Enhanced removal of uranium(VI) from aqueous solution by a novel Mg-MOF-74-derived porous MgO/carbon adsorbent
[Display omitted] The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) remova...
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| Published in | Journal of colloid and interface science Vol. 537; pp. A1 - A10 |
|---|---|
| Main Authors | , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
United States
Elsevier Inc
01.03.2019
|
| Subjects | |
| Online Access | Get full text |
| ISSN | 0021-9797 1095-7103 1095-7103 |
| DOI | 10.1016/j.jcis.2018.11.062 |
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| Abstract | [Display omitted]
The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) removal from aqueous solution. Characteristic results indicated that the as-prepared composite was a typical porous structure. The adsorption performance of the MgO/carbon towards U(VI) was studied by batch experiments. The results indicated that the MgO/carbon can rapidly and effectively remove U(VI) and showed an excellent adsorption capacity (777.51 mg/g), which is much higher than other reported adsorbent materials. In addition, the intraparticle diffusion model provides a good explanation for each adsorption process. The adsorption capacity of the MgO/carbon towards U(VI) is greatly promoted by the large specific surface area and well-defined porous structure. Based on the zeta potential and XPS analysis, the possible mechanism for U(VI) removal involved the surface complexation and electrostatic attraction. The results indicate that the MgO/carbon can be regarded as an efficient adsorbent for U(VI) removal from wastewater, which has a very broad application prospect. |
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| AbstractList | The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) removal from aqueous solution. Characteristic results indicated that the as-prepared composite was a typical porous structure. The adsorption performance of the MgO/carbon towards U(VI) was studied by batch experiments. The results indicated that the MgO/carbon can rapidly and effectively remove U(VI) and showed an excellent adsorption capacity (777.51 mg/g), which is much higher than other reported adsorbent materials. In addition, the intraparticle diffusion model provides a good explanation for each adsorption process. The adsorption capacity of the MgO/carbon towards U(VI) is greatly promoted by the large specific surface area and well-defined porous structure. Based on the zeta potential and XPS analysis, the possible mechanism for U(VI) removal involved the surface complexation and electrostatic attraction. The results indicate that the MgO/carbon can be regarded as an efficient adsorbent for U(VI) removal from wastewater, which has a very broad application prospect.The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) removal from aqueous solution. Characteristic results indicated that the as-prepared composite was a typical porous structure. The adsorption performance of the MgO/carbon towards U(VI) was studied by batch experiments. The results indicated that the MgO/carbon can rapidly and effectively remove U(VI) and showed an excellent adsorption capacity (777.51 mg/g), which is much higher than other reported adsorbent materials. In addition, the intraparticle diffusion model provides a good explanation for each adsorption process. The adsorption capacity of the MgO/carbon towards U(VI) is greatly promoted by the large specific surface area and well-defined porous structure. Based on the zeta potential and XPS analysis, the possible mechanism for U(VI) removal involved the surface complexation and electrostatic attraction. The results indicate that the MgO/carbon can be regarded as an efficient adsorbent for U(VI) removal from wastewater, which has a very broad application prospect. The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) removal from aqueous solution. Characteristic results indicated that the as-prepared composite was a typical porous structure. The adsorption performance of the MgO/carbon towards U(VI) was studied by batch experiments. The results indicated that the MgO/carbon can rapidly and effectively remove U(VI) and showed an excellent adsorption capacity (777.51 mg/g), which is much higher than other reported adsorbent materials. In addition, the intraparticle diffusion model provides a good explanation for each adsorption process. The adsorption capacity of the MgO/carbon towards U(VI) is greatly promoted by the large specific surface area and well-defined porous structure. Based on the zeta potential and XPS analysis, the possible mechanism for U(VI) removal involved the surface complexation and electrostatic attraction. The results indicate that the MgO/carbon can be regarded as an efficient adsorbent for U(VI) removal from wastewater, which has a very broad application prospect. [Display omitted] The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry. In this work, a MgO/carbon adsorbent was successfully prepared by one-step Mg-MOF-74 pyrolyzation and used for U(VI) removal from aqueous solution. Characteristic results indicated that the as-prepared composite was a typical porous structure. The adsorption performance of the MgO/carbon towards U(VI) was studied by batch experiments. The results indicated that the MgO/carbon can rapidly and effectively remove U(VI) and showed an excellent adsorption capacity (777.51 mg/g), which is much higher than other reported adsorbent materials. In addition, the intraparticle diffusion model provides a good explanation for each adsorption process. The adsorption capacity of the MgO/carbon towards U(VI) is greatly promoted by the large specific surface area and well-defined porous structure. Based on the zeta potential and XPS analysis, the possible mechanism for U(VI) removal involved the surface complexation and electrostatic attraction. The results indicate that the MgO/carbon can be regarded as an efficient adsorbent for U(VI) removal from wastewater, which has a very broad application prospect. |
| Author | Wang, Haiyan Lv, Zhimin Chen, Lei Chen, Changlun Yang, Shimin Alsaedi, Ahmed Hayat, Tasawar |
| Author_xml | – sequence: 1 givenname: Zhimin surname: Lv fullname: Lv, Zhimin organization: College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, PR China – sequence: 2 givenname: Haiyan surname: Wang fullname: Wang, Haiyan organization: Institute of Physical Science and Information Technology, Anhui University, Hefei 230601, Anhui, PR China – sequence: 3 givenname: Changlun orcidid: 0000-0003-1636-2412 surname: Chen fullname: Chen, Changlun email: clchen@ipp.ac.cn organization: College of Environmental Science and Engineering, North China Electric Power University, Beijing 102206, PR China – sequence: 4 givenname: Shimin surname: Yang fullname: Yang, Shimin organization: School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255049, Shandong, PR China – sequence: 5 givenname: Lei surname: Chen fullname: Chen, Lei organization: School of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo 255049, Shandong, PR China – sequence: 6 givenname: Ahmed surname: Alsaedi fullname: Alsaedi, Ahmed organization: NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia – sequence: 7 givenname: Tasawar surname: Hayat fullname: Hayat, Tasawar organization: NAAM Research Group, Faculty of Science, King Abdulaziz University, Jeddah 21589, Saudi Arabia |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/30459090$$D View this record in MEDLINE/PubMed |
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The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the... The elimination and safe treatment of U(VI) from radioactive wastewater has attracted widespread attention with the development of the nuclear power industry.... |
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| SubjectTerms | adsorbents Adsorption aqueous solutions carbon electrostatic interactions magnesium oxide MgO/carbon nuclear power industry Porous structure surface area U(VI) uranium wastewater X-ray photoelectron spectroscopy zeta potential |
| Title | Enhanced removal of uranium(VI) from aqueous solution by a novel Mg-MOF-74-derived porous MgO/carbon adsorbent |
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