2D CoOOH Sheet-Encapsulated Ni2P into Tubular Arrays Realizing 1000 mA cm−2-Level-Current-Density Hydrogen Evolution Over 100 h in Neutral Water

Highlights The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was conceptually proposed. The designed electrocatalysts realize expectant 1000 mA cm −2 -level-current-density hydrogen evolution in...

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Published inNano-micro letters Vol. 12; no. 1; pp. 140 - 16
Main Authors Zhang, Shucong, Wang, Wenbin, Hu, Feilong, Mi, Yan, Wang, Shuzhe, Liu, Youwen, Ai, Xiaomeng, Fang, Jiakun, Li, Huiqiao, Zhai, Tianyou
Format Journal Article
LanguageEnglish
Published Singapore Springer Singapore 01.12.2020
Springer Nature B.V
SpringerOpen
Subjects
2D adaptive material
Arrays
Bubbles
Catalysis
Charge transfer
Convection
Current density
Electrocatalysts
Electrolysis
Electrolytes
Electronic structure
Encapsulation
Engineering
High current
Hydrogen
Hydrogen evolution
Interfacial charge modulation
Large-scale hydrogen production
Mass transfer
Mass transport
Multiscale coordinated regulation
Nanoscale Science and Technology
Nanotechnology
Nanotechnology and Microengineering
Porosity
Structural stability
Mass transport
Interfacial charge modulation
Multiscale coordinated regulation
2D adaptive material
Large-scale hydrogen production
Online AccessGet full text
ISSN2311-6706
2150-5551
2150-5551
DOI10.1007/s40820-020-00476-4

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Abstract Highlights The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was conceptually proposed. The designed electrocatalysts realize expectant 1000 mA cm −2 -level-current-density hydrogen evolution in neutral water for over 100 h. Water electrolysis at high current density (1000 mA cm −2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm −2 -level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
AbstractList Water electrolysis at high current density (1000 mA cm-2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm-2-level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.Water electrolysis at high current density (1000 mA cm-2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm-2-level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
HighlightsThe 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was conceptually proposed.The designed electrocatalysts realize expectant 1000 mA cm−2-level-current-density hydrogen evolution in neutral water for over 100 h.Water electrolysis at high current density (1000 mA cm−2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm−2-level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
Abstract Water electrolysis at high current density (1000 mA cm−2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm−2-level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
Highlights The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was conceptually proposed. The designed electrocatalysts realize expectant 1000 mA cm −2 -level-current-density hydrogen evolution in neutral water for over 100 h. Water electrolysis at high current density (1000 mA cm −2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm −2 -level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
Water electrolysis at high current density (1000 mA cm −2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm −2 -level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was conceptually proposed. The designed electrocatalysts realize expectant 1000 mA cm −2 -level-current-density hydrogen evolution in neutral water for over 100 h. Water electrolysis at high current density (1000 mA cm −2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green hydrogen from experiment to industrialization. In addition to the high intrinsic activity determined by the electronic structure, electrocatalysts are also required to be capable of fast mass transfer (electrolyte recharge and bubble overflow) and high mechanical stability. Herein, the 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system was proposed and realized 1000 mA cm −2 -level-current-density hydrogen evolution over 100 h in neutral water. In designed catalysts, 2D stack structure as an adaptive material can buffer the shock of electrolyte convection, hydrogen bubble rupture, and evolution through the release of stress, which insure the long cycle stability. Meanwhile, the rich porosity between stacked units contributed the good infiltration of electrolyte and slippage of hydrogen bubbles, guaranteeing electrolyte fast recharge and bubble evolution at the high-current catalysis. Beyond that, the electron structure modulation induced by interfacial charge transfer is also beneficial to enhance the intrinsic activity. Profoundly, the multiscale coordinated regulation will provide a guide to design high-efficiency industrial electrocatalysts.
ArticleNumber 140
Author Li, Huiqiao
Wang, Shuzhe
Fang, Jiakun
Liu, Youwen
Hu, Feilong
Zhang, Shucong
Ai, Xiaomeng
Zhai, Tianyou
Mi, Yan
Wang, Wenbin
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  organization: Guangxi Key Laboratory of Chemistry and Engineering of Forest Products, Guangxi University for Nationalities
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  email: miyan@gxun.edu.cn
  organization: Guangxi Key Laboratory of Chemistry and Engineering of Forest Products, Guangxi University for Nationalities, State Key Laboratory of Material Processing and Die and Mould Technology, and School of Materials Science and Engineering, Huazhong University of Science and Technology
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  email: ywliu@hust.edu.cn
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Issue 1
Keywords Mass transport
Interfacial charge modulation
Multiscale coordinated regulation
2D adaptive material
Large-scale hydrogen production
Language English
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Snippet Highlights The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned...
Water electrolysis at high current density (1000 mA cm −2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green...
HighlightsThe 2D CoOOH sheet-encapsulated Ni2P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned...
Water electrolysis at high current density (1000 mA cm-2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for green...
The 2D CoOOH sheet-encapsulated Ni 2 P into tubular arrays electrocatalytic system with expediting mass transport, structural stability, and tuned electron was...
Abstract Water electrolysis at high current density (1000 mA cm−2 level) with excellent durability especially in neutral electrolyte is the pivotal issue for...
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SubjectTerms 2D adaptive material
Arrays
Bubbles
Catalysis
Charge transfer
Convection
Current density
Electrocatalysts
Electrolysis
Electrolytes
Electronic structure
Encapsulation
Engineering
High current
Hydrogen
Hydrogen evolution
Interfacial charge modulation
Large-scale hydrogen production
Mass transfer
Mass transport
Multiscale coordinated regulation
Nanoscale Science and Technology
Nanotechnology
Nanotechnology and Microengineering
Porosity
Structural stability
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Title 2D CoOOH Sheet-Encapsulated Ni2P into Tubular Arrays Realizing 1000 mA cm−2-Level-Current-Density Hydrogen Evolution Over 100 h in Neutral Water
URI https://link.springer.com/article/10.1007/s40820-020-00476-4
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