Detection of Rashba spin splitting in 2D organic-inorganic perovskite via precessional carrier spin relaxation

The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (e.g., Pb and I) makes these materials interesting for applications in spintronics. In conjunction with a lack of inversion symmetry associated with distortions of the metal-halide octa...

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Published inAPL materials Vol. 7; no. 8; pp. 81116 - 081116-8
Main Authors Todd, Seth B., Riley, Drew B., Binai-Motlagh, Ali, Clegg, Charlotte, Ramachandran, Ajan, March, Samuel A., Hoffman, Justin M., Hill, Ian G., Stoumpos, Constantinos C., Kanatzidis, Mercouri G., Yu, Zhi-Gang, Hall, Kimberley C.
Format Journal Article
LanguageEnglish
Published United States American Institute of Physics 01.08.2019
AIP Publishing LLC
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ISSN2166-532X
2166-532X
DOI10.1063/1.5099352

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Abstract The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (e.g., Pb and I) makes these materials interesting for applications in spintronics. In conjunction with a lack of inversion symmetry associated with distortions of the metal-halide octahedra, surfaces and interfaces, or the application of a bias, the Rashba effect (used in spin field-effect transistors and spin filters) has been predicted to be much larger in these materials than in traditional III-V semiconductors such as GaAs. Evidence of strong Rashba coupling has been observed in both 3D (bulk) and 2D perovskites, with the relative role of bulk and surface Rashba contributions in the former case under active debate. The varying size of the reported spin splittings points to the need for more experimental studies of Rashba effects in the organic-inorganic perovskite family of materials. Here, we apply time-resolved circular dichroism techniques to the study of carrier spin dynamics in a 2D perovskite thin film [(BA)2MAPb2I7; BA = CH3(CH2)3NH3, MA = CH3NH3]. Our findings confirm the presence of a Rashba spin splitting via the dominance of precessional spin relaxation induced by the Rashba effective magnetic field (also known as D’yakonov Perel spin relaxation). The size of the Rashba spin splitting in our system was extracted from simulations of the measured spin dynamics incorporating LO-phonon and electron-electron scattering, yielding a value of 10 meV at an electron energy of 50 meV above the band gap, representing a 20 times larger value than in GaAs quantum wells.
AbstractList The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (e.g., Pb and I) makes these materials interesting for applications in spintronics. In conjunction with a lack of inversion symmetry associated with distortions of the metal-halide octahedra, surfaces and interfaces, or the application of a bias, the Rashba effect (used in spin field-effect transistors and spin filters) has been predicted to be much larger in these materials than in traditional III-V semiconductors such as GaAs. Evidence of strong Rashba coupling has been observed in both 3D (bulk) and 2D perovskites, with the relative role of bulk and surface Rashba contributions in the former case under active debate. The varying size of the reported spin splittings points to the need for more experimental studies of Rashba effects in the organic-inorganic perovskite family of materials. Here, we apply time-resolved circular dichroism techniques to the study of carrier spin dynamics in a 2D perovskite thin film [(BA)2MAPb2I7; BA = CH3(CH2)3NH3, MA = CH3NH3]. Our findings confirm the presence of a Rashba spin splitting via the dominance of precessional spin relaxation induced by the Rashba effective magnetic field (also known as D’yakonov Perel spin relaxation). The size of the Rashba spin splitting in our system was extracted from simulations of the measured spin dynamics incorporating LO-phonon and electron-electron scattering, yielding a value of 10 meV at an electron energy of 50 meV above the band gap, representing a 20 times larger value than in GaAs quantum wells.
Author Ramachandran, Ajan
Stoumpos, Constantinos C.
March, Samuel A.
Hill, Ian G.
Todd, Seth B.
Hoffman, Justin M.
Kanatzidis, Mercouri G.
Yu, Zhi-Gang
Riley, Drew B.
Clegg, Charlotte
Hall, Kimberley C.
Binai-Motlagh, Ali
Author_xml – sequence: 1
  givenname: Seth B.
  surname: Todd
  fullname: Todd, Seth B.
  organization: Department of Physics and Atmospheric Science, Dalhousie University
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  surname: Clegg
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  organization: Department of Physics and Atmospheric Science, Dalhousie University
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  surname: Ramachandran
  fullname: Ramachandran, Ajan
  organization: Department of Physics and Atmospheric Science, Dalhousie University
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  organization: Department of Physics and Atmospheric Science, Dalhousie University
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  organization: Department of Chemistry, Northwestern University
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  givenname: Zhi-Gang
  surname: Yu
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  organization: Washington State University
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  givenname: Kimberley C.
  surname: Hall
  fullname: Hall, Kimberley C.
  organization: Department of Physics and Atmospheric Science, Dalhousie University
BackLink https://www.osti.gov/biblio/1567930$$D View this record in Osti.gov
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Snippet The strong spin-orbit interaction in the organic-inorganic perovskites tied to the incorporation of heavy elements (e.g., Pb and I) makes these materials...
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Title Detection of Rashba spin splitting in 2D organic-inorganic perovskite via precessional carrier spin relaxation
URI http://dx.doi.org/10.1063/1.5099352
https://www.osti.gov/biblio/1567930
https://doaj.org/article/7a1a974e4e09463aa69caf5449f5de71
Volume 7
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