Statistical comparison of leaching behavior of incineration bottom ash using seawater and deionized water: Significant findings based on several leaching methods
•Metal leaching statistically correlated to the leachant types, i.e., seawater or DI.•Metals with higher leached amounts with DI were subject to more effects by seawater.•Seawater tended to enhance most metal leaching in column leaching test.•Scenario-based leaching tests shall be established for IB...
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| Published in | Journal of hazardous materials Vol. 344; pp. 635 - 648 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Netherlands
Elsevier B.V
15.02.2018
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0304-3894 1873-3336 1873-3336 |
| DOI | 10.1016/j.jhazmat.2017.11.004 |
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| Abstract | •Metal leaching statistically correlated to the leachant types, i.e., seawater or DI.•Metals with higher leached amounts with DI were subject to more effects by seawater.•Seawater tended to enhance most metal leaching in column leaching test.•Scenario-based leaching tests shall be established for IBA application.
Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains elevated heavy metals posing a challenge for its free usage. Different leaching methods are developed to quantify leaching potential of incineration bottom ashes meanwhile guide its environmentally friendly application. Yet, there are diverse IBA applications while the in situ environment is always complicated, challenging its legislation. In this study, leaching tests were conveyed using batch and column leaching methods with seawater as opposed to deionized water, to unveil the metal leaching potential of IBA subjected to salty environment, which is commonly encountered when using IBA in land reclamation yet not well understood. Statistical analysis for different leaching methods suggested disparate performance between seawater and deionized water primarily ascribed to ionic strength. Impacts of leachant are metal-specific dependent on leaching methods and have a function of intrinsic characteristics of incineration bottom ashes. Leaching performances were further compared on additional perspectives, e.g. leaching approach and liquid to solid ratio, indicating sophisticated leaching potentials dominated by combined geochemistry. It is necessary to develop application-oriented leaching methods with corresponding leaching criteria to preclude discriminations between different applications, e.g., terrestrial applications vs. land reclamation. |
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| AbstractList | Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains elevated heavy metals posing a challenge for its free usage. Different leaching methods are developed to quantify leaching potential of incineration bottom ashes meanwhile guide its environmentally friendly application. Yet, there are diverse IBA applications while the in situ environment is always complicated, challenging its legislation. In this study, leaching tests were conveyed using batch and column leaching methods with seawater as opposed to deionized water, to unveil the metal leaching potential of IBA subjected to salty environment, which is commonly encountered when using IBA in land reclamation yet not well understood. Statistical analysis for different leaching methods suggested disparate performance between seawater and deionized water primarily ascribed to ionic strength. Impacts of leachant are metal-specific dependent on leaching methods and have a function of intrinsic characteristics of incineration bottom ashes. Leaching performances were further compared on additional perspectives, e.g. leaching approach and liquid to solid ratio, indicating sophisticated leaching potentials dominated by combined geochemistry. It is necessary to develop application-oriented leaching methods with corresponding leaching criteria to preclude discriminations between different applications, e.g., terrestrial applications vs. land reclamation. Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains elevated heavy metals posing a challenge for its free usage. Different leaching methods are developed to quantify leaching potential of incineration bottom ashes meanwhile guide its environmentally friendly application. Yet, there are diverse IBA applications while the in situ environment is always complicated, challenging its legislation. In this study, leaching tests were conveyed using batch and column leaching methods with seawater as opposed to deionized water, to unveil the metal leaching potential of IBA subjected to salty environment, which is commonly encountered when using IBA in land reclamation yet not well understood. Statistical analysis for different leaching methods suggested disparate performance between seawater and deionized water primarily ascribed to ionic strength. Impacts of leachant are metal-specific dependent on leaching methods and have a function of intrinsic characteristics of incineration bottom ashes. Leaching performances were further compared on additional perspectives, e.g. leaching approach and liquid to solid ratio, indicating sophisticated leaching potentials dominated by combined geochemistry. It is necessary to develop application-oriented leaching methods with corresponding leaching criteria to preclude discriminations between different applications, e.g., terrestrial applications vs. land reclamation.Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains elevated heavy metals posing a challenge for its free usage. Different leaching methods are developed to quantify leaching potential of incineration bottom ashes meanwhile guide its environmentally friendly application. Yet, there are diverse IBA applications while the in situ environment is always complicated, challenging its legislation. In this study, leaching tests were conveyed using batch and column leaching methods with seawater as opposed to deionized water, to unveil the metal leaching potential of IBA subjected to salty environment, which is commonly encountered when using IBA in land reclamation yet not well understood. Statistical analysis for different leaching methods suggested disparate performance between seawater and deionized water primarily ascribed to ionic strength. Impacts of leachant are metal-specific dependent on leaching methods and have a function of intrinsic characteristics of incineration bottom ashes. Leaching performances were further compared on additional perspectives, e.g. leaching approach and liquid to solid ratio, indicating sophisticated leaching potentials dominated by combined geochemistry. It is necessary to develop application-oriented leaching methods with corresponding leaching criteria to preclude discriminations between different applications, e.g., terrestrial applications vs. land reclamation. •Metal leaching statistically correlated to the leachant types, i.e., seawater or DI.•Metals with higher leached amounts with DI were subject to more effects by seawater.•Seawater tended to enhance most metal leaching in column leaching test.•Scenario-based leaching tests shall be established for IBA application. Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains elevated heavy metals posing a challenge for its free usage. Different leaching methods are developed to quantify leaching potential of incineration bottom ashes meanwhile guide its environmentally friendly application. Yet, there are diverse IBA applications while the in situ environment is always complicated, challenging its legislation. In this study, leaching tests were conveyed using batch and column leaching methods with seawater as opposed to deionized water, to unveil the metal leaching potential of IBA subjected to salty environment, which is commonly encountered when using IBA in land reclamation yet not well understood. Statistical analysis for different leaching methods suggested disparate performance between seawater and deionized water primarily ascribed to ionic strength. Impacts of leachant are metal-specific dependent on leaching methods and have a function of intrinsic characteristics of incineration bottom ashes. Leaching performances were further compared on additional perspectives, e.g. leaching approach and liquid to solid ratio, indicating sophisticated leaching potentials dominated by combined geochemistry. It is necessary to develop application-oriented leaching methods with corresponding leaching criteria to preclude discriminations between different applications, e.g., terrestrial applications vs. land reclamation. |
| Author | Dou, Xiaomin Chan, Wei-Ping Chang, Victor Wei-Chung Ren, Fei Yin, Ke |
| Author_xml | – sequence: 1 givenname: Ke surname: Yin fullname: Yin, Ke organization: Residue and Resource Reclamation Centre (R3C), Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Singapore – sequence: 2 givenname: Xiaomin surname: Dou fullname: Dou, Xiaomin organization: Residue and Resource Reclamation Centre (R3C), Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Singapore – sequence: 3 givenname: Fei surname: Ren fullname: Ren, Fei organization: Residue and Resource Reclamation Centre (R3C), Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Singapore – sequence: 4 givenname: Wei-Ping surname: Chan fullname: Chan, Wei-Ping email: wpchan@ntu.edu.sg, chan0378@e.ntu.edu.sg organization: Residue and Resource Reclamation Centre (R3C), Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Singapore – sequence: 5 givenname: Victor Wei-Chung surname: Chang fullname: Chang, Victor Wei-Chung organization: Residue and Resource Reclamation Centre (R3C), Nanyang Environment and Water Research Institute, Nanyang Technological University, 1 Cleantech Loop, CleanTech One, Singapore 637141, Singapore |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/29112922$$D View this record in MEDLINE/PubMed |
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| Snippet | •Metal leaching statistically correlated to the leachant types, i.e., seawater or DI.•Metals with higher leached amounts with DI were subject to more effects... Bottom ashes generated from municipal solid waste incineration have gained increasing popularity as alternative construction materials, however, they contains... |
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| SubjectTerms | bottom ash construction materials geochemistry heavy metals Incineration bottom ashes ionic strength land restoration laws and regulations leaching Leaching methods liquids Metal leaching municipal solid waste Seawater statistical analysis Utilization waste incineration |
| Title | Statistical comparison of leaching behavior of incineration bottom ash using seawater and deionized water: Significant findings based on several leaching methods |
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