Benzothiazole derivatives based colorimetric and fluorescent probes for detection of amine/ammonia and monitoring the decomposition of urea by urease
[Display omitted] •Two probes have instant ratiometric and colourimetic response to amines.•Highly sensitive amine probes were based on strips and electrospun membranes.•The fluorescent probes provide reusability for monitoring amine vapours.•The demonstrated probes could be applied in monitoring ur...
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| Published in | Spectrochimica acta. Part A, Molecular and biomolecular spectroscopy Vol. 267; no. Pt 2; p. 120616 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
England
Elsevier B.V
15.02.2022
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1386-1425 1873-3557 |
| DOI | 10.1016/j.saa.2021.120616 |
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| Abstract | [Display omitted]
•Two probes have instant ratiometric and colourimetic response to amines.•Highly sensitive amine probes were based on strips and electrospun membranes.•The fluorescent probes provide reusability for monitoring amine vapours.•The demonstrated probes could be applied in monitoring urea decomposition.
Amines play critical roles in chemical, agrochemical and pharmaceutical industries. However, volatile amine vapours cause widespread pollution and threaten human health. An efficient, highly sensitive and recyclable sensor for monitoring amine vapours is highly demanded. Typically, 2-(2-hydroxy-5-methyl) benzothiazole (HBT) derivates exhibit excellent aggregation-induced emission (AIE) phenomena in keto form originated from a unique excited-state intramolecular proton transfer (ESIPT) process. In this work, we have designed and synthesized two HBT-based fluorescent probes for ratiometric detection toward amine vapours and ammonia. In addition, the detection limits for ammonia were calculated as 226 ppm and 13 ppm respectively. Additionally, the test strips and electrospinning film dopped with fluorescent probes were utilized to recognize amine vapours and ammonia colorimetric with high sensitivity in solid states. According to the above characteristics, probes could monitor the biological activity of urease conveniently and rapidly. |
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| AbstractList | [Display omitted]
•Two probes have instant ratiometric and colourimetic response to amines.•Highly sensitive amine probes were based on strips and electrospun membranes.•The fluorescent probes provide reusability for monitoring amine vapours.•The demonstrated probes could be applied in monitoring urea decomposition.
Amines play critical roles in chemical, agrochemical and pharmaceutical industries. However, volatile amine vapours cause widespread pollution and threaten human health. An efficient, highly sensitive and recyclable sensor for monitoring amine vapours is highly demanded. Typically, 2-(2-hydroxy-5-methyl) benzothiazole (HBT) derivates exhibit excellent aggregation-induced emission (AIE) phenomena in keto form originated from a unique excited-state intramolecular proton transfer (ESIPT) process. In this work, we have designed and synthesized two HBT-based fluorescent probes for ratiometric detection toward amine vapours and ammonia. In addition, the detection limits for ammonia were calculated as 226 ppm and 13 ppm respectively. Additionally, the test strips and electrospinning film dopped with fluorescent probes were utilized to recognize amine vapours and ammonia colorimetric with high sensitivity in solid states. According to the above characteristics, probes could monitor the biological activity of urease conveniently and rapidly. Amines play critical roles in chemical, agrochemical and pharmaceutical industries. However, volatile amine vapours cause widespread pollution and threaten human health. An efficient, highly sensitive and recyclable sensor for monitoring amine vapours is highly demanded. Typically, 2-(2-hydroxy-5-methyl) benzothiazole (HBT) derivates exhibit excellent aggregation-induced emission (AIE) phenomena in keto form originated from a unique excited-state intramolecular proton transfer (ESIPT) process. In this work, we have designed and synthesized two HBT-based fluorescent probes for ratiometric detection toward amine vapours and ammonia. In addition, the detection limits for ammonia were calculated as 226 ppm and 13 ppm respectively. Additionally, the test strips and electrospinning film dopped with fluorescent probes were utilized to recognize amine vapours and ammonia colorimetric with high sensitivity in solid states. According to the above characteristics, probes could monitor the biological activity of urease conveniently and rapidly. |
| ArticleNumber | 120616 |
| Author | Chen, Yahui Chen, Xiaoqiang Kong, Qing Wang, Fang Zheng, Shiyue Fang, Yu |
| Author_xml | – sequence: 1 givenname: Shiyue surname: Zheng fullname: Zheng, Shiyue – sequence: 2 givenname: Yu surname: Fang fullname: Fang, Yu – sequence: 3 givenname: Yahui surname: Chen fullname: Chen, Yahui – sequence: 4 givenname: Qing surname: Kong fullname: Kong, Qing – sequence: 5 givenname: Fang surname: Wang fullname: Wang, Fang email: fangwang@njtech.edu.cn – sequence: 6 givenname: Xiaoqiang surname: Chen fullname: Chen, Xiaoqiang email: chenxq@njtech.edu.cn |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/34840048$$D View this record in MEDLINE/PubMed |
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| Keywords | Fluorescent probes Amines Aggregation-induced emission Electrospinning film Benzothiazole-based derivatives Excited-state intramolecular proton transfer |
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•Two probes have instant ratiometric and colourimetic response to amines.•Highly sensitive amine probes were based on strips and electrospun... Amines play critical roles in chemical, agrochemical and pharmaceutical industries. However, volatile amine vapours cause widespread pollution and threaten... |
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| SubjectTerms | Aggregation-induced emission Amines Ammonia Benzothiazole-based derivatives Benzothiazoles Colorimetry Electrospinning film Excited-state intramolecular proton transfer Fluorescent Dyes Fluorescent probes Humans Urea Urease |
| Title | Benzothiazole derivatives based colorimetric and fluorescent probes for detection of amine/ammonia and monitoring the decomposition of urea by urease |
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