Recyclable Graphene Sheets as a Growth Template for Crystalline ZnO Nanowires

Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly desirable for the recycling substrates. In this work, we report recycling of monolayer graphene as a growth template for synthesis of single...

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Published in	Nanomaterials (Basel, Switzerland) Vol. 11; no. 8; p. 2093
Main Authors	Kim, Yeonhoo, Kim, Dongheun, Auchter, Eric, Marquez, Justin, Tutchton, Roxanne, Li, Nan, Luk, Ting S., Dervishi, Enkeleda, Kim, Yong-Jin, Zhu, Jian-Xin, Yoo, Jinkyoung
Format	Journal Article
Language	English
Published	Basel MDPI AG 18.08.2021 MDPI
Subjects	chemistry Crystal structure Crystallinity Density functional theory Graphene hydrothermal synthesis MATERIALS SCIENCE Monolayers Nanocrystals Nanomaterials Nanotechnology Nanowires Nucleation Photovoltaic cells physics raman spectroscopy Recycling Scanning electron microscopy science & technology Spectrum analysis Substrates Thin films Two dimensional materials Zinc oxide ZnO United States > US
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ISSN	2079-4991 2079-4991
DOI	10.3390/nano11082093

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Abstract	Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly desirable for the recycling substrates. In this work, we report recycling of monolayer graphene as a growth template for synthesis of single crystalline ZnO nanowires. Selective nucleation of ZnO nanowires on graphene was elucidated by scanning electron microscopy and density functional theory calculation. Growth and subsequent separation of ZnO nanowires was repeated up to seven times on the same monolayer graphene film. Raman analyses were also performed to investigate the quality of graphene structure along the recycling processes. The chemical robustness of graphene enables the repetitive ZnO nanowire growth without noticeable degradation of the graphene quality. This work presents a route for graphene as a multifunctional growth template for diverse nanomaterials such as nanocrystals, aligned nanowires, other two-dimensional materials, and semiconductor thin films.
AbstractList	Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly desirable for the recycling substrates. In this work, we report recycling of monolayer graphene as a growth template for synthesis of single crystalline ZnO nanowires. Selective nucleation of ZnO nanowires on graphene was elucidated by scanning electron microscopy and density functional theory calculation. Growth and subsequent separation of ZnO nanowires was repeated up to seven times on the same monolayer graphene film. Raman analyses were also performed to investigate the quality of graphene structure along the recycling processes. The chemical robustness of graphene enables the repetitive ZnO nanowire growth without noticeable degradation of the graphene quality. This work presents a route for graphene as a multifunctional growth template for diverse nanomaterials such as nanocrystals, aligned nanowires, other two-dimensional materials, and semiconductor thin films. Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly desirable for the recycling substrates. In this work, we report recycling of monolayer graphene as a growth template for synthesis of single crystalline ZnO nanowires. Selective nucleation of ZnO nanowires on graphene was elucidated by scanning electron microscopy and density functional theory calculation. Growth and subsequent separation of ZnO nanowires was repeated up to seven times on the same monolayer graphene film. Raman analyses were also performed to investigate the quality of graphene structure along the recycling processes. The chemical robustness of graphene enables the repetitive ZnO nanowire growth without noticeable degradation of the graphene quality. This work presents a route for graphene as a multifunctional growth template for diverse nanomaterials such as nanocrystals, aligned nanowires, other two-dimensional materials, and semiconductor thin films.Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly desirable for the recycling substrates. In this work, we report recycling of monolayer graphene as a growth template for synthesis of single crystalline ZnO nanowires. Selective nucleation of ZnO nanowires on graphene was elucidated by scanning electron microscopy and density functional theory calculation. Growth and subsequent separation of ZnO nanowires was repeated up to seven times on the same monolayer graphene film. Raman analyses were also performed to investigate the quality of graphene structure along the recycling processes. The chemical robustness of graphene enables the repetitive ZnO nanowire growth without noticeable degradation of the graphene quality. This work presents a route for graphene as a multifunctional growth template for diverse nanomaterials such as nanocrystals, aligned nanowires, other two-dimensional materials, and semiconductor thin films.
