少铅钙钛矿CH3NH3SrxPb(1-x)I3的合成及其在全固态薄膜太阳能电池中的应用
近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降....
Saved in:
Published in | 物理化学学报 Vol. 31; no. 2; pp. 285 - 290 |
---|---|
Main Author | |
Format | Journal Article |
Language | Chinese |
Published |
大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024
2015
九州工业大学生命体工学研究科,北九州808-0196,福冈,日本 |
Subjects | |
Online Access | Get full text |
ISSN | 1000-6818 |
DOI | 10.3866/PKU.WHXB201412241 |
Cover
Abstract | 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降. |
---|---|
AbstractList | 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降. O644; 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降. |
Abstract_FL | Hybrid organic-inorganic lead halide perovskite solar cel s (PSCs) have recently undergone rapid progress and exhibit high photoelectric conversion efficiencies of up to 19.3%. As light-absorber in PSCs, the hybrid organic-inorganic lead halide perovskite cannot be used in large-scale applications because of its high Pb content. In this work, we replaced some Pb with Sr to synthesize a novel perovskite CH3NH3SrxPb(1-x)I3 and used it as a light-absorber in PSCs. Compared with CH3NH3PbI3, CH3NH3Sr0.3Pb0.7I3 is a better light-absorber but the corresponding photovoltaic performance in PSCs decreased obviously. |
Author | 白晓功 史彦涛 王开 董庆顺 邢玉瑾 张鸿 王亮 马廷丽 |
AuthorAffiliation | 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024 九州工业大学生命体工学研究科,北九州808-0196,福冈,日本 |
AuthorAffiliation_xml | – name: 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024; 九州工业大学生命体工学研究科,北九州808-0196,福冈,日本 |
Author_FL | BAI Xiao-Gong MA Ting-Li SHI Yan-Tao ZHANG Hong WANG Liang DONG Qing-Shun WANG Kai XING Yu-Jin |
Author_FL_xml | – sequence: 1 fullname: BAI Xiao-Gong – sequence: 2 fullname: SHI Yan-Tao – sequence: 3 fullname: WANG Kai – sequence: 4 fullname: DONG Qing-Shun – sequence: 5 fullname: XING Yu-Jin – sequence: 6 fullname: ZHANG Hong – sequence: 7 fullname: WANG Liang – sequence: 8 fullname: MA Ting-Li |
Author_xml | – sequence: 1 fullname: 白晓功 史彦涛 王开 董庆顺 邢玉瑾 张鸿 王亮 马廷丽 |
BookMark | eNotkE9LAkEAxedgkJkfoGuXTmvzZ3d2PZZUK0kJGXWTmdldNWwtJdxuRRrWJTOJSqEOHSQIiihCjL5M6-rJr9CGXd67_N578KZAwC7YJgAzCEaIRul8cnUzsqVvL2KIZISxjAIgiCCEEtWQNgnCpVKOQ4gQVDDVgoC5L5fDq-qwcTtstLz775hO1nSyUXSSfNSrIckZ9c7ixLuruPVav1Z3L87d6ofb7rjVjtvq9o-OB9eVwWnbfXwa3rwNTr685nv_9eHn8_kv0m16zc40mLBYvmSG_z0EUstLqZguJdZX4rGFhCSUKJaobFERJYqhqpbKkWoomsVVaJgCciyiAnGIDI4ZRwZjqsn8jKEILFQihFCRTEJgblxbZrbF7Ex6p3BQtP3BdDmfdRzu_6FAX7BPzo5JkS3Ymf2cz-4Vc7useJimlFCiIaqRX6gvgDw |
