A sulfur–microporous carbon composite positive electrode for lithium/sulfur and silicon/sulfur rechargeble batteries
Sulfur is an advantageous material as a promising next-generation positive electrode material for high-energy lithium batteries due to a high theoretical capacity of 1672 m A h g 1although its discharge potential is somewhat modest:ca.2 V vs Li/Lit.However,a sulfur positive electrode has some crucia...
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| Published in | Progress in natural science Vol. 25; no. 6; pp. 612 - 621 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.12.2015
Department of Chemistry and Materials Engineering, Faculty of Chemistry, Materials and Bioengineering, Kansai University, 3-3-35 Yamate-cho, Suita 564-8680,Japan |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1002-0071 |
| DOI | 10.1016/j.pnsc.2015.11.011 |
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| Abstract | Sulfur is an advantageous material as a promising next-generation positive electrode material for high-energy lithium batteries due to a high theoretical capacity of 1672 m A h g 1although its discharge potential is somewhat modest:ca.2 V vs Li/Lit.However,a sulfur positive electrode has some crucial problems for practical use,which are mainly attributed to the dissolution of its intermediate products in charge–discharge processes.In order to resolve the dissolution problem of lithium polysulfide,we attempted to synthesize a sulfur–microporous activated carbon(AC) composite positive electrode.Moreover,we have systematically researched the battery performance of sulfur–microporous AC positive electrode with variations of electrolytes as well as negative electrodes,and found its promising positive electrode performance for a nextgeneration rechargeable battery. |
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| AbstractList | Sulfur is an advantageous material as a promising next-generation positive electrode material for high-energy lithium batteries due to a high theoretical capacity of 1672mAhg−1 although its discharge potential is somewhat modest: ca. 2V vs Li/Li+. However, a sulfur positive electrode has some crucial problems for practical use, which are mainly attributed to the dissolution of its intermediate products in charge–discharge processes. In order to resolve the dissolution problem of lithium polysulfide, we attempted to synthesize a sulfur–microporous activated carbon (AC) composite positive electrode. Moreover, we have systematically researched the battery performance of sulfur–microporous AC positive electrode with variations of electrolytes as well as negative electrodes, and found its promising positive electrode performance for a next-generation rechargeable battery. Sulfur is an advantageous material as a promising next-generation positive electrode material for high-energy lithium batteries due to a high theoretical capacity of 1672 m A h g 1although its discharge potential is somewhat modest:ca.2 V vs Li/Lit.However,a sulfur positive electrode has some crucial problems for practical use,which are mainly attributed to the dissolution of its intermediate products in charge–discharge processes.In order to resolve the dissolution problem of lithium polysulfide,we attempted to synthesize a sulfur–microporous activated carbon(AC) composite positive electrode.Moreover,we have systematically researched the battery performance of sulfur–microporous AC positive electrode with variations of electrolytes as well as negative electrodes,and found its promising positive electrode performance for a nextgeneration rechargeable battery. |
| Author | Takuya Takahashi Masaki Yamagata Masashi Ishikawa |
| AuthorAffiliation | Department of Chemistry and Materials Engineering,Faculty of Chemistry,Materials and Bioengineering,Kansai University |
| AuthorAffiliation_xml | – name: Department of Chemistry and Materials Engineering, Faculty of Chemistry, Materials and Bioengineering, Kansai University, 3-3-35 Yamate-cho, Suita 564-8680,Japan |
| Author_xml | – sequence: 1 givenname: Takuya surname: Takahashi fullname: Takahashi, Takuya – sequence: 2 givenname: Masaki surname: Yamagata fullname: Yamagata, Masaki – sequence: 3 givenname: Masashi surname: Ishikawa fullname: Ishikawa, Masashi email: masaishi@kansai-u.ac.jp |
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| Keywords | Lithium-ion battery Silicon Micropore Sulfur Ionic liquid |
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| Notes | Takuya Takahashi;Masaki Yamagata;Masashi Ishikawa;Department of Chemistry and Materials Engineering,Faculty of Chemistry,Materials and Bioengineering,Kansai University 11-3853/N |
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| SubjectTerms | battery Ionic liquid liquid;Silicon;Lithium-ion Lithium-ion battery Micropore Silicon Sulfur Sulfur;Micropore;Ionic |
| Title | A sulfur–microporous carbon composite positive electrode for lithium/sulfur and silicon/sulfur rechargeble batteries |
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