少铅钙钛矿CH3NH3SrxPb(1-x)I3的合成及其在全固态薄膜太阳能电池中的应用

近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降....

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Published in物理化学学报 Vol. 31; no. 2; pp. 285 - 290
Main Author 白晓功 史彦涛 王开 董庆顺 邢玉瑾 张鸿 王亮 马廷丽
Format Journal Article
LanguageChinese
Published 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024 2015
九州工业大学生命体工学研究科,北九州808-0196,福冈,日本
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ISSN1000-6818
DOI10.3866/PKU.WHXB201412241

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Abstract 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降.
AbstractList 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降.
O644; 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化铅卤钙钛矿,从长远来看, Pb的毒性将制约其大规模应用.本文从减少吸光材料中Pb的含量出发,尝试用Sr部分取代Pb制备一系列少铅钙钛矿CH3NH3SrxPb(1-x)I3,并将其应用于钙钛矿太阳能电池进行光电性能的研究.研究结果表明,相比于全Pb钙钛矿(CH3NH3PbI3)材料, Sr取代量为30%(x=0.3)时,所形成的CH3NH3Sr0.3Pb0.7I3光谱吸收大范围增强,但基于此材料制备的电池器件性能明显下降.
Abstract_FL Hybrid organic-inorganic lead halide perovskite solar cel s (PSCs) have recently undergone rapid progress and exhibit high photoelectric conversion efficiencies of up to 19.3%. As light-absorber in PSCs, the hybrid organic-inorganic lead halide perovskite cannot be used in large-scale applications because of its high Pb content. In this work, we replaced some Pb with Sr to synthesize a novel perovskite CH3NH3SrxPb(1-x)I3 and used it as a light-absorber in PSCs. Compared with CH3NH3PbI3, CH3NH3Sr0.3Pb0.7I3 is a better light-absorber but the corresponding photovoltaic performance in PSCs decreased obviously.
Author 白晓功 史彦涛 王开 董庆顺 邢玉瑾 张鸿 王亮 马廷丽
AuthorAffiliation 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024 九州工业大学生命体工学研究科,北九州808-0196,福冈,日本
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Author_FL BAI Xiao-Gong
MA Ting-Li
SHI Yan-Tao
ZHANG Hong
WANG Liang
DONG Qing-Shun
WANG Kai
XING Yu-Jin
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DocumentTitleAlternate Synthesis of CH3NH3SrxPb(1-x)I3 with Less Pb Content and Its Application in All-Solid Thin Film Solar Cells
DocumentTitle_FL Synthesis of CH3NH3SrxPb(1-x)I3 with Less Pb Content and Its Application in All-Solid Thin Film Solar Cells
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Keywords 钙钛矿太阳能电池
Perovskite solar cel
Less Pb
锶取代
Sr replacing
CH3NH3SrxPb(1-x)I3
少铅
Language Chinese
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Notes 11-1892/06
Hybrid organic-inorganic lead halide perovskite solar cel s (PSCs) have recently undergone rapid progress and exhibit high photoelectric conversion efficiencies of up to 19.3%. As light-absorber in PSCs, the hybrid organic-inorganic lead halide perovskite cannot be used in large-scale applications because of its high Pb content. In this work, we replaced some Pb with Sr to synthesize a novel perovskite CH3NH3SrxPb(1-x)I3 and used it as a light-absorber in PSCs. Compared with CH3NH3PbI3, CH3NH3Sr0.3Pb0.7I3 is a better light-absorber but the corresponding photovoltaic performance in PSCs decreased obviously.
BAI Xiao-Gong SHI Yan-Tao WANG Kai DONG Qing-Shun XlNG Yu-Jin ZHANG Hong WANG Liang MA Ting(1State Key Laboratory of Fine Chemicals, College of Chemistry, Dalian University of Technology, Dalian 116024, Liaoning Province, R R. China; 2Graduate School of Life Science and Systems Engineering, Kyushu Institute of Technology, Kitakyushu 808-0196, Fukuoka, Japan)
Perovskite solar cell; Less Pb; Sr replac
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PublicationTitle 物理化学学报
PublicationTitleAlternate Acta Physico-Chimica Sinica
PublicationTitle_FL Acta Physico-Chimica Sinica
PublicationYear 2015
Publisher 大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024%大连理工大学化学学院,精细化工国家重点实验室,辽宁大连116024
九州工业大学生命体工学研究科,北九州808-0196,福冈,日本
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Snippet 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机杂化...
O644; 近年来,有机-无机杂化铅卤化物钙钛矿太阳能电池(PSCs)得到了迅猛发展,其最高光电转换效率已经达到19.3%.该类型太阳能电池使用的钙钛矿型吸光材料为含Pb的有机-无机...
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SubjectTerms CH3NH3SrxPb(1-x)I3
少铅
钙钛矿太阳能电池
锶取代
Title 少铅钙钛矿CH3NH3SrxPb(1-x)I3的合成及其在全固态薄膜太阳能电池中的应用
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