Lignin-based electrospun carbon nanofibrous webs as free-standing and binder-free electrodes for sodium ion batteries
Low-cost and bio-based carbon nanofibrous webs (PL-CNFs) are fabricated from polyacrylonitrile (PAN) - refined lignin (RL) which is extracted from hardwood lignosulfonate via simple eletrospinning followed by stabilization and carbonization. The effects of the PAN/RL mass ratios varying from 9/1,7/3...
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| Published in | Journal of power sources Vol. 272; pp. 800 - 807 |
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| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Amsterdam
Elsevier
25.12.2014
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0378-7753 |
| DOI | 10.1016/j.jpowsour.2014.08.119 |
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| Abstract | Low-cost and bio-based carbon nanofibrous webs (PL-CNFs) are fabricated from polyacrylonitrile (PAN) - refined lignin (RL) which is extracted from hardwood lignosulfonate via simple eletrospinning followed by stabilization and carbonization. The effects of the PAN/RL mass ratios varying from 9/1,7/3 to 5/5 and heat-treatment temperatures (HTTs) in the range from 800,1000 to 1300 [degrees]C on morphology and structure of PL-CNFs are systematically studied. Due to unique morphology and weakly ordered turbostratic microstructure of the 3-D conductive composite networks, the PL-CNFs anode obtained at 1300 [degrees]C with a mass ratio of 5/5 exhibits a high reversible capacity of 292.6 mA h g super(-1) with an initial efficiency of 70.5% at a constant current density of 0.02 A g super(-1) when used as free-standing and binder-free anodes for sodium ion batteries (SIBs). The anode also presents high rate capability (210 and 80 mA h g super(-1) at 0.4 and 1 A g super(-1), respectively) and excellent cycle stability (247 mA h g super(-1) reversible capacity with 90.2% capacity retention ratio at 0.1 A g super(-1) over 200 cycles). It is demonstrated that biomass waste lignin can be applied as a promising precursor to fabricate low-cost-high performance carbon electrode materials for SIBs. |
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| AbstractList | Low-cost and bio-based carbon nanofibrous webs (PL-CNFs) are fabricated from polyacrylonitrile (PAN) - refined lignin (RL) which is extracted from hardwood lignosulfonate via simple eletrospinning followed by stabilization and carbonization. The effects of the PAN/RL mass ratios varying from 9/1,7/3 to 5/5 and heat-treatment temperatures (HTTs) in the range from 800,1000 to 1300 [degrees]C on morphology and structure of PL-CNFs are systematically studied. Due to unique morphology and weakly ordered turbostratic microstructure of the 3-D conductive composite networks, the PL-CNFs anode obtained at 1300 [degrees]C with a mass ratio of 5/5 exhibits a high reversible capacity of 292.6 mA h g super(-1) with an initial efficiency of 70.5% at a constant current density of 0.02 A g super(-1) when used as free-standing and binder-free anodes for sodium ion batteries (SIBs). The anode also presents high rate capability (210 and 80 mA h g super(-1) at 0.4 and 1 A g super(-1), respectively) and excellent cycle stability (247 mA h g super(-1) reversible capacity with 90.2% capacity retention ratio at 0.1 A g super(-1) over 200 cycles). It is demonstrated that biomass waste lignin can be applied as a promising precursor to fabricate low-cost-high performance carbon electrode materials for SIBs. |
| Author | Yu, Bao-jun Wang, Cheng-yang Chong, Chuan-bin Jin, Juan Shi, Zhi-qiang |
| Author_xml | – sequence: 1 givenname: Juan surname: Jin fullname: Jin, Juan – sequence: 2 givenname: Bao-jun surname: Yu fullname: Yu, Bao-jun – sequence: 3 givenname: Zhi-qiang surname: Shi fullname: Shi, Zhi-qiang – sequence: 4 givenname: Cheng-yang surname: Wang fullname: Wang, Cheng-yang – sequence: 5 givenname: Chuan-bin surname: Chong fullname: Chong, Chuan-bin |
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| Keywords | Electrodes Lignin Sodium-ion battery Electrospinning Free-standing film Carbon nanofibers Secondary cell Nanostructure Sodium ion batteries Carbon Lignosulfonate Carbon fiber |
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| SubjectTerms | Anodes Applied sciences Carbon Direct energy conversion and energy accumulation Electric batteries Electrical engineering. Electrical power engineering Electrical power engineering Electrochemical conversion: primary and secondary batteries, fuel cells Exact sciences and technology Heat treatment Morphology Nanostructure Sodium Webs |
| Title | Lignin-based electrospun carbon nanofibrous webs as free-standing and binder-free electrodes for sodium ion batteries |
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