Enhancement of Photoluminescence Properties via Polymer Infiltration in a Colloidal Photonic Glass
Photonic glasses (PGs) based on the self-assembly of monosized nanoparticles can be an effective tool for realizing disordered structures capable of tailoring light diffusion due to the establishment of Mie resonances. In particular, the wavelength position of these resonances depends mainly on the...
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| Published in | Molecules Vol. 29; no. 3; p. 654 |
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| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Switzerland
MDPI AG
30.01.2024
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| Online Access | Get full text |
| ISSN | 1420-3049 1433-1373 1420-3049 1433-1373 |
| DOI | 10.3390/molecules29030654 |
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| Abstract | Photonic glasses (PGs) based on the self-assembly of monosized nanoparticles can be an effective tool for realizing disordered structures capable of tailoring light diffusion due to the establishment of Mie resonances. In particular, the wavelength position of these resonances depends mainly on the morphology (dimension) and optical properties (refractive index) of the building blocks. In this study, we report the fabrication and optical characterization of photonic glasses obtained via a self-assembling technique. Furthermore, we have demonstrated that the infiltration of these systems with a green-emitting polymer enhances the properties of the polymer, resulting in a large increase in its photoluminescence quantum yield and a 3 ps growing time of the photoluminescence time decay Finally, the development of the aforementioned system can serve as a suitable low-cost platform for the realization of lasers and fluorescence-based bio-sensors. |
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| AbstractList | Photonic glasses (PGs) based on the self-assembly of monosized nanoparticles can be an effective tool for realizing disordered structures capable of tailoring light diffusion due to the establishment of Mie resonances. In particular, the wavelength position of these resonances depends mainly on the morphology (dimension) and optical properties (refractive index) of the building blocks. In this study, we report the fabrication and optical characterization of photonic glasses obtained via a self-assembling technique. Furthermore, we have demonstrated that the infiltration of these systems with a green-emitting polymer enhances the properties of the polymer, resulting in a large increase in its photoluminescence quantum yield and a 3 ps growing time of the photoluminescence time decay Finally, the development of the aforementioned system can serve as a suitable low-cost platform for the realization of lasers and fluorescence-based bio-sensors. Photonic glasses (PGs) based on the self-assembly of monosized nanoparticles can be an effective tool for realizing disordered structures capable of tailoring light diffusion due to the establishment of Mie resonances. In particular, the wavelength position of these resonances depends mainly on the morphology (dimension) and optical properties (refractive index) of the building blocks. In this study, we report the fabrication and optical characterization of photonic glasses obtained via a self-assembling technique. Furthermore, we have demonstrated that the infiltration of these systems with a green-emitting polymer enhances the properties of the polymer, resulting in a large increase in its photoluminescence quantum yield and a 3 ps growing time of the photoluminescence time decay Finally, the development of the aforementioned system can serve as a suitable low-cost platform for the realization of lasers and fluorescence-based bio-sensors.Photonic glasses (PGs) based on the self-assembly of monosized nanoparticles can be an effective tool for realizing disordered structures capable of tailoring light diffusion due to the establishment of Mie resonances. In particular, the wavelength position of these resonances depends mainly on the morphology (dimension) and optical properties (refractive index) of the building blocks. In this study, we report the fabrication and optical characterization of photonic glasses obtained via a self-assembling technique. Furthermore, we have demonstrated that the infiltration of these systems with a green-emitting polymer enhances the properties of the polymer, resulting in a large increase in its photoluminescence quantum yield and a 3 ps growing time of the photoluminescence time decay Finally, the development of the aforementioned system can serve as a suitable low-cost platform for the realization of lasers and fluorescence-based bio-sensors. |
| Audience | Academic |
| Author | D’Andrea, Cosimo Scavia, Guido Faccialà, Davide Chiappini, Andrea Novikova, Nina I. Virgili, Tersilla Botta, Chiara Sardar, Samim |
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| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/38338398$$D View this record in MEDLINE/PubMed |
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| Cites_doi | 10.1021/acsami.0c05449 10.1039/c1cp21826c 10.3390/s23031433 10.1364/OE.19.011623 10.1103/PhysRevB.77.235404 10.1038/srep27264 10.1016/j.optmat.2019.02.039 10.1039/c3tc30704b 10.1063/5.0006203 10.1038/nature03376 10.1038/srep07636 10.1002/adma.201803362 10.1016/j.talanta.2023.125154 10.1038/am.2016.156 10.1038/s41377-022-01021-1 10.1016/j.dyepig.2022.110589 10.1007/s11172-022-3627-7 10.1021/acs.chemrev.6b00172 10.1002/adma.200602426 10.1016/j.nantod.2018.08.008 10.1364/OE.18.007101 10.1016/j.jnoncrysol.2009.01.054 10.1021/acsnano.2c07756 10.1021/acs.chemmater.9b00307 10.1038/s41598-018-26119-8 10.1103/PhysRevA.80.013833 10.1063/1.1576906 10.1080/00107510410001676795 10.1038/asiamat.2010.192 10.3390/mi11030290 10.1002/adom.202202370 10.1126/science.281.5378.802 10.1038/35013024 10.1103/PhysRevA.78.023823 10.1002/cphc.200800682 |
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| SubjectTerms | Crystals F8BT Fourier transforms Glass substrates Light Morphology Nanoparticles optical features Optical properties Photoluminescence photoluminescence properties photonic glasses Polymers quantum yield Scanning electron microscopy Sensors Spheres Thin films |
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| Title | Enhancement of Photoluminescence Properties via Polymer Infiltration in a Colloidal Photonic Glass |
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