Ultrafine particles produced by ozone/limonene reactions in indoor air under low/closed ventilation conditions
Formation of ultrafine particles, dp<100nm, from gas-phase reaction of limonene with O3 was studied. The concentration of reactants was chosen as close to realistic indoor conditions as possible. Two reaction chambers (1 and 14m3) were used. Particle number concentrations were measured using a CP...
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| Published in | Atmospheric environment (1994) Vol. 42; no. 18; pp. 4149 - 4159 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Oxford
Elsevier Ltd
01.06.2008
Elsevier Science |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1352-2310 1873-2844 1873-2844 |
| DOI | 10.1016/j.atmosenv.2008.01.034 |
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| Abstract | Formation of ultrafine particles, dp<100nm, from gas-phase reaction of limonene with O3 was studied. The concentration of reactants was chosen as close to realistic indoor conditions as possible. Two reaction chambers (1 and 14m3) were used. Particle number concentrations were measured using a CPC and size distributions by using a scanning mobility particle sizer (SMPS) system. Rapid formation of new particles was observed at low concentrations of reactants and close to zero ventilation rates. The maximum number of particles was correlated with the initial rate of formation of reaction products. An excess of O3 tends to give higher maximum particle concentrations. Modeling work lead to the conclusion that significant nucleation starts when the mixing ratio of “product” from the reaction Limonene+O3→productox exceeds 0.5–1ppb. The secondary particles formed by atmospheric chemistry in indoor air contribute to the total particulate matter indoors and should be considered in terms of low-dose long-term exposure. |
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| AbstractList | Formation of ultrafine particles, d sub(p) < 100nm, from gas-phase reaction of limonene with O sub(3) was studied. The concentration of reactants was chosen as close to realistic indoor conditions as possible. Two reaction chambers (1 and 14m super(3)) were used. Particle number concentrations were measured using a CPC and size distributions by using a scanning mobility particle sizer (SMPS) system. Rapid formation of new particles was observed at low concentrations of reactants and close to zero ventilation rates. The maximum number of particles was correlated with the initial rate of formation of reaction products. An excess of O sub(3) tends to give higher maximum particle concentrations. Modeling work lead to the conclusion that significant nucleation starts when the mixing ratio of ''product'' from the reaction Limonene+O sub(3)- > product sub(o) sub(x) exceeds 0.5-1ppb. The secondary particles formed by atmospheric chemistry in indoor air contribute to the total particulate matter indoors and should be considered in terms of low-dose long-term exposure. Formation of ultrafine particles from gas-phase reaction of limonene with ozone (O sub(3)) was studied. Particle number concentrations were measured using a CPC and size distributions using a scanning mobility particle sizer (SMPS) system. A scanning mobility particle sizer (SMPS) consisting of a TSI model 3085 Differential Mobility Analyzer with a TSI 3080 analyzer coupled to a TSI 3010 condensation particle counter (CNC) was used to determine number size distributions. The SMPS is maintained and calibrated on a routine basis. The CNC was operated with a temperature difference between saturator and condenser of 25 degree C, giving a lower size detection limit of around 5 nm. Formation of ultrafine particles, dp Formation of ultrafine particles, dp<100nm, from gas-phase reaction of limonene with O3 was studied. The concentration of reactants was chosen as close to realistic indoor conditions as possible. Two reaction chambers (1 and 14m3) were used. Particle number concentrations were measured using a CPC and size distributions by using a scanning mobility particle sizer (SMPS) system. Rapid formation of new particles was observed at low concentrations of reactants and close to zero ventilation rates. The maximum number of particles was correlated with the initial rate of formation of reaction products. An excess of O3 tends to give higher maximum particle concentrations. Modeling work lead to the conclusion that significant nucleation starts when the mixing ratio of “product” from the reaction Limonene+O3→productox exceeds 0.5–1ppb. The secondary particles formed by atmospheric chemistry in indoor air contribute to the total particulate matter indoors and should be considered in terms of low-dose long-term exposure. |
| Author | Ekberg, Lars Langer, Sarka Arrhenius, Karine Moldanová, Jana Ljungström, Evert |
| Author_xml | – sequence: 1 givenname: Sarka surname: Langer fullname: Langer, Sarka email: sarka.langer@sp.se organization: SP Technical Research Institute of Sweden, Department of Chemistry and Materials Technology, Brinellgatan 4, PO Box 857, SE-501 15 Borås, Sweden – sequence: 2 givenname: Jana surname: Moldanová fullname: Moldanová, Jana organization: IVL Swedish Environmental Institute, Box 5302, SE-400 14 Göteborg, Sweden – sequence: 3 givenname: Karine surname: Arrhenius fullname: Arrhenius, Karine organization: SP Technical Research Institute of Sweden, Department of Chemistry and Materials Technology, Brinellgatan 4, PO Box 857, SE-501 15 Borås, Sweden – sequence: 4 givenname: Evert surname: Ljungström fullname: Ljungström, Evert organization: Chalmers University of Technology, Inorganic Environmental Chemistry and the Chemistry Department, Atmospheric Science, Göteborg University, SE-412 96 Göteborg, Sweden – sequence: 5 givenname: Lars surname: Ekberg fullname: Ekberg, Lars organization: CIT Energy Management, SE-412 96 Göteborg, Sweden |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=20410070$$DView record in Pascal Francis https://research.chalmers.se/publication/75863$$DView record from Swedish Publication Index |
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| Keywords | Indoor air chemistry Ozone Secondary organic aerosol Limonene Ultrafine particles 1,8-p-Menthadiene Pollutant formation Secondary pollutant Air quality Ultrafine particle Precursor Biogenic factor Terpene Aerosols Reaction mechanism Indoor pollution Ventilation Oxidation Organic compounds |
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| Snippet | Formation of ultrafine particles, dp<100nm, from gas-phase reaction of limonene with O3 was studied. The concentration of reactants was chosen as close to... Formation of ultrafine particles from gas-phase reaction of limonene with ozone (O sub(3)) was studied. Particle number concentrations were measured using a... Formation of ultrafine particles, d sub(p)<100nm, from gas-phase reaction of limonene with O sub(3) was studied. The concentration of reactants was chosen as... Formation of ultrafine particles, d sub(p) < 100nm, from gas-phase reaction of limonene with O sub(3) was studied. The concentration of reactants was chosen as... Formation of ultrafine particles, dp |
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| SubjectTerms | Applied sciences Atmospheric pollution Buildings. Public works Exact sciences and technology Indoor air chemistry Indoor pollution and occupational exposure Limonene Ozone Pollution Pollution indoor buildings Secondary organic aerosol Ultrafine particles |
| Title | Ultrafine particles produced by ozone/limonene reactions in indoor air under low/closed ventilation conditions |
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