天津300072 中国科学院广州能源研究所,中国科学院可再生能源重点实验室,广东广州510640 南京师范大学化学与材料科学学院,江苏省生物功能材料重点实验室,江苏南京210097 |
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| Author_FL | Lianhua Li Yongming Sun Zhenhong Yuan Xiaoying Kong Pengmei Lü Guanyi Chen Gaixiu Yang Tianhong Lu |
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| DOI | 10.1016/S1872-2067(14)60023-1 |
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| DocumentTitleAlternate | Application of surface-modified carbon powder in microbial fuel cells |
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| Keywords | 产电性能 Vulcan XC-72R碳黑 Surface modification 氧还原反应 Oxygen reduction reaction 微生物燃料电池 碳粉 Microbial fuel cell Carbon powder Electricity generation 表面改性 Vulcan XC-72R |
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| Notes | The catalytic activity of surface-modified carbon powder, Vulcan XC-72R （XC）, for the oxygen reduc-tion reaction （ORR） at an air cathode in a microbial fuel cell （MFC） has been investigated. The effects of treatment with different chemicals such as nitric acid and ammonia on the chemical characteris-tics of XC were studied. The catalysts were characterized by Fourier transform infrared spectrosco-py （FTIR）, Boehm titration, and X-ray photoelectron spectroscopy. FTIR analysis showed that the functional groups of the materials were changed by chemical treatment, with nitric acid causing the introduction of oxygen-containing groups, and ammonia leading to the introduction of nitro-gen-containing groups. Electrochemical measurements of MFCs containing various modified carbon materials as ORR catalysts were performed, and the results showed that chemically modified car-bon materials are promising catalysts in MFCs. Gaixiu Yang, Yongming Sun, Zhenhong Yuan, Pengmei L＆#252;, Xiaoying Kong, Lianhua Li, Guanyi Chen, Ti |
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| PublicationTitle | 催化学报 |
| PublicationTitleAlternate | Chinese Journal of Catalysis |
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| PublicationYear | 2014 |
| Publisher | 中国科学院广州能源研究所，中国科学院可再生能源重点实验室，广东广州510640%中国科学院广州能源研究所，中国科学院可再生能源重点实验室，广东广州510640%天津大学环境科学与工程学院，内燃机燃烧学国家重点实验室，天津300072%南京师范大学化学与材料科学学院，江苏省生物功能材料重点实验室，江苏南京210097 天津大学环境科学与工程学院，内燃机燃烧学国家重点实验室，天津300072 |
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| Snippet | 研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱（FTIR）、Boehm滴定法... 研究了在空气阴极微生物燃料电池中修饰方法如硝酸处理和硝酸-氨水酸碱等对XC-72R作为阴极氧还原催化剂催化活性的影响，并且使用傅里叶变换红外光谱(FTIR)、Boehm滴定法和X... |
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| SubjectTerms | Vulcan XC-72R碳黑 产电性能 微生物燃料电池 氧还原反应 碳粉 表面改性 |
| Title | 表面改性炭材料在微生物燃料电池中的应用 |
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