Pervaporation of Aqueous Solution of Acetaldehyde Through ZSM-5 Filled PDMS Composite Membrane
Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane （PDMS） composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray...
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| Published in | Chinese journal of chemical engineering Vol. 20; no. 4; pp. 625 - 632 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.08.2012
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(11)60227-9 |
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| Abstract | Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane （PDMS） composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25℃, |
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| AbstractList | Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane (PDMS) composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25°C, suggesting that the membranes have stronger sorption capacity in acetaldehyde solution. The effects of ZSM-5 filling content and acetaldehyde concentration on pervaporation performance of composite membranes were investigated. The permeation experiments at different temperatures showed that both selectivity and permeation flux of composite membranes increased with temperature. With 5%ZSM-5-PDMS/Nylon membrane at acetaldehyde mass concentration of 8% and 25°C, the separation factor of acetaldehyde/water achieved 35 and the permeation flux was 233.3 g·m−2·h−1. Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane （PDMS） composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25℃, Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane (PDMS) composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25ADGC, suggesting that the membranes have stronger sorption capacity in acetaldehyde solution. The effects of ZSM-5 filling content and acetaldehyde concentration on pervaporation performance of composite membranes were investigated. The permeation experiments at different temperatures showed that both selectivity and permeation flux of composite membranes increased with temperature. With 5%ZSM-5-PDMS/Nylon membrane at acetaldehyde mass concentration of 8% and 25ADGC, the separation factor of acetaldehyde/water achieved 35 and the permeation flux was 233.3 gADTma2ADTha1. Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane (PDMS) composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25 degree C, suggesting that the membranes have stronger sorption capacity in acetaldehyde solution. The effects of ZSM-5 filling content and acetaldehyde concentration on pervaporation performance of composite membranes were investigated. The permeation experiments at different temperatures showed that both selectivity and permeation flux of composite membranes increased with temperature. With 5%ZSM-5-PDMS/Nylon membrane at acetaldehyde mass concentration of 8% and 25 degree C, the separation factor of acetaldehyde/water achieved 35 and the permeation flux was 233.3 gADTm-2ADTh-1. |
| Author | 伍艳辉 谭惠芬 李佟茗 金源 |
| AuthorAffiliation | Department of Chemistry, Tongji University, Shanghai 200092, China |
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| CitedBy_id | crossref_primary_10_1080_03602559_2018_1471712 crossref_primary_10_1002_app_49611 crossref_primary_10_1016_j_memsci_2013_11_010 crossref_primary_10_3390_su14116540 crossref_primary_10_3390_membranes12111040 crossref_primary_10_1016_j_mcat_2017_09_014 crossref_primary_10_3390_polym15183777 crossref_primary_10_1016_j_jece_2022_108317 crossref_primary_10_1016_j_memsci_2019_03_049 crossref_primary_10_3390_polym14091680 crossref_primary_10_1016_j_psep_2020_07_001 |
| Cites_doi | 10.1016/j.seppur.2007.09.012 10.1006/jcis.1999.6654 10.1016/0144-2449(95)96829-P 10.1016/j.desal.2007.11.085 10.1080/01496390903018103 10.1016/0009-2797(95)03632-V 10.1002/ceat.200800252 10.1016/j.seppur.2007.04.001 10.1016/j.cej.2007.05.002 10.1016/j.seppur.2005.07.029 10.1016/j.alcohol.2004.01.005 10.1080/01496395.2010.527896 10.1002/app.21566 10.1016/0376-7388(95)00319-3 10.1016/S0021-9673(02)01146-9 10.1016/j.chroma.2006.06.031 10.1016/0003-2670(96)00171-7 10.1016/j.memsci.2007.04.007 |
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| Keywords | polydimethylsiloxane membrane acetaldehyde ZSM-5 pervaporation |
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| Notes | Hydrophobic ZSM-5 zeolite filled polydimethylsiloxane （PDMS） composite membranes with Nylon micro-filtration membrane as the support layer were prepared to separate acetaldehyde from its aqueous solution. The composite membranes were characterized by Fourier transform infrared spectroscopy and X-ray diffraction. Their structural morphology and thermal stability were also examined. The swelling study showed that the composite membranes presented higher degree of swelling in aqueous solution of acetaldehyde than in pure water at 25 WU Yanhui, TAN Huifen , LI Dongming and JIN Yuan Department of Chemistry, Tongji University, Shanghai 200092, China pervaporation, acetaldehyde, polydimethylsiloxane membrane, Z5M-5 11-3270/TQ ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-1 content type line 23 ObjectType-Article-1 ObjectType-Feature-2 |
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| SubjectTerms | Acetaldehyde Aqueous solutions Flux Membranes Nylons PDMS复合膜 Penetration Permeation pervaporation polydimethylsiloxane membrane Silicone resins ZSM-5 ZSM-5沸石 乙醛 傅里叶变换红外光谱 填充 水溶液 渗透汽化 聚二甲基硅氧烷 |
| Title | Pervaporation of Aqueous Solution of Acetaldehyde Through ZSM-5 Filled PDMS Composite Membrane |
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