Characteristics, Sources, and Risks of Polycyclic Aromatic Hydrocarbons in Topsoil and Surface Water from the Liuxi River Basin, South China

The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng...

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Published inArchives of environmental contamination and toxicology Vol. 78; no. 3; pp. 401 - 415
Main Authors Xie, Zhenglan, Gao, Lei, Liang, Zuobing, Chen, Jianyao, Li, Shaoheng, Zhu, Aiping, Wu, Yu, Yang, Zhigang, Li, Rui, Wang, Zhuowei
Format Journal Article
LanguageEnglish
Published New York Springer US 01.04.2020
Springer Nature B.V
Subjects
basins
Carbon content
China
Coking
Correlation analysis
Earth and Environmental Science
Ecology
Ecotoxicology
Emissions
Environment
Environmental Chemistry
Environmental Health
Environmental Monitoring - methods
Fossil fuels
Fuel combustion
Geologic Sediments - chemistry
guidelines
Monitoring/Environmental Analysis
Organic carbon
particulate emissions
Pollutant deposition
Pollutants
Pollution
Polycyclic aromatic hydrocarbons
Polycyclic Aromatic Hydrocarbons - analysis
Public health
Quality assessment
risk
Risk Assessment
River basins
Rivers
Rivers - chemistry
Soil - chemistry
Soil Pollutants - analysis
Soil quality
Soil Science & Conservation
Spatial distribution
Surface water
Topsoil
Total organic carbon
toxicity
Tributaries
Vehicle emissions
Water Pollutants, Chemical - analysis
Water pollution
watersheds
Wet deposition
China
Online AccessGet full text
ISSN0090-4341
1432-0703
1432-0703
DOI10.1007/s00244-020-00711-4

