Steam Reforming of Dimethyl Ether by Gliding Arc Gas Discharge Plasma for Hydrogen Production
Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether （DME）. A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly w...
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| Published in | Chinese journal of chemical engineering Vol. 22; no. 1; pp. 104 - 112 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(14)60020-3 |
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| Abstract | Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether （DME）. A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml. min^-1. Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H2- Among the five electrodes, electrode 2# with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. |
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| AbstractList | Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether (DME). A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml[middot]min super(-1). Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H sub(2). Among the five electrodes, electrode 2 super(#) with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether (DME). A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml·min−1. Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H2. Among the five electrodes, electrode 2# with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether (DME). A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml.min-1. Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H2. Among the five electrodes, electrode 2# with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether （DME）. A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml. min^-1. Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H2- Among the five electrodes, electrode 2# with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. |
| Author | 王保伟 孙启梅 吕一军 杨美琳 闫文娟 |
| AuthorAffiliation | Key Laboratory for Green Chemical Technology, School of Chemical Engineering Technology, Tianjin University,Tianjin 300072, China |
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| CitedBy_id | crossref_primary_10_1016_j_cjche_2022_03_002 crossref_primary_10_1007_s40201_019_00369_8 crossref_primary_10_1016_j_jcou_2018_12_019 crossref_primary_10_1007_s11705_019_1811_6 crossref_primary_10_1016_j_apenergy_2016_01_092 crossref_primary_10_1016_j_ijhydene_2019_07_042 crossref_primary_10_4236_jpee_2016_45004 crossref_primary_10_1016_j_cjche_2018_01_006 |
| Cites_doi | 10.1088/0963-0252/16/4/014 10.1021/ef060098o 10.1016/j.cej.2009.10.009 10.1016/S1003-9953(08)60140-1 10.1021/ie101920n 10.1016/j.ijhydene.2006.09.023 10.1016/j.ijhydene.2006.07.013 10.1016/S1872-5813(10)60030-8 10.1016/j.energy.2008.11.006 10.1016/j.ijhydene.2008.05.101 10.1007/s10562-005-5855-5 10.1016/j.jpowsour.2006.02.078 10.1016/j.ijhydene.2008.07.090 10.1016/j.cattod.2009.09.019 10.1016/j.jpowsour.2005.05.082 10.1016/j.surfcoat.2008.06.076 10.1007/s11144-007-5082-8 10.1021/jp905082s 10.1016/j.fuel.2009.11.039 10.1016/j.cattod.2009.01.026 10.1016/j.apcata.2006.02.021 10.1063/1.367003 10.1016/j.surfcoat.2011.01.061 10.1016/j.apcatb.2010.11.011 |
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| Keywords | dimethyl ether gliding arc gas discharge steam reforming hydrogen production |
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| Notes | WANG Baowei, SUN Qimei , LU Yijun, YANG Meilin and YAN Wenjuan Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether （DME）. A systemic procedure was employed to determine the suitable experimental conditions. It was found that DME conversion first increased up to the maximum and then decreased slightly with the increase of added water and air. The increase of total feed gas flow rate resulted in the decrease of DME conversion and hydrogen yield, but hydrogen energy consumption dropped down to the lowest as total feed gas flow rate increased to 76 ml. min^-1. Larger electrode gap and higher discharge voltage were advantageous. Electrode shape had an important effect on the conversion of DME and production of H2- Among the five electrodes, electrode 2# with valid length of 55 mm and the radian of 34 degrees of the top electrode section was the best option, which enhanced obviously the conversion of DME. 11-3270/TQ dimethyl ether; steam reforming; hydrogen production; gliding arc gas discharge ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-1 content type line 23 ObjectType-Article-1 ObjectType-Feature-2 |
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| Snippet | Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether （DME）. A systemic procedure was employed to... Gliding arc gas discharge plasma was used for the generation of hydrogen from steam reforming of dimethyl ether (DME). A systemic procedure was employed to... |
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| SubjectTerms | Conversion Dimethyl ether Electric arcs Electrodes Gas discharges Gas flow Gliding gliding arc gas discharge hydrogen production Reforming steam reforming 二甲醚 制氢 放电等离子体 气体 水蒸气重整 滑动弧 电极间隙 进气流量 |
| Title | Steam Reforming of Dimethyl Ether by Gliding Arc Gas Discharge Plasma for Hydrogen Production |
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