Catalytic Ozonation Treatment of Coal Chemical Reverse Osmosis Concentrate: Water Quality Analysis, Parameter Optimization, and Catalyst Deactivation Investigation

Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater treatments. However, problems such as a low organic pollutant removal efficiency and unstable operation during the catalytic ozone treatment pro...

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Published inToxics (Basel) Vol. 12; no. 9; p. 681
Main Authors Qin, Yihe, Yuan, Run, Wang, Shaozhou, Zhang, Xuewei, Luo, Shaojun, He, Xuwen
Format Journal Article
LanguageEnglish
Published Switzerland MDPI AG 01.09.2024
MDPI
Subjects
catalyst deactivation
Catalysts
Catalytic oxidation
catalytic ozonation
Chemical oxygen demand
Coal
Deactivation
Fixed bed reactors
Indicators
Investigations
Organic wastes
Oxidation
Oxidation process
Ozonation
Ozone
Ozonization
Pollutant removal
Pollutants
Purification
Quality control
Reverse osmosis
reverse osmosis concentrate
Sewage
Spectrum analysis
Toxicity
Wastewater treatment
Water quality
water quality analysis
Water treatment
China
United States > US
catalytic ozonation
reverse osmosis concentrate
catalyst deactivation
water quality analysis
Online AccessGet full text
ISSN2305-6304
2305-6304
DOI10.3390/toxics12090681

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Abstract Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater treatments. However, problems such as a low organic pollutant removal efficiency and unstable operation during the catalytic ozone treatment process for wastewater remain. To address these disadvantages, in this study, the treatment efficacy of catalytic ozone oxidation on a coal chemical reverse osmosis concentrate was investigated. The basic water quality indicators of the chemical reverse osmosis concentrate were analyzed. The effects of initial pollutant concentration, pH, ozone concentration, and catalyst concentration on the COD removal rate from the coal chemical reverse osmosis concentrate were explored. Water quality indicators of the chemical reverse osmosis concentrate before and after the catalytic ozone treatment were studied using spectroscopic analysis methods. The RO concentrate demonstrated large water quality fluctuations, and the catalytic ozonation process removed most of the pollutants from the treated wastewater. A possible deactivation mechanism of the ozone catalyst was also proposed. This study provides a theoretical reference and technical support for the long-term, efficient, and stable removal of organic pollutants from coal chemical reverse osmosis concentrate using a catalytic ozone oxidation process in practical engineering applications.
AbstractList Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater treatments. However, problems such as a low organic pollutant removal efficiency and unstable operation during the catalytic ozone treatment process for wastewater remain. To address these disadvantages, in this study, the treatment efficacy of catalytic ozone oxidation on a coal chemical reverse osmosis concentrate was investigated. The basic water quality indicators of the chemical reverse osmosis concentrate were analyzed. The effects of initial pollutant concentration, pH, ozone concentration, and catalyst concentration on the COD removal rate from the coal chemical reverse osmosis concentrate were explored. Water quality indicators of the chemical reverse osmosis concentrate before and after the catalytic ozone treatment were studied using spectroscopic analysis methods. The RO concentrate demonstrated large water quality fluctuations, and the catalytic ozonation process removed most of the pollutants from the treated wastewater. A possible deactivation mechanism of the ozone catalyst was also proposed. This study provides a theoretical reference and technical support for the long-term, efficient, and stable removal of organic pollutants from coal chemical reverse osmosis concentrate using a catalytic ozone oxidation process in practical engineering applications.
Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater treatments. However, problems such as a low organic pollutant removal efficiency and unstable operation during the catalytic ozone treatment process for wastewater remain. To address these disadvantages, in this study, the treatment efficacy of catalytic ozone oxidation on a coal chemical reverse osmosis concentrate was investigated. The basic water quality indicators of the chemical reverse osmosis concentrate were analyzed. The effects of initial pollutant concentration, pH, ozone concentration, and catalyst concentration on the COD removal rate from the coal chemical reverse osmosis concentrate were explored. Water quality indicators of the chemical reverse osmosis concentrate before and after the catalytic ozone treatment were studied using spectroscopic analysis methods. The RO concentrate demonstrated large water quality fluctuations, and the catalytic ozonation process removed most of the pollutants from the treated wastewater. A possible deactivation mechanism of the ozone catalyst was also proposed. This study provides a theoretical reference and technical support for the long-term, efficient, and stable removal of organic pollutants from coal chemical reverse osmosis concentrate using a catalytic ozone oxidation process in practical engineering applications.Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater treatments. However, problems such as a low organic pollutant removal efficiency and unstable operation during the catalytic ozone treatment process for wastewater remain. To address these disadvantages, in this study, the treatment efficacy of catalytic ozone oxidation on a coal chemical reverse osmosis concentrate was investigated. The basic water quality indicators of the chemical reverse osmosis concentrate were analyzed. The effects of initial pollutant concentration, pH, ozone concentration, and catalyst concentration on the COD removal rate from the coal chemical reverse osmosis concentrate were explored. Water quality indicators of the chemical reverse osmosis concentrate before and after the catalytic ozone treatment were studied using spectroscopic analysis methods. The RO concentrate demonstrated large water quality fluctuations, and the catalytic ozonation process removed most of the pollutants from the treated wastewater. A possible deactivation mechanism of the ozone catalyst was also proposed. This study provides a theoretical reference and technical support for the long-term, efficient, and stable removal of organic pollutants from coal chemical reverse osmosis concentrate using a catalytic ozone oxidation process in practical engineering applications.
Audience Academic
Author He, Xuwen
Zhang, Xuewei
Qin, Yihe
Luo, Shaojun
Wang, Shaozhou
Yuan, Run
AuthorAffiliation 2 School of Chemical and Environmental Engineering, China University of Mining & Technology, Beijing 100083, China; wangshaozhou95@163.com (S.W.); ethan-z@foxmail.com (X.Z.); shaojun_luo@163.com (S.L.)
1 School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan 523808, China; qinyihely@163.com (Y.Q.); qyuanrun@163.com (R.Y.)
AuthorAffiliation_xml – name: 1 School of Environment and Civil Engineering, Dongguan University of Technology, Dongguan 523808, China; qinyihely@163.com (Y.Q.); qyuanrun@163.com (R.Y.)
– name: 2 School of Chemical and Environmental Engineering, China University of Mining & Technology, Beijing 100083, China; wangshaozhou95@163.com (S.W.); ethan-z@foxmail.com (X.Z.); shaojun_luo@163.com (S.L.)
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BackLink https://www.ncbi.nlm.nih.gov/pubmed/39330609$$D View this record in MEDLINE/PubMed
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Keywords catalytic ozonation
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catalyst deactivation
water quality analysis
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Snippet Catalytic ozone oxidation, which is characterized by strong oxidizing properties and environmental friendliness, has been widely used in organic wastewater...
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SubjectTerms catalyst deactivation
Catalysts
Catalytic oxidation
catalytic ozonation
Chemical oxygen demand
Coal
Deactivation
Fixed bed reactors
Indicators
Investigations
Organic wastes
Oxidation
Oxidation process
Ozonation
Ozone
Ozonization
Pollutant removal
Pollutants
Purification
Quality control
Reverse osmosis
reverse osmosis concentrate
Sewage
Spectrum analysis
Toxicity
Wastewater treatment
Water quality
water quality analysis
Water treatment
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Title Catalytic Ozonation Treatment of Coal Chemical Reverse Osmosis Concentrate: Water Quality Analysis, Parameter Optimization, and Catalyst Deactivation Investigation
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