Tin Halide Perovskites: Progress and Challenges

The chemical composition engineering of lead halide perovskites via a partial or complete replacement of toxic Pb with tin has been widely reported as a feasible process due to the suitable ionic radius of Sn and its possibility of existing in the +2 state. Interestingly, a complete replacement narr...

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Published inAdvanced energy materials Vol. 10; no. 13
Main Authors Yang, Wen‐Fan, Igbari, Femi, Lou, Yan‐Hui, Wang, Zhao‐Kui, Liao, Liang‐Sheng
Format Journal Article
LanguageEnglish
Published Weinheim Wiley Subscription Services, Inc 01.04.2020
Subjects
Chemical composition
Energy gap
Lead compounds
Metal halides
Perovskites
Photovoltaic cells
Properties (attributes)
stability
Thin films
Tin
tin halide perovskites
toxicity
Online AccessGet full text
ISSN1614-6832
1614-6840
DOI10.1002/aenm.201902584

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Abstract The chemical composition engineering of lead halide perovskites via a partial or complete replacement of toxic Pb with tin has been widely reported as a feasible process due to the suitable ionic radius of Sn and its possibility of existing in the +2 state. Interestingly, a complete replacement narrows the bandgap while a partial replacement gives an anomalous phenomenon involving a further narrowing of bandgap relative to the pure Pb and Sn halide perovskite compounds. Unfortunately, the merits of this anomalous behavior have not been properly harnessed. Although promising progress has been made to advance the properties and performance of Sn‐based perovskite systems, their photovoltaic (PV) parameters are still significantly inferior to those of the Pb‐based analogs. This review summarizes the current progress and challenges in the preparation, morphological and photophysical properties of Sn‐based halide perovskites, and how these affect their PV performance. Although it can be argued that the Pb halide perovskite systems may remain the most sought after technology in the field of thin film perovskite PV, prospective research directions are suggested to advance the properties of Sn halide perovskite materials for improved device performance. The replacement of lead with tin in halide perovskites is feasible due to suitable ionic radius and valency. However, easy oxidation, high cost and toxicity concerns in Sn halide perovskite systems may limit the consideration of Sn as a suitable alternative to Pb.
AbstractList The chemical composition engineering of lead halide perovskites via a partial or complete replacement of toxic Pb with tin has been widely reported as a feasible process due to the suitable ionic radius of Sn and its possibility of existing in the +2 state. Interestingly, a complete replacement narrows the bandgap while a partial replacement gives an anomalous phenomenon involving a further narrowing of bandgap relative to the pure Pb and Sn halide perovskite compounds. Unfortunately, the merits of this anomalous behavior have not been properly harnessed. Although promising progress has been made to advance the properties and performance of Sn‐based perovskite systems, their photovoltaic (PV) parameters are still significantly inferior to those of the Pb‐based analogs. This review summarizes the current progress and challenges in the preparation, morphological and photophysical properties of Sn‐based halide perovskites, and how these affect their PV performance. Although it can be argued that the Pb halide perovskite systems may remain the most sought after technology in the field of thin film perovskite PV, prospective research directions are suggested to advance the properties of Sn halide perovskite materials for improved device performance. The replacement of lead with tin in halide perovskites is feasible due to suitable ionic radius and valency. However, easy oxidation, high cost and toxicity concerns in Sn halide perovskite systems may limit the consideration of Sn as a suitable alternative to Pb.
The chemical composition engineering of lead halide perovskites via a partial or complete replacement of toxic Pb with tin has been widely reported as a feasible process due to the suitable ionic radius of Sn and its possibility of existing in the +2 state. Interestingly, a complete replacement narrows the bandgap while a partial replacement gives an anomalous phenomenon involving a further narrowing of bandgap relative to the pure Pb and Sn halide perovskite compounds. Unfortunately, the merits of this anomalous behavior have not been properly harnessed. Although promising progress has been made to advance the properties and performance of Sn‐based perovskite systems, their photovoltaic (PV) parameters are still significantly inferior to those of the Pb‐based analogs. This review summarizes the current progress and challenges in the preparation, morphological and photophysical properties of Sn‐based halide perovskites, and how these affect their PV performance. Although it can be argued that the Pb halide perovskite systems may remain the most sought after technology in the field of thin film perovskite PV, prospective research directions are suggested to advance the properties of Sn halide perovskite materials for improved device performance.
Author Wang, Zhao‐Kui
Liao, Liang‐Sheng
Igbari, Femi
Yang, Wen‐Fan
Lou, Yan‐Hui
Author_xml – sequence: 1
  givenname: Wen‐Fan
  surname: Yang
  fullname: Yang, Wen‐Fan
  organization: Soochow University
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  givenname: Femi
  surname: Igbari
  fullname: Igbari, Femi
  organization: Soochow University
– sequence: 3
  givenname: Yan‐Hui
  surname: Lou
  fullname: Lou, Yan‐Hui
  email: yhlou@suda.edu.cn
  organization: Soochow University
– sequence: 4
  givenname: Zhao‐Kui
  orcidid: 0000-0003-1707-499X
  surname: Wang
  fullname: Wang, Zhao‐Kui
  email: zkwang@suda.edu.cn
  organization: Soochow University
– sequence: 5
  givenname: Liang‐Sheng
  surname: Liao
  fullname: Liao, Liang‐Sheng
  organization: Soochow University
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Snippet The chemical composition engineering of lead halide perovskites via a partial or complete replacement of toxic Pb with tin has been widely reported as a...
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wiley
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SubjectTerms Chemical composition
Energy gap
Lead compounds
Metal halides
Perovskites
Photovoltaic cells
Properties (attributes)
stability
Thin films
Tin
tin halide perovskites
toxicity
Title Tin Halide Perovskites: Progress and Challenges
URI https://onlinelibrary.wiley.com/doi/abs/10.1002%2Faenm.201902584
https://www.proquest.com/docview/2387184534
Volume 10
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