Highly conductive carbon nanotube micro-spherical network for high-rate silicon anode
We report on a highly conductive CNT micro-spherical network for high-rate silicon anode materials prepared by one-pot spray drying for lithium-ion batteries. The anode material contains silicon nanoparticles bound to CNTs through a small amount of sucrose-derived carbon. The first charge and discha...
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| Published in | Journal of power sources Vol. 394; pp. 94 - 101 |
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| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.08.2018
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| Subjects | |
| Online Access | Get full text |
| ISSN | 0378-7753 1873-2755 |
| DOI | 10.1016/j.jpowsour.2018.04.112 |
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| Abstract | We report on a highly conductive CNT micro-spherical network for high-rate silicon anode materials prepared by one-pot spray drying for lithium-ion batteries. The anode material contains silicon nanoparticles bound to CNTs through a small amount of sucrose-derived carbon. The first charge and discharge capacities of the Si/CNT/C microsphere electrode are measured to be 3152 and 2302 mA h g−1 of the composite, respectively, at 0.1 A g−1. The Si/CNT/C microsphere electrode exhibits an initial capacity of 1989 mA h g−1 at current density of 1.0 A g−1 and retains ∼70% of the initial capacity after 100 cycles. Even at a high current density of 10 A g−1, the Si/CNT/C microsphere electrode exhibits a capacity of 784 mA h g−1 with a stable charge/discharge behavior. The superior rate capability of the Si/CNT/C microsphere composites can be attributable to the unhindered Li-ion transport through the highly conductive CNT buffer matrix, to which Si NPs are strongly bound by the sucrose-derived carbon. These salient results give further impetus to the study of CNTs for use as a buffer matrix to improve the rate capability of high-capacity electrode materials with large volume changes during charge storage.
•Si NPs are bound to CNT network through a very tiny amount of sucrose-derived carbon.•The Si/CNT/C microsphere has an interconnected pore facilitating Li-ion transport.•The Si/CNT/C microsphere exhibited superior rate capability with high capacity. |
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| AbstractList | We report on a highly conductive CNT micro-spherical network for high-rate silicon anode materials prepared by one-pot spray drying for lithium-ion batteries. The anode material contains silicon nanoparticles bound to CNTs through a small amount of sucrose-derived carbon. The first charge and discharge capacities of the Si/CNT/C microsphere electrode are measured to be 3152 and 2302 mA h g−1 of the composite, respectively, at 0.1 A g−1. The Si/CNT/C microsphere electrode exhibits an initial capacity of 1989 mA h g−1 at current density of 1.0 A g−1 and retains ∼70% of the initial capacity after 100 cycles. Even at a high current density of 10 A g−1, the Si/CNT/C microsphere electrode exhibits a capacity of 784 mA h g−1 with a stable charge/discharge behavior. The superior rate capability of the Si/CNT/C microsphere composites can be attributable to the unhindered Li-ion transport through the highly conductive CNT buffer matrix, to which Si NPs are strongly bound by the sucrose-derived carbon. These salient results give further impetus to the study of CNTs for use as a buffer matrix to improve the rate capability of high-capacity electrode materials with large volume changes during charge storage.
•Si NPs are bound to CNT network through a very tiny amount of sucrose-derived carbon.•The Si/CNT/C microsphere has an interconnected pore facilitating Li-ion transport.•The Si/CNT/C microsphere exhibited superior rate capability with high capacity. |
| Author | Park, Byung Hoon Roh, Kwang Chul Kim, Kwang-Bum Lee, Geon-Woo Jeong, Jun Hui Kim, Young-Hwan |
| Author_xml | – sequence: 1 givenname: Byung Hoon surname: Park fullname: Park, Byung Hoon organization: Department of Materials Science and Engineering, Yonsei University, 50 Yonsei-ro, Seodaemoon-gu, Seoul, 03722, Republic of Korea – sequence: 2 givenname: Jun Hui surname: Jeong fullname: Jeong, Jun Hui organization: Department of Materials Science and Engineering, Yonsei University, 50 Yonsei-ro, Seodaemoon-gu, Seoul, 03722, Republic of Korea – sequence: 3 givenname: Geon-Woo surname: Lee fullname: Lee, Geon-Woo organization: Department of Materials Science and Engineering, Yonsei University, 50 Yonsei-ro, Seodaemoon-gu, Seoul, 03722, Republic of Korea – sequence: 4 givenname: Young-Hwan surname: Kim fullname: Kim, Young-Hwan organization: Department of Materials Science and Engineering, Yonsei University, 50 Yonsei-ro, Seodaemoon-gu, Seoul, 03722, Republic of Korea – sequence: 5 givenname: Kwang Chul orcidid: 0000-0002-1618-791X surname: Roh fullname: Roh, Kwang Chul email: rkc@kicet.re.kr organization: Energy and Environmental Division, Korea Institute of Ceramic Engineering and Technology, 101 Soho-ro, Jinju-si, Gyeongsangnam-do, 52851, Republic of Korea – sequence: 6 givenname: Kwang-Bum orcidid: 0000-0002-2184-6617 surname: Kim fullname: Kim, Kwang-Bum email: kbkim@yonsei.ac.kr organization: Department of Materials Science and Engineering, Yonsei University, 50 Yonsei-ro, Seodaemoon-gu, Seoul, 03722, Republic of Korea |
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| Keywords | Lithium-ion batteries Spray dry High-rate Si anode Silicon/CNT microsphere |
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| SubjectTerms | High-rate Si anode Lithium-ion batteries Silicon/CNT microsphere Spray dry |
| Title | Highly conductive carbon nanotube micro-spherical network for high-rate silicon anode |
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