ClassificationCodes | O644 |
ContentType | Journal Article |
Copyright | Copyright © Wanfang Data Co. Ltd. All Rights Reserved. |
Copyright_xml | – notice: Copyright © Wanfang Data Co. Ltd. All Rights Reserved. |
DBID | 2RA 92L CQIGP ~WA 2B. 4A8 92I 93N PSX TCJ |
DOI | 10.3866/PKU.WHXB201412241 |
DatabaseName | 维普_期刊 中文科技期刊数据库-CALIS站点 中文科技期刊数据库-7.0平台 中文科技期刊数据库- 镜像站点 Wanfang Data Journals - Hong Kong WANFANG Data Centre Wanfang Data Journals 万方数据期刊 - 香港版 China Online Journals (COJ) China Online Journals (COJ) |
DatabaseTitleList | |
DeliveryMethod | fulltext_linktorsrc |
Discipline | Chemistry |
DocumentTitleAlternate | Synthesis of CH3NH3SrxPb(1-x)I3 with Less Pb Content and Its Application in All-Solid Thin Film Solar Cells |
DocumentTitle_FL | Synthesis of CH3NH3SrxPb(1-x)I3 with Less Pb Content and Its Application in All-Solid Thin Film Solar Cells |
EndPage | 290 |
ExternalDocumentID | wlhxxb201502012 663638168 |
GrantInformation_xml | – fundername: The project was supported by the National Natural Science Foundation of China; International Science&Technology Cooperation Program of China (2013DFA51000).国家自然科学基金; 中国国际科技合作计划 funderid: (51402036,51273032,91333104); (51402036,51273032,91333104); (2013DFA51000) |
GroupedDBID | -02 2B. 2C. 2RA 5XA 5XC 92E 92I 92L ACGFS AENEX ALMA_UNASSIGNED_HOLDINGS CCEZO CDRFL CQIGP CW9 EBS EJD FIJ OK1 P2P RIG TCJ TGP U1G U5L ~WA 4A8 93N AAXUO AAYWO ADMLS FDB M41 PSX ROL UY8 |
ID | FETCH-LOGICAL-c592-64f6c935d77f7b17d58fb70dec0b2c9c1b01db2ab1daa7ea592d5c2c73ccc7143 |
ISSN | 1000-6818 |
IngestDate | Thu May 29 03:54:35 EDT 2025 Wed Feb 14 10:38:14 EST 2024 |
IsPeerReviewed | true |
IsScholarly | true |
Issue | 2 |
Keywords | 钙钛矿太阳能电池 Perovskite solar cel Less Pb 锶取代 Sr replacing CH3NH3SrxPb(1-x)I3 少铅 |
Language | Chinese |
LinkModel | OpenURL |
MergedId | FETCHMERGED-LOGICAL-c592-64f6c935d77f7b17d58fb70dec0b2c9c1b01db2ab1daa7ea592d5c2c73ccc7143 |
Notes | 11-1892/06 Hybrid organic-inorganic lead halide perovskite solar cel s (PSCs) have recently undergone rapid progress and exhibit high photoelectric conversion efficiencies of up to 19.3%. As light-absorber in PSCs, the hybrid organic-inorganic lead halide perovskite cannot be used in large-scale applications because of its high Pb content. In this work, we replaced some Pb with Sr to synthesize a novel perovskite CH3NH3SrxPb(1-x)I3 and used it as a light-absorber in PSCs. Compared with CH3NH3PbI3, CH3NH3Sr0.3Pb0.7I3 is a better light-absorber but the corresponding