Extension of Tao-Mason Equation of State to Heavy n-Alkanes
In our previous paper we extended the Tao and Mason equation of state （TM EOS） to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C 9 to C 20 have been...
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| Published in | Chinese journal of chemical engineering Vol. 21; no. 8; pp. 894 - 900 |
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| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.08.2013
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(13)60548-0 |
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| Abstract | In our previous paper we extended the Tao and Mason equation of state （TM EOS） to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C 9 to C 20 have been calculated using an analytical equation of state based on the statistical-mechanical perturbation theory. The second virial coefficients of these n-alkanes are scarce and there is no accurate potential energy function for their theoretical calculation. In this work the second virial coefficients are calculated using a corresponding state correlation based on surface tension and liquid density at the freezing point. The deviation of calculated densities of these alkanes is within 0.5% from experimental data. The densities of n-alkanes obtained from the TM EOS are compared with those calculated from Ihm-Song-Mason equation of state and the corresponding-states liquid densities （COSTALD）. Our results are in favor of the preference of the TM EOS over other two equations of state. |
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| AbstractList | In our previous paper we extended the Tao and Mason equation of state (TM EOS) to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C9 to C20 have been calculated using an analytical equation of state based on the statistical-mechanical perturbation theory. The second virial coefficients of these n-alkanes are scarce and there is no accurate potential energy function for their theoretical calculation. In this work the second virial coefficients are calculated using a corresponding state correlation based on surface tension and liquid density at the freezing point. The deviation of calculated densities of these alkanes is within 0.5% from experimental data. The densities of n-alkanes obtained from the TM EOS are compared with those calculated from Ihm-Song-Mason equation of state and the corresponding-states liquid densities (COSTALD). Our results are in favor of the preference of the TM EOS over other two equations of state. In our previous paper we extended the Tao and Mason equation of state （TM EOS） to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C 9 to C 20 have been calculated using an analytical equation of state based on the statistical-mechanical perturbation theory. The second virial coefficients of these n-alkanes are scarce and there is no accurate potential energy function for their theoretical calculation. In this work the second virial coefficients are calculated using a corresponding state correlation based on surface tension and liquid density at the freezing point. The deviation of calculated densities of these alkanes is within 0.5% from experimental data. The densities of n-alkanes obtained from the TM EOS are compared with those calculated from Ihm-Song-Mason equation of state and the corresponding-states liquid densities （COSTALD）. Our results are in favor of the preference of the TM EOS over other two equations of state. In our previous paper we extended the Tao and Mason equation of state (TM EOS) to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C(9) to C(20) have been calculated using an analytical equation of state based on the statistical-mechanical perturbation theory. The second virial coefficients of these n-alkanes are scarce and there is no accurate potential energy function for their theoretical calculation. In this work the second virial coefficients are calculated using a corresponding state correlation based on surface tension and liquid density at the freezing point. The deviation of calculated densities of these alkanes is within 0.5% from experimental data. The densities of n-alkanes obtained from the TM EOS are compared with those calculated from Ihm-Song-Mason equation of state and the corresponding-states liquid densities (COSTALD). Our results are in favor of the preference of the TM EOS over other two equations of state. |
| Author | Fakhri Yousefi Hajir Karimi Mohammad Mehdi Papari |
| AuthorAffiliation | Department of Chemistry, Yasouj University Department of Chemical Engineering, Yasouj University Department of Chemistry, Shiraz University of Technology |
| Author_xml | – sequence: 1 givenname: Fakhri surname: Yousefi fullname: Yousefi, Fakhri email: fyousefi@mail.yu.ac.ir organization: Department of Chemistry, Yasouj University, Yasouj, 75914-353, Iran – sequence: 2 givenname: Hajir surname: Karimi fullname: Karimi, Hajir organization: Department of Chemical Engineering, Yasouj University, Yasouj, 75914-353, Iran – sequence: 3 givenname: Mohammad Mehdi surname: Papari fullname: Papari, Mohammad Mehdi organization: Department of Chemistry, Shiraz University of Technology, Shiraz 71555-313, Iran |
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| CitedBy_id | crossref_primary_10_1016_j_cjche_2016_10_016 crossref_primary_10_1007_s00396_014_3391_9 crossref_primary_10_1016_j_molliq_2017_10_075 |
| Cites_doi | 10.1063/1.460684 10.1063/1.466713 10.1002/aic.690210435 10.1007/BF01439197 10.1103/PhysRevA.42.4743 10.1002/aic.690200209 10.1002/aic.690250412 10.1252/jcej.10we145 10.1016/S0378-3812(99)00331-3 10.1007/BF01141215 10.1016/S1004-9541(11)60012-8 10.1080/00268976400100611 10.1021/ja01567a007 10.1103/RevModPhys.41.316 10.1007/s11581-011-0605-8 10.1016/0378-3812(92)87011-B 10.1002/aic.690240625 10.1016/0378-3812(92)87010-K 10.1063/1.457252 10.1063/1.1672048 10.1007/BF00502114 10.1021/ie8016658 10.1063/1.345684 10.1063/1.1701689 |
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| Keywords | heavy n-alkanes density Tao-Mason equation of state Ihm-Song-Mason equation of state |
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| Notes | In our previous paper we extended the Tao and Mason equation of state （TM EOS） to refrigerant fluids, using the speed of sound data. This is a continuation for evaluating TM EOS in predicting PVT properties of heavy n-alkanes. Liquid density of long-chain n-alkane systems from C 9 to C 20 have been calculated using an analytical equation of state based on the statistical-mechanical perturbation theory. The second virial coefficients of these n-alkanes are scarce and there is no accurate potential energy function for their theoretical calculation. In this work the second virial coefficients are calculated using a corresponding state correlation based on surface tension and liquid density at the freezing point. The deviation of calculated densities of these alkanes is within 0.5% from experimental data. The densities of n-alkanes obtained from the TM EOS are compared with those calculated from Ihm-Song-Mason equation of state and the corresponding-states liquid densities （COSTALD）. Our results are in favor of the preference of the TM EOS over other two equations of state. Fakhri Yousefi1＇＊, Hajir Karimi2 and Mohammad Mehdi Papari3 l Department of Chemistry, Yasouj University, Yasouj, 75914-353, Iran - 2 Department of Chemical Engineering, Yasouj University, Yasouj, 75914-353, Iran 3 Dep~ment