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Abstract The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng/L in surface water, indicating mild pollution. The PAHs in topsoil exhibited an even spatial distribution, suggesting that they originated primarily from dry and wet deposition of transported pollutants. The concentration of PAHs in surface water did not differ significantly geographically, but the concentrations of total, three-, and four-ring PAHs were significantly lower in the Liuxi River than in its tributaries. Three- and two-ring PAHs predominated in topsoil and surface water, respectively. A correlation analysis suggested that the total organic carbon content and pH exerted a negligible effect on the spatial distribution of PAHs in topsoil, and they may have common sources. Fossil fuel combustion (particularly vehicle emissions) and coking production were the dominant sources of PAHs in topsoil, whereas those in surface water were derived from a variety of sources. The total toxic equivalent concentrations of 16 PAHs in topsoil ranged from 3.73 to 105.66 ng/g (mean, 30.93 ng/g), suggesting that exposure to the basin’s topsoil does not pose a risk to the environment or public health according to the Canadian soil quality guidelines. A risk assessment revealed that the total PAH concentrations in surface water posed a low ecological risk.
AbstractList The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng/L in surface water, indicating mild pollution. The PAHs in topsoil exhibited an even spatial distribution, suggesting that they originated primarily from dry and wet deposition of transported pollutants. The concentration of PAHs in surface water did not differ significantly geographically, but the concentrations of total, three-, and four-ring PAHs were significantly lower in the Liuxi River than in its tributaries. Three- and two-ring PAHs predominated in topsoil and surface water, respectively. A correlation analysis suggested that the total organic carbon content and pH exerted a negligible effect on the spatial distribution of PAHs in topsoil, and they may have common sources. Fossil fuel combustion (particularly vehicle emissions) and coking production were the dominant sources of PAHs in topsoil, whereas those in surface water were derived from a variety of sources. The total toxic equivalent concentrations of 16 PAHs in topsoil ranged from 3.73 to 105.66 ng/g (mean, 30.93 ng/g), suggesting that exposure to the basin's topsoil does not pose a risk to the environment or public health according to the Canadian soil quality guidelines. A risk assessment revealed that the total PAH concentrations in surface water posed a low ecological risk.
The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng/L in surface water, indicating mild pollution. The PAHs in topsoil exhibited an even spatial distribution, suggesting that they originated primarily from dry and wet deposition of transported pollutants. The concentration of PAHs in surface water did not differ significantly geographically, but the concentrations of total, three-, and four-ring PAHs were significantly lower in the Liuxi River than in its tributaries. Three- and two-ring PAHs predominated in topsoil and surface water, respectively. A correlation analysis suggested that the total organic carbon content and pH exerted a negligible effect on the spatial distribution of PAHs in topsoil, and they may have common sources. Fossil fuel combustion (particularly vehicle emissions) and coking production were the dominant sources of PAHs in topsoil, whereas those in surface water were derived from a variety of sources. The total toxic equivalent concentrations of 16 PAHs in topsoil ranged from 3.73 to 105.66 ng/g (mean, 30.93 ng/g), suggesting that exposure to the basin's topsoil does not pose a risk to the environment or public health according to the Canadian soil quality guidelines. A risk assessment revealed that the total PAH concentrations in surface water posed a low ecological risk.The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng/L in surface water, indicating mild pollution. The PAHs in topsoil exhibited an even spatial distribution, suggesting that they originated primarily from dry and wet deposition of transported pollutants. The concentration of PAHs in surface water did not differ significantly geographically, but the concentrations of total, three-, and four-ring PAHs were significantly lower in the Liuxi River than in its tributaries. Three- and two-ring PAHs predominated in topsoil and surface water, respectively. A correlation analysis suggested that the total organic carbon content and pH exerted a negligible effect on the spatial distribution of PAHs in topsoil, and they may have common sources. Fossil fuel combustion (particularly vehicle emissions) and coking production were the dominant sources of PAHs in topsoil, whereas those in surface water were derived from a variety of sources. The total toxic equivalent concentrations of 16 PAHs in topsoil ranged from 3.73 to 105.66 ng/g (mean, 30.93 ng/g), suggesting that exposure to the basin's topsoil does not pose a risk to the environment or public health according to the Canadian soil quality guidelines. A risk assessment revealed that the total PAH concentrations in surface water posed a low ecological risk.
The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south China were analyzed in this study. The total concentrations of 16 PAHs ranged from 296.26 to 888.14 ng/g in topsoil and from 156.73 to 422.03 ng/L in surface water, indicating mild pollution. The PAHs in topsoil exhibited an even spatial distribution, suggesting that they originated primarily from dry and wet deposition of transported pollutants. The concentration of PAHs in surface water did not differ significantly geographically, but the concentrations of total, three-, and four-ring PAHs were significantly lower in the Liuxi River than in its tributaries. Three- and two-ring PAHs predominated in topsoil and surface water, respectively. A correlation analysis suggested that the total organic carbon content and pH exerted a negligible effect on the spatial distribution of PAHs in topsoil, and they may have common sources. Fossil fuel combustion (particularly vehicle emissions) and coking production were the dominant sources of PAHs in topsoil, whereas those in surface water were derived from a variety of sources. The total toxic equivalent concentrations of 16 PAHs in topsoil ranged from 3.73 to 105.66 ng/g (mean, 30.93 ng/g), suggesting that exposure to the basin’s topsoil does not pose a risk to the environment or public health according to the Canadian soil quality guidelines. A risk assessment revealed that the total PAH concentrations in surface water posed a low ecological risk.
Author Zhu, Aiping
Gao, Lei
Liang, Zuobing
Wang, Zhuowei
Wu, Yu
Chen, Jianyao
Li, Rui
Xie, Zhenglan
Li, Shaoheng
Yang, Zhigang
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  organization: School of Geography and Planning, Sun Yat-sen University, Guangdong Key Laboratory for Urbanization and Geo-simulation, Sun Yat-sen University
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  givenname: Zhigang
  surname: Yang
  fullname: Yang, Zhigang
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  organization: School of Geography and Planning, Sun Yat-sen University, Guangdong Key Laboratory for Urbanization and Geo-simulation, Sun Yat-sen University
BackLink https://www.ncbi.nlm.nih.gov/pubmed/32008048$$D View this record in MEDLINE/PubMed
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Snippet The concentrations, composition, sources, and risks of polycyclic aromatic hydrocarbons (PAHs) in topsoil and surface water of the Liuxi River basin, south...
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SubjectTerms basins
Carbon content
China
Coking
Correlation analysis
Earth and Environmental Science
Ecology
Ecotoxicology
Emissions
Environment
Environmental Chemistry
Environmental Health
Environmental Monitoring - methods
Fossil fuels
Fuel combustion
Geologic Sediments - chemistry
guidelines
Monitoring/Environmental Analysis
Organic carbon
particulate emissions
Pollutant deposition
Pollutants
Pollution
Polycyclic aromatic hydrocarbons
Polycyclic Aromatic Hydrocarbons - analysis
Public health
Quality assessment
risk
Risk Assessment
River basins
Rivers
Rivers - chemistry
Soil - chemistry
Soil Pollutants - analysis
Soil quality
Soil Science & Conservation
Spatial distribution
Surface water
Topsoil
Total organic carbon
toxicity
Tributaries
Vehicle emissions
Water Pollutants, Chemical - analysis
Water pollution
watersheds
Wet deposition
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Title Characteristics, Sources, and Risks of Polycyclic Aromatic Hydrocarbons in Topsoil and Surface Water from the Liuxi River Basin, South China
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