photovoltaic performance in PSCs decreased obviously. BAI Xiao-Gong SHI Yan-Tao WANG Kai DONG Qing-Shun XlNG Yu-Jin ZHANG Hong WANG Liang MA Ting(1State Key Laboratory of Fine Chemicals, College of Chemistry, Dalian University of Technology, Dalian 116024, Liaoning Province, R R. China; 2Graduate School of Life Science and Systems Engineering, Kyushu Institute of Technology, Kitakyushu 808-0196, Fukuoka, Japan) Perovskite solar cell; Less Pb; Sr replac |
PageCount | 6 |
ParticipantIDs | wanfang_journals_wlhxxb201502012 chongqing_primary_663638168 |
PublicationCentury | 2000 |
PublicationDate | 2015 |
PublicationDateYYYYMMDD | 2015-01-01 |
PublicationDate_xml | – year: 2015 text: 2015 |
PublicationDecade | 2010 |
PublicationTitle | 物理化学学报 |
PublicationTitleAlternate | Acta Physico-Chimica Sinica |
PublicationTitle_FL | Acta Physico-Chimica Sinica |
PublicationYear | 2015 |
Publisher | 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024 九州工业大学生命体工学研究科,北九州808-0196,福冈,日本 |
Publisher_xml | – name: 九州工业大学生命体工学研究科,北九州808-0196,福冈,日本 – name: 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024 |
SSID | ssib001105268 ssj0030168 ssib024507715 ssib002258135 ssib051374152 ssib057925156 |
Score | 2.078325 |
Snippet | 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化... O644; 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机... |
SourceID | wanfang chongqing |
SourceType | Aggregation Database Publisher |
StartPage | 285 |
SubjectTerms | CH3NH3SrxPb(1-x)I3 少铅 钙钛矿太阳能电池 锶取代 |
Title | 少铅钙钛矿CH3NH3SrxPb(1-x)I3的合成及其在全固态薄膜太阳能电池中的应用 |
URI | http://lib.cqvip.com/qk/92644X/201502/663638168.html https://d.wanfangdata.com.cn/periodical/wlhxxb201502012 |
Volume | 31 |
hasFullText | 1 |
inHoldings | 1 |
isFullTextHit | |
isPrint | |
journalDatabaseRights | – providerCode: PRVALS databaseName: IngentaConnect Open Access Journals issn: 1000-6818 databaseCode: FIJ dateStart: 20080115 customDbUrl: isFulltext: true dateEnd: 20150615 titleUrlDefault: http://www.ingentaconnect.com/content/title?j_type=online&j_startat=Aa&j_endat=Af&j_pagesize=200&j_page=1 omitProxy: true ssIdentifier: ssj0030168 providerName: Ingenta |
