A Review of Modeling of Diffusion Controlled Polymerization Reactions
A plethora of models have been developed quantifying the effect of diffusion‐controlled phenomena on polymerization reactions. The most prominent approaches are reviewed here, including innovative ones that have emerged over the last decade. Free‐radical and step‐growth polymerizations are considere...
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| Published in | Macromolecular theory and simulations Vol. 16; no. 4; pp. 319 - 347 |
|---|---|
| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Weinheim
WILEY-VCH Verlag
25.05.2007
WILEY‐VCH Verlag Wiley |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1022-1344 1521-3919 |
| DOI | 10.1002/mats.200700003 |
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| Abstract | A plethora of models have been developed quantifying the effect of diffusion‐controlled phenomena on polymerization reactions. The most prominent approaches are reviewed here, including innovative ones that have emerged over the last decade. Free‐radical and step‐growth polymerizations are considered in a way to show that similar models have been used in both mechanisms. In free‐radical polymerization the models proposed are subdivided according to their theoretical background into four categories: (i) based on a Fickian description of reactant diffusion; (ii) free‐volume theory based; (iii) chain‐length dependent; and, (iv) empirical. The reversible addition‐fragmentation technique is discussed, together with two industrially important case‐studies, solid state polycondensation and epoxy‐amine curing. |
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| AbstractList | A plethora of models have been developed quantifying the effect of diffusion-controlled phenomena on polymerization reactions. The most prominent approaches are reviewed here, including innovative ones that have emerged over the last decade. Free-radical and step-growth polymerizations are considered in a way to show that similar models have been used in both mechanisms. In free-radical polymerization the models proposed are subdivided according to their theoretical background into four categories: (i) based on a Fickian description of reactant diffusion; (ii) free-volume theory based; (iii) chain-length dependent; and, (iv) empirical. The reversible addition-fragmentation technique is discussed, together with two industrially important case-studies, solid state polycondensation and epoxy-amine curing. A plethora of models have been developed quantifying the effect of diffusion‐controlled phenomena on polymerization reactions. The most prominent approaches are reviewed here, including innovative ones that have emerged over the last decade. Free‐radical and step‐growth polymerizations are considered in a way to show that similar models have been used in both mechanisms. In free‐radical polymerization the models proposed are subdivided according to their theoretical background into four categories: (i) based on a Fickian description of reactant diffusion; (ii) free‐volume theory based; (iii) chain‐length dependent; and, (iv) empirical. The reversible addition‐fragmentation technique is discussed, together with two industrially important case‐studies, solid state polycondensation and epoxy‐amine curing. magnified image |
| Author | Achilias, Dimitris S. |
| Author_xml | – sequence: 1 givenname: Dimitris S. surname: Achilias fullname: Achilias, Dimitris S. email: axilias@chem.auth.gr organization: Laboratory of Organic Chemical Technology, Department of Chemistry, Aristotle University of Thessaloniki, GR-541 24 Thessaloniki, Greece |
| BackLink | http://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=18826720$$DView record in Pascal Francis |
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| Copyright | Copyright © 2007 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim 2007 INIST-CNRS |
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| Issue | 4 |
| Keywords | Epoxy resin Condensation polymerization Review Modeling Chemical reaction kinetics Diamine Kinetic model Free radical polymerization Diffusion-controlled reactions Curing(plastics) free-radical step-growth Solid state reaction |
| Language | English |
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| PublicationDate | May 25, 2007 |
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| PublicationPlace | Weinheim |
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| PublicationTitle | Macromolecular theory and simulations |
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| Publisher | WILEY-VCH Verlag WILEY‐VCH Verlag Wiley |
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| Snippet | A plethora of models have been developed quantifying the effect of diffusion‐controlled phenomena on polymerization reactions. The most prominent approaches... A plethora of models have been developed quantifying the effect of diffusion-controlled phenomena on polymerization reactions. The most prominent approaches... |
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| SubjectTerms | Applied sciences Diffusion-controlled reactions Exact sciences and technology free-radical modeling Organic polymers Physicochemistry of polymers Polycondensation Polymerization Preparation, kinetics, thermodynamics, mechanism and catalysts step-growth |
| Title | A Review of Modeling of Diffusion Controlled Polymerization Reactions |
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