Fine tuning of graphene-metal adhesion by surface alloying
We show that bimetallic surface alloying provides a viable route for governing the interaction between graphene and metal through the selective choice of the elemental composition of the surface alloy. This concept is illustrated by an experimental and theoretical characterization of the properties...
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| Published in | Scientific reports Vol. 3; no. 1; p. 2430 |
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| Main Authors | , , , , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
London
Nature Publishing Group UK
13.08.2013
Nature Publishing Group |
| Subjects | |
| Online Access | Get full text |
| ISSN | 2045-2322 2045-2322 |
| DOI | 10.1038/srep02430 |
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| Abstract | We show that bimetallic surface alloying provides a viable route for governing the interaction between graphene and metal through the selective choice of the elemental composition of the surface alloy. This concept is illustrated by an experimental and theoretical characterization of the properties of graphene on a model PtRu surface alloy on Ru(0001), with a concentration of Pt atoms in the first layer between 0 and 50%. The progressive increase of the Pt content determines the gradual detachment of graphene from the substrate, which results from the modification of the carbon orbital hybridization promoted by Pt. Alloying is also found to affect the morphology of graphene, which is strongly corrugated on bare Ru, but becomes flat at a Pt coverage of 50%. The method here proposed can be readily extended to several supports, thus opening the way to the conformal growth of graphene on metals and to a full tunability of the graphene-substrate interaction. |
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| AbstractList | We show that bimetallic surface alloying provides a viable route for governing the interaction between graphene and metal through the selective choice of the elemental composition of the surface alloy. This concept is illustrated by an experimental and theoretical characterization of the properties of graphene on a model PtRu surface alloy on Ru(0001), with a concentration of Pt atoms in the first layer between 0 and 50%. The progressive increase of the Pt content determines the gradual detachment of graphene from the substrate, which results from the modification of the carbon orbital hybridization promoted by Pt. Alloying is also found to affect the morphology of graphene, which is strongly corrugated on bare Ru, but becomes flat at a Pt coverage of 50%. The method here proposed can be readily extended to several supports, thus opening the way to the conformal growth of graphene on metals and to a full tunability of the graphene-substrate interaction.We show that bimetallic surface alloying provides a viable route for governing the interaction between graphene and metal through the selective choice of the elemental composition of the surface alloy. This concept is illustrated by an experimental and theoretical characterization of the properties of graphene on a model PtRu surface alloy on Ru(0001), with a concentration of Pt atoms in the first layer between 0 and 50%. The progressive increase of the Pt content determines the gradual detachment of graphene from the substrate, which results from the modification of the carbon orbital hybridization promoted by Pt. Alloying is also found to affect the morphology of graphene, which is strongly corrugated on bare Ru, but becomes flat at a Pt coverage of 50%. The method here proposed can be readily extended to several supports, thus opening the way to the conformal growth of graphene on metals and to a full tunability of the graphene-substrate interaction. We show that bimetallic surface alloying provides a viable route for governing the interaction between graphene and metal through the selective choice of the elemental composition of the surface alloy. This concept is illustrated by an experimental and theoretical characterization of the properties of graphene on a model PtRu surface alloy on Ru(0001), with a concentration of Pt atoms in the first layer between 0 and 50%. The progressive increase of the Pt content determines the gradual detachment of graphene from the substrate, which results from the modification of the carbon orbital hybridization promoted by Pt. Alloying is also found to affect the morphology of graphene, which is strongly corrugated on bare Ru, but becomes flat at a Pt coverage of 50%. The method here proposed can be readily extended to several supports, thus opening the way to the conformal growth of graphene on metals and to a full tunability of the graphene-substrate interaction. |
| ArticleNumber | 2430 |
| Author | Menteş, T. O. Miniussi, E. Baraldi, A. Pozzo, M. Larciprete, R. Lacovig, P. Locatelli, A. Günther, S. Burgos, B. Santos Lizzit, S. Alfè, D. |
| Author_xml | – sequence: 1 givenname: D. surname: Alfè fullname: Alfè, D. organization: Department of Earth Sciences, Department of Physics and Astronomy, TYC@UCL and London Centre for Nanotechnology, University College London, IOM-CNR, DEMOCRITOS National Simulation Centre – sequence: 2 givenname: M. surname: Pozzo fullname: Pozzo, M. organization: Department of Earth Sciences, Department of Physics and Astronomy, TYC@UCL and London Centre for Nanotechnology, University College London – sequence: 3 givenname: E. surname: Miniussi fullname: Miniussi, E. organization: Physics Department and CENMAT, University of Trieste, IOM-CNR, Laboratorio TASC – sequence: 4 givenname: S. surname: Günther fullname: Günther, S. organization: Chemie Department, Technische Universität München, Physikalische Chemie mit Schwerpunkt Katalyse – sequence: 5 givenname: P. surname: Lacovig fullname: Lacovig, P. organization: Elettra - Sincrotrone Trieste S.C.p.A – sequence: 6 givenname: S. surname: Lizzit fullname: Lizzit, S. organization: Elettra - Sincrotrone Trieste S.C.p.A – sequence: 7 givenname: R. surname: Larciprete fullname: Larciprete, R. organization: CNR-Institute for Complex Systems – sequence: 8 givenname: B. Santos surname: Burgos fullname: Burgos, B. Santos organization: Elettra - Sincrotrone Trieste S.C.p.A – sequence: 9 givenname: T. O. surname: Menteş fullname: Menteş, T. O. organization: Elettra - Sincrotrone Trieste S.C.p.A – sequence: 10 givenname: A. surname: Locatelli fullname: Locatelli, A. organization: Elettra - Sincrotrone Trieste S.C.p.A – sequence: 11 givenname: A. surname: Baraldi fullname: Baraldi, A. organization: Physics Department and CENMAT, University of Trieste, IOM-CNR, Laboratorio TASC |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/23938361$$D View this record in MEDLINE/PubMed |
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| SubjectTerms | 639/301/357/537 639/301/357/918 639/301/357/918/1053 639/301/357/918/1055 Adhesiveness Adsorption Alloys - chemistry Carbon Chemical composition Crystallization - methods Graphene Graphite - chemistry Humanities and Social Sciences Hybridization Materials Testing Metal Nanoparticles - chemistry Metals Morphology multidisciplinary Science Surface Properties |
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| Title | Fine tuning of graphene-metal adhesion by surface alloying |
| URI | https://link.springer.com/article/10.1038/srep02430 https://www.ncbi.nlm.nih.gov/pubmed/23938361 https://www.proquest.com/docview/1897435205 https://www.proquest.com/docview/1420616087 https://pubmed.ncbi.nlm.nih.gov/PMC3741623 https://www.nature.com/articles/srep02430.pdf |
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