Tip-induced heating in apertureless near-field optics

Tip‐enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many problems. In this paper we provide insight into the level of sample heating by the laser light in the presence of a metal‐coated atomic force...

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Published inJournal of Raman spectroscopy Vol. 40; no. 10; pp. 1349 - 1354
Main Authors Malkovskiy, A. V., Malkovsky, V. I., Kisliuk, A. M., Barrios, C. A., Foster, M. D., Sokolov, A. P.
Format Journal Article
LanguageEnglish
Published Chichester, UK John Wiley & Sons, Ltd 01.10.2009
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ISSN0377-0486
1097-4555
DOI10.1002/jrs.2388

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Abstract Tip‐enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many problems. In this paper we provide insight into the level of sample heating by the laser light in the presence of a metal‐coated atomic force microscope (AFM) tip. The heating is attributed to the presence of an optical field enhanced by the tip. Sample temperatures were estimated using measurements of the ratio of the Stokes and anti‐Stokes signals from a thin 50‐nm sample on an Al substrate. A correlation between the heating and optical properties of the tips is established. The results demonstrate significant tip‐induced heating (100 K and more) even at very low laser power. Copyright © 2009 John Wiley & Sons, Ltd. In this paper we report on the level of an additional sample heating by the laser light in the presence of a metal‐coated AFM tip (TERS experiments). The results show significant heating even at low laser power.
AbstractList Tip-enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many problems. In this paper we provide insight into the level of sample heating by the laser light in the presence of a metal-coated atomic force microscope (AFM) tip. The heating is attributed to the presence of an optical field enhanced by the tip. Sample temperatures were estimated using measurements of the ratio of the Stokes and anti-Stokes signals from a thin 50-nm sample on an Al substrate. A correlation between the heating and optical properties of the tips is established. The results demonstrate significant tip-induced heating (100 K and more) even at very low laser power.
Tip‐enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many problems. In this paper we provide insight into the level of sample heating by the laser light in the presence of a metal‐coated atomic force microscope (AFM) tip. The heating is attributed to the presence of an optical field enhanced by the tip. Sample temperatures were estimated using measurements of the ratio of the Stokes and anti‐Stokes signals from a thin 50‐nm sample on an Al substrate. A correlation between the heating and optical properties of the tips is established. The results demonstrate significant tip‐induced heating (100 K and more) even at very low laser power. Copyright © 2009 John Wiley & Sons, Ltd. In this paper we report on the level of an additional sample heating by the laser light in the presence of a metal‐coated AFM tip (TERS experiments). The results show significant heating even at low laser power.
Tip‐enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many problems. In this paper we provide insight into the level of sample heating by the laser light in the presence of a metal‐coated atomic force microscope (AFM) tip. The heating is attributed to the presence of an optical field enhanced by the tip. Sample temperatures were estimated using measurements of the ratio of the Stokes and anti‐Stokes signals from a thin 50‐nm sample on an Al substrate. A correlation between the heating and optical properties of the tips is established. The results demonstrate significant tip‐induced heating (100 K and more) even at very low laser power. Copyright © 2009 John Wiley & Sons, Ltd.
Author Sokolov, A. P.
Malkovskiy, A. V.
Kisliuk, A. M.
Barrios, C. A.
Foster, M. D.
Malkovsky, V. I.
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Snippet Tip‐enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many...
Tip-enhanced Raman spectroscopy is considered a promising technique for imaging with nanoscale lateral resolution. However, its developments and use face many...
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SubjectTerms Aluminum
apertureless
Heating
Lasers
Nanocomposites
Nanomaterials
Nanostructure
Optical properties
Raman spectroscopy
SNOM
TERS
Title Tip-induced heating in apertureless near-field optics
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