link | http://utb.summon.serialssolutions.com/2.0.0/link/0/eLvHCXMw5R1Na9RANBR70Iv4ibUqPTg3UzNJJpk5ZrJZthVKwRZ7W_Kx2x5kq7XFpSfFVqoXay2itqAHD0UQFFGkVPwzbrd76l_wvUl2N10VP65ewtuZ9_1mk_eG-dC0iyw0Y1q1Yp2JKtPtqJrooe1Q3WXw-XOcMDHSVb5jTmnSHp1iU339l3Krlhbmo-F48af7Sv4lqtAGccVdsn8R2Q5TaAAY4gtPiDA8_yjGJGBEGkRQEggiLMKZAkwiRBuQJHCJKBJZ9EvWWMm6Olcfj0gADT7hnOr1NixGLIXqEW4jX2FAPwkcfAIMLbxIuKcAkOooHJ94PGtJAZAnPUUF5KAW0DqKISfcQXzA8WzieUo_TqSluiwiC0q6TSRDckmJB0LhJyde4YBiwB_QUmSP55NrbOSCeEL1GigRdfNRB5RbIF4ecNAcj7WHnCISShEHAfAnUoO0YhdFeUGaSo82F_CFkHkuPCBcKhTwq9Ht4Rgpz8qMQO1AWUqyqZJs6iXddqr-Jm1nuUgqi0QEBwyTLmifw8lZ-EubBVrmme2g-8gQzJGKs5S9LuuIwLgWFJ9AxV4QDnaqwHAgF1kXaigwutzPWkC3riyOgjp8cHz0GkipA-kcMdl_a3suS8DjGBzeTRw68zdZFpDeQpUllGZ6H25vrmJxB6fNxq9MDl8rTUkTV1xjPt1NzDrLZW9fn6nXIxyBUNzhler9pgt5NR5qOzLaLX6oOrspl5wzTrvFkGlD6ed2k39GLawmOsUNcwXUOniyVprHwpc_20icGZuuCUG1L_-gNJ5MMzNbm74J-bba_lirhrXpXKY-cUw7mpXYQ176vjyu9S3OnNAO--2bLU9qYePd49aT5dba89baRvPl19ybcX9nBd6J-zsPRqzmi6XG6sruymrj0cPG8qfG5lZjeauxsb175-7e06W9-5uN129azz7s3fvSXP-4-_7Vt89vkWR7vbm-dUqbKAYTfknPrprRYyZM3bGrTiwslrhu1Y2omzBejVwjqcRGZMYippFBk8gMI5qEoVsJgSZhsRm7VhzHLpScp7VDtdla5Yw2ZFSYZVbcCM-xtGPLjCJT0JAaPOYJZDvhgDbY8VT5RnqiUBnKPgdXcPABbSjzXTn7ztwq90T_7O9RBrUjCKczxee0Q_NzC5XzUDvNRxfUkPkOCjIMTA |
linkProvider | Ingenta |
openUrl | ctx_ver=Z39.88-2004&ctx_enc=info%3Aofi%2Fenc%3AUTF-8&rfr_id=info%3Asid%2Fsummon.serialssolutions.com&rft_val_fmt=info%3Aofi%2Ffmt%3Akev%3Amtx%3Ajournal&rft.genre=article&rft.atitle=%E5%B0%91%E9%93%85%E9%92%99%E9%92%9B%E7%9F%BFCH3NH3SrxPb%EF%BC%881-x%EF%BC%89I3%E7%9A%84%E5%90%88%E6%88%90%E5%8F%8A%E5%85%B6%E5%9C%A8%E5%85%A8%E5%9B%BA%E6%80%81%E8%96%84%E8%86%9C%E5%A4%AA%E9%98%B3%E8%83%BD%E7%94%B5%E6%B1%A0%E4%B8%AD%E7%9A%84%E5%BA%94%E7%94%A8&rft.jtitle=%E7%89%A9%E7%90%86%E5%8C%96%E5%AD%A6%E5%AD%A6%E6%8A%A5&rft.au=%E7%99%BD%E6%99%93%E5%8A%9F&rft.au=%E5%8F%B2%E5%BD%A6%E6%B6%9B&rft.au=%E7%8E%8B%E5%BC%80&rft.au=%E8%91%A3%E5%BA%86%E9%A1%BA&rft.date=2015&rft.pub=%E5%A4%A7%E8%BF%9E%E7%90%86%E5%B7%A5%E5%A4%A7%E5%AD%A6%E5%8C%96%E5%AD%A6%E5%AD%A6%E9%99%A2%EF%BC%8C%E7%B2%BE%E7%BB%86%E5%8C%96%E5%B7%A5%E5%9B%BD%E5%AE%B6%E9%87%8D%E7%82%B9%E5%AE%9E%E9%AA%8C%E5%AE%A4%EF%BC%8C%E8%BE%BD%E5%AE%81%E5%A4%A7%E8%BF%9E116024%25%E5%A4%A7%E8%BF%9E%E7%90%86%E5%B7%A5%E5%A4%A7%E5%AD%A6%E5%8C%96%E5%AD%A6%E5%AD%A6%E9%99%A2%EF%BC%8C%E7%B2%BE%E7%BB%86%E5%8C%96%E5%B7%A5%E5%9B%BD%E5%AE%B6%E9%87%8D%E7%82%B9%E5%AE%9E%E9%AA%8C%E5%AE%A4%EF%BC%8C%E8%BE%BD%E5%AE%81%E5%A4%A7%E8%BF%9E116024&rft.issn=1000-6818&rft.issue=2&rft.spage=285&rft.epage=290&rft_id=info:doi/10.3866%2FPKU.WHXB201412241&rft.externalDocID=wlhxxb201502012 |
thumbnail_s | http://utb.summon.serialssolutions.com/2.0.0/image/custom?url=http%3A%2F%2Fimage.cqvip.com%2Fvip1000%2Fqk%2F92644X%2F92644X.jpg http://utb.summon.serialssolutions.com/2.0.0/image/custom?url=http%3A%2F%2Fwww.wanfangdata.com.cn%2Fimages%2FPeriodicalImages%2Fwlhxxb%2Fwlhxxb.jpg |