Author	Kim, Yeonhoo Dervishi, Enkeleda Marquez, Justin Tutchton, Roxanne Luk, Ting S. Auchter, Eric Li, Nan Zhu, Jian-Xin Kim, Yong-Jin Yoo, Jinkyoung Kim, Dongheun
AuthorAffiliation	2 T-4, Los Alamos National Laboratory, Los Alamos, NM 87545, USA; rtutchton@lanl.gov (R.T.); jxzhu@lanl.gov (J.-X.Z.) 1 Center for Integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, NM 87545, USA; yeonhoo@lanl.gov (Y.K.); heun82@gmail.com (D.K.); elauchter@gmail.com (E.A.); jmarquezche@gmail.com (J.M.); nanli@lanl.gov (N.L.) 3 Center for Integrated Nanotechnologies, Sandia National Laboratories, Albuquerque, NM 87185, USA; tsluk@sandia.gov 4 SIGMA-2, Los Alamos National Laboratory, Los Alamos, NM 87545, USA 5 School of Physics and Astronomy, University of Manchester, Oxford Road, Manchester M13 9PL, UK; dibykim@gmail.com
AuthorAffiliation_xml	– name: 5 School of Physics and Astronomy, University of Manchester, Oxford Road, Manchester M13 9PL, UK; dibykim@gmail.com – name: 4 SIGMA-2, Los Alamos National Laboratory, Los Alamos, NM 87545, USA – name: 3 Center for Integrated Nanotechnologies, Sandia National Laboratories, Albuquerque, NM 87185, USA; tsluk@sandia.gov – name: 1 Center for Integrated Nanotechnologies, Los Alamos National Laboratory, Los Alamos, NM 87545, USA; yeonhoo@lanl.gov (Y.K.); heun82@gmail.com (D.K.); elauchter@gmail.com (E.A.); jmarquezche@gmail.com (J.M.); nanli@lanl.gov (N.L.) – name: 2 T-4, Los Alamos National Laboratory, Los Alamos, NM 87545, USA; rtutchton@lanl.gov (R.T.); jxzhu@lanl.gov (J.-X.Z.)
Author_xml	– sequence: 1 givenname: Yeonhoo surname: Kim fullname: Kim, Yeonhoo – sequence: 2 givenname: Dongheun surname: Kim fullname: Kim, Dongheun – sequence: 3 givenname: Eric surname: Auchter fullname: Auchter, Eric – sequence: 4 givenname: Justin surname: Marquez fullname: Marquez, Justin – sequence: 5 givenname: Roxanne orcidid: 0000-0001-8521-3504 surname: Tutchton fullname: Tutchton, Roxanne – sequence: 6 givenname: Nan surname: Li fullname: Li, Nan – sequence: 7 givenname: Ting S. surname: Luk fullname: Luk, Ting S. – sequence: 8 givenname: Enkeleda surname: Dervishi fullname: Dervishi, Enkeleda – sequence: 9 givenname: Yong-Jin surname: Kim fullname: Kim, Yong-Jin – sequence: 10 givenname: Jian-Xin surname: Zhu fullname: Zhu, Jian-Xin – sequence: 11 givenname: Jinkyoung orcidid: 0000-0002-9578-6979 surname: Yoo fullname: Yoo, Jinkyoung
BackLink	https://www.osti.gov/biblio/1813880$$D View this record in Osti.gov
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CitedBy_id	crossref_primary_10_1016_j_chemosphere_2022_137161
Cites_doi	10.1063/1.5001357 10.1038/ncomms5836 10.1088/1361-6528/aab4a4 10.1016/j.matlet.2012.09.089 10.1016/j.jallcom.2008.01.093 10.1021/acs.nanolett.7b00514 10.1016/j.surfcoat.2012.12.001 10.1021/nl904286r 10.1038/nature09054 10.1103/PhysRevLett.97.187401 10.1002/adma.200600200 10.1063/1.3266836 10.1063/1.4986780 10.1038/nature22053 10.1103/PhysRevB.29.793 10.1021/nl061702a 10.1039/C8NR08084D 10.1002/adma.201201966 10.1016/0038-1098(96)00340-7 10.1021/acsanm.0c01656 10.1063/1.116699 10.1007/s12274-011-0100-6 10.1088/0957-4484/19/31/315202 10.1021/acs.nanolett.6b01453 10.1103/PhysRevB.68.241312 10.1039/b816034a 10.1021/ja100329d 10.1088/0957-4484/24/30/305401 10.1039/C9NR05345J 10.1002/smll.201800240 10.1038/s41563-019-0341-4 10.1088/0957-4484/22/24/245603 10.1021/nl3018115 10.1002/adom.201400362 10.1021/nl204109t 10.1002/pssb.201600774 10.1021/nl201432g 10.1103/PhysRevB.64.075414
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Snippet	Recent advances in nanoscience have opened ways of recycling substrates for nanomaterial growth. Novel materials, such as atomically thin materials, are highly...
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SubjectTerms	chemistry Crystal structure Crystallinity Density functional theory Graphene hydrothermal synthesis MATERIALS SCIENCE Monolayers Nanocrystals Nanomaterials Nanotechnology Nanowires Nucleation Photovoltaic cells physics raman spectroscopy Recycling Scanning electron microscopy science & technology Spectrum analysis Substrates Thin films Two dimensional materials Zinc oxide ZnO
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Title	Recyclable Graphene Sheets as a Growth Template for Crystalline ZnO Nanowires
URI	https://www.proquest.com/docview/2565475841 https://www.proquest.com/docview/2566027780 https://www.osti.gov/biblio/1813880 https://pubmed.ncbi.nlm.nih.gov/PMC8399327 https://doaj.org/article/8bd200cdafe448fba976d380071e4efb
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