PCDD/Fs atmospheric deposition fluxes and soil contamination close to a municipal solid waste incinerator
► Atmospheric Bulk deposition flows of PCDD/Fs were monitored nearby a MSW incinerator. ► PCDD/F congeners patterns in industrial and environmental samples are presented. ► Urban contribution to PCDD/Fs deposition resulted higher than industrial one. Bulk depositions and surface soil were collected...
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| Published in | Chemosphere (Oxford) Vol. 83; no. 10; pp. 1366 - 1373 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Kidlington
Elsevier Ltd
01.05.2011
Elsevier |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0045-6535 1879-1298 1879-1298 |
| DOI | 10.1016/j.chemosphere.2011.02.072 |
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| Abstract | ► Atmospheric Bulk deposition flows of PCDD/Fs were monitored nearby a MSW incinerator. ► PCDD/F congeners patterns in industrial and environmental samples are presented. ► Urban contribution to PCDD/Fs deposition resulted higher than industrial one.
Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area’s total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3
pg
m
−2
d
−1 to 89.9
pg
m
−2
d
−1 (0.75
pg-TEQ
m
−2
d
−1 to 3.73
pg-TEQ
m
−2
d
−1) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8
ng
kg
−1 d.w. and 1.35
ng-TEQ
kg
−1
d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. |
|---|---|
| AbstractList | Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area's total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3 pg m(-2)d(-1) to 89.9 pg m(-2)d(-1) (0.75 pg-TEQ m(-2)d(-1) to 3.73 pg-TEQ m(-2)d(-1)) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8 ng kg(-1) d.w. and 1.35 ng-TEQ kg(-1)d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area’s total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3pgm⁻²d⁻¹ to 89.9pgm⁻²d⁻¹ (0.75pg-TEQm⁻²d⁻¹ to 3.73pg-TEQm⁻²d⁻¹) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8ngkg⁻¹ d.w. and 1.35ng-TEQkg⁻¹d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area's total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3 pg m(-2)d(-1) to 89.9 pg m(-2)d(-1) (0.75 pg-TEQ m(-2)d(-1) to 3.73 pg-TEQ m(-2)d(-1)) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8 ng kg(-1) d.w. and 1.35 ng-TEQ kg(-1)d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area.Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area's total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3 pg m(-2)d(-1) to 89.9 pg m(-2)d(-1) (0.75 pg-TEQ m(-2)d(-1) to 3.73 pg-TEQ m(-2)d(-1)) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8 ng kg(-1) d.w. and 1.35 ng-TEQ kg(-1)d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area's total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3pgm super(-2) d super(-1) to 89.9pgm super(-2) d super(-1) (0.75pg-TEQm super(-2) d super(-1) to 3.73pg-TEQm super(-2) d super(-1)) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8ngkg super(-1) d.w. and 1.35ng-TEQkg super(-1) d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. ► Atmospheric Bulk deposition flows of PCDD/Fs were monitored nearby a MSW incinerator. ► PCDD/F congeners patterns in industrial and environmental samples are presented. ► Urban contribution to PCDD/Fs deposition resulted higher than industrial one. Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste incinerator to the area’s total contamination with polychlorinated dibenzodioxins and polychlorinated dibenzofurans (PCDDs and PCDFs). Samples were collected at two sites, situated in the area most affected by plant emissions (according to the results of the Calpuff air dispersion model), and at an external site, considered as a reference. Results show that the studied area is subject to low contamination, as far as these compounds are concerned. Deposition fluxes range from 14.3 pg m −2 d −1 to 89.9 pg m −2 d −1 (0.75 pg-TEQ m −2 d −1 to 3.73 pg-TEQ m −2 d −1) and no significant flow differences are observed among the three monitored sites. Total soil concentration amounts to 93.8 ng kg −1 d.w. and 1.35 ng-TEQ kg −1 d.w, on average, and confirms a strong homogeneity in the studied area. Furthermore, from 2006 to 2009, no PCDD/Fs enrichment in the soil was noticed. Comparing the relative congener distributions in environmental samples with those found in stack emissions from the incineration plant, significant differences are observed in the PCDD:PCDF ratio and in the contribution of the most chlorinated congeners. From this study we can conclude that the incineration plant is not the main source of PCDD/Fs in the studied area, which is apparently characterized by a homogeneous and widespread contamination situation, typical of an urban area. |
| Author | Passarini, Fabrizio Morselli, Luciano Vassura, Ivano Bernardi, Elena Ferroni, Laura |
| Author_xml | – sequence: 1 givenname: Ivano surname: Vassura fullname: Vassura, Ivano organization: University of Bologna, Department of Industrial Chemistry and Materials, Viale Risorgimento 4, I-40146 Bologna, Italy – sequence: 2 givenname: Fabrizio surname: Passarini fullname: Passarini, Fabrizio organization: University of Bologna, Department of Industrial Chemistry and Materials, Viale Risorgimento 4, I-40146 Bologna, Italy – sequence: 3 givenname: Laura surname: Ferroni fullname: Ferroni, Laura organization: University of Bologna, Rimini Branch, Via Angherà 22, I-47900 Rimini, Italy – sequence: 4 givenname: Elena surname: Bernardi fullname: Bernardi, Elena organization: University of Bologna, Department of Industrial Chemistry and Materials, Viale Risorgimento 4, I-40146 Bologna, Italy – sequence: 5 givenname: Luciano surname: Morselli fullname: Morselli, Luciano email: luciano.morselli@unibo.it organization: University of Bologna, Department of Industrial Chemistry and Materials, Viale Risorgimento 4, I-40146 Bologna, Italy |
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| Keywords | Air pollution Atmospheric fallout PCDD/Fs Stack emissions Bulk deposition Monitoring Dioxin derivatives Pollutant behavior Urban waste Soil pollution Persistent organic pollutant Incineration plant Flux density Surveillance Chlorine Organic compounds Solid waste Organic compounds |
| Language | English |
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| Snippet | ► Atmospheric Bulk deposition flows of PCDD/Fs were monitored nearby a MSW incinerator. ► PCDD/F congeners patterns in industrial and environmental samples are... Bulk depositions and surface soil were collected in a suburban area, near the Adriatic Sea, in order to assess the contribution of a municipal solid waste... |
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| SubjectTerms | Adriatic Sea air Air Pollutants Air Pollutants - analysis Air pollution analogs & derivatives analysis Applied sciences Atmosphere Atmosphere - chemistry atmospheric deposition Atmospheric fallout Benzofurans Benzofurans - analysis Bulk deposition chemistry Cities Dibenzofurans, Polychlorinated dispersions emissions Environmental Monitoring Environmental Pollution Environmental Pollution - statistics & numerical data Exact sciences and technology Incineration Monitoring municipal solid waste PCDD/Fs Pollution polychlorinated dibenzodioxins Polychlorinated Dibenzodioxins - analogs & derivatives Polychlorinated Dibenzodioxins - analysis polychlorinated dibenzofurans soil Soil - chemistry Soil Pollutants Soil Pollutants - analysis soil pollution Stack emissions statistics & numerical data suburban areas urban areas |
| Title | PCDD/Fs atmospheric deposition fluxes and soil contamination close to a municipal solid waste incinerator |
| URI | https://dx.doi.org/10.1016/j.chemosphere.2011.02.072 https://www.ncbi.nlm.nih.gov/pubmed/21459405 https://www.proquest.com/docview/1365038117 https://www.proquest.com/docview/865695492 https://www.proquest.com/docview/883015840 |
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