Lead-Free Inverted Planar Formamidinium Tin Triiodide Perovskite Solar Cells Achieving Power Conversion Efficiencies up to 6.22
Efficient lead (Pb)‐free inverted planar formamidinium tin triiodide (FASnI3) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% ± 0.46% and a maximum PCE of 6.22% under forward voltage scan. The PVSCs exhibit small photoc...
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| Published in | Advanced materials (Weinheim) Vol. 28; no. 42; pp. 9333 - 9340 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Germany
Blackwell Publishing Ltd
01.11.2016
Wiley |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0935-9648 1521-4095 |
| DOI | 10.1002/adma.201602992 |
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| Abstract | Efficient lead (Pb)‐free inverted planar formamidinium tin triiodide (FASnI3) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% ± 0.46% and a maximum PCE of 6.22% under forward voltage scan. The PVSCs exhibit small photocurrent–voltage hysteresis and high reproducibility. The champion cell shows a steady‐state efficiency of ≈6.00% for over 100 s. |
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| AbstractList | Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI
) perovskite solar cells (PVSCs) are demonstrated. Our FASnI
PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% ± 0.46% and a maximum PCE of 6.22% under forward voltage scan. The PVSCs exhibit small photocurrent-voltage hysteresis and high reproducibility. The champion cell shows a steady-state efficiency of ≈6.00% for over 100 s. Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI3 ) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% ± 0.46% and a maximum PCE of 6.22% under forward voltage scan. The PVSCs exhibit small photocurrent-voltage hysteresis and high reproducibility. The champion cell shows a steady-state efficiency of ≈6.00% for over 100 s. Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI3) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% ± 0.46% and a maximum PCE of 6.22% under forward voltage scan. Here, the PVSCs exhibit small photocurrent–voltage hysteresis and high reproducibility. The champion cell shows a steady-state efficiency of ≈6.00% for over 100 s. Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI sub(3)) perovskite solar cells (PVSCs) are demonstrated. Our FASnI sub(3) PVSCs achieved average power conversion efficiencies (PCEs) of 5.41% plus or minus 0.46% and a maximum PCE of 6.22% under forward voltage scan. The PVSCs exhibit small photocurrent-voltage hysteresis and high reproducibility. The champion cell shows a steady-state efficiency of approximately 6.00% for over 100 s. |
| Author | Zhao, Dewei Cimaroli, Alexander J. Yu, Yue Wang, Changlei Xiong, Ren-Gen Schulz, Philip Meng, Weiwei Liao, Weiqiang Zhu, Kai Grice, Corey R. Yan, Yanfa |
| Author_xml | – sequence: 1 givenname: Weiqiang surname: Liao fullname: Liao, Weiqiang organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, 43606, Toledo, OH, USA – sequence: 2 givenname: Dewei surname: Zhao fullname: Zhao, Dewei email: dewei.zhao@utoledo.edu, dewei.zhao@utoledo.edu organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 3 givenname: Yue surname: Yu fullname: Yu, Yue organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 4 givenname: Corey R. surname: Grice fullname: Grice, Corey R. organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 5 givenname: Changlei surname: Wang fullname: Wang, Changlei organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 6 givenname: Alexander J. surname: Cimaroli fullname: Cimaroli, Alexander J. organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 7 givenname: Philip surname: Schulz fullname: Schulz, Philip organization: Chemistry and Nanoscience Center, National Renewable Energy Laboratory, CO, 80401, Golden, USA – sequence: 8 givenname: Weiwei surname: Meng fullname: Meng, Weiwei organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA – sequence: 9 givenname: Kai surname: Zhu fullname: Zhu, Kai organization: Chemistry and Nanoscience Center, National Renewable Energy Laboratory, CO, 80401, Golden, USA – sequence: 10 givenname: Ren-Gen surname: Xiong fullname: Xiong, Ren-Gen email: xiongrg@seu.edu.cn, dewei.zhao@utoledo.edu organization: Ordered Matter Science Research Center, Southeast University, 211189, Nanjing, P. R. China – sequence: 11 givenname: Yanfa surname: Yan fullname: Yan, Yanfa email: yanfa.yan@utoledo.edu, dewei.zhao@utoledo.edu organization: Department of Physics and Astronomy and Wright Center for Photovoltaics Innovation and Commercialization, The University of Toledo, OH, 43606, Toledo, USA |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/27571446$$D View this record in MEDLINE/PubMed https://www.osti.gov/servlets/purl/1331968$$D View this record in Osti.gov |
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| Copyright | 2016 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Discipline | Engineering |
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| Issue | 42 |
| Keywords | lead-free, perovskite solar cells uniform perovskites SnF2 additives pinhole-free |
| Language | English |
| License | http://onlinelibrary.wiley.com/termsAndConditions#am http://onlinelibrary.wiley.com/termsAndConditions#vor 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
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| Notes | U.S. Department of Energy U.S. Department of Energy - No. DE-FOA-0000990 Solar Energy Technologies Office Office of Energy Efficiency and Renewable Energy National Science Foundation - No. CHE−1230246; No. DMR−1534686 Ohio Research Scholar Program ArticleID:ADMA201602992 istex:E033BEE5B0F49A472F2981FB15C1A06F56934636 ark:/67375/WNG-6VZB6KV9-Z ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 NREL/JA-5K00-67095 USDOE Office of Energy Efficiency and Renewable Energy (EERE) AC36-08GO28308; DE‐FOA‐0000990 |
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| Snippet | Efficient lead (Pb)‐free inverted planar formamidinium tin triiodide (FASnI3) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved... Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI ) perovskite solar cells (PVSCs) are demonstrated. Our FASnI PVSCs achieved average... Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI3 ) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved... Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI sub(3)) perovskite solar cells (PVSCs) are demonstrated. Our FASnI sub(3) PVSCs... Efficient lead (Pb)-free inverted planar formamidinium tin triiodide (FASnI3) perovskite solar cells (PVSCs) are demonstrated. Our FASnI3 PVSCs achieved... |
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| SubjectTerms | Efficiency Electric potential Energy conversion efficiency FASnI3 lead-free lead‐free, perovskite solar cells MATERIALS SCIENCE perovskite solar cells Perovskites Photovoltaic cells pinhole-free Reproducibility SnF2 additives Solar cells SOLAR ENERGY uniform perovskites Voltage |
| Title | Lead-Free Inverted Planar Formamidinium Tin Triiodide Perovskite Solar Cells Achieving Power Conversion Efficiencies up to 6.22 |
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