A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0

The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the modeling framework was limited to a zero-dimensional box model approach without resolving spatial gradients in aerosol concentrations. This pap...

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Published inGeoscientific Model Development Vol. 10; no. 11; pp. 4057 - 4079
Main Authors Curtis, Jeffrey H., Riemer, Nicole, West, Matthew
Format Journal Article
LanguageEnglish
Published Katlenburg-Lindau Copernicus GmbH 09.11.2017
Copernicus Publications, EGU
Copernicus Publications
Subjects
Aerodynamics
Aerosol concentrations
Aerosol particles
Aerosols
Algorithms
Altitude
Analysis
Atmosphere
Atmospheric aerosols
Atmospheric models
Black carbon
Boundary conditions
Boundary layers
Carbon
Chemical reactions
Chemistry
Computer simulation
Distribution
Dry deposition
Dye dispersion
Eddy diffusion
Environmental aspects
ENVIRONMENTAL SCIENCES
Evolution
Exact solutions
Frameworks
Gases
Mathematical models
Methods
Modelling
Numerical weather prediction
Optical properties
Particle dynamics
Particle methods (mathematics)
Planetary boundary layer
Spatial distribution
Turbulence
Turbulent diffusion
Vertical distribution
Online AccessGet full text
ISSN1991-9603
1991-959X
1991-962X
1991-9603
1991-962X
DOI10.5194/gmd-10-4057-2017

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Abstract The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the modeling framework was limited to a zero-dimensional box model approach without resolving spatial gradients in aerosol concentrations. This paper presents the development of stochastic particle methods to simulate turbulent diffusion and dry deposition of aerosol particles in a vertical column within the planetary boundary layer. The new model, WRF-PartMC-MOSAIC-SCM, resolves the vertical distribution of aerosol mixing state. We verified the new algorithms with analytical solutions for idealized test cases and illustrate the capabilities with results from a 2-day urban scenario that shows the evolution of black carbon mixing state in a vertical column.
AbstractList The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the modeling framework was limited to a zero-dimensional box model approach without resolving spatial gradients in aerosol concentrations. This paper presents the development of stochastic particle methods to simulate turbulent diffusion and dry deposition of aerosol particles in a vertical column within the planetary boundary layer. The new model, WRF-PartMC-MOSAIC-SCM, resolves the vertical distribution of aerosol mixing state. We verified the new algorithms with analytical solutions for idealized test cases and illustrate the capabilities with results from a 2-day urban scenario that shows the evolution of black carbon mixing state in a vertical column.
Audience Academic
Author Curtis, Jeffrey H.
Riemer, Nicole
West, Matthew
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  givenname: Matthew
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  surname: West
  fullname: West, Matthew
BackLink https://www.osti.gov/biblio/1460002$$D View this record in Osti.gov
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Snippet The PartMC-MOSAIC particle-resolved aerosol model was previously developed to predict the aerosol mixing state as it evolves in the atmosphere. However, the...
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StartPage 4057
SubjectTerms Aerodynamics
Aerosol concentrations
Aerosol particles
Aerosols
Algorithms
Altitude
Analysis
Atmosphere
Atmospheric aerosols
Atmospheric models
Black carbon
Boundary conditions
Boundary layers
Carbon
Chemical reactions
Chemistry
Computer simulation
Distribution
Dry deposition
Dye dispersion
Eddy diffusion
Environmental aspects
ENVIRONMENTAL SCIENCES
Evolution
Exact solutions
Frameworks
Gases
Mathematical models
Methods
Modelling
Numerical weather prediction
Optical properties
Particle dynamics
Particle methods (mathematics)
Planetary boundary layer
Spatial distribution
Turbulence
Turbulent diffusion
Vertical distribution
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Title A single-column particle-resolved model for simulating the vertical distribution of aerosol mixing state: WRF-PartMC-MOSAIC-SCM v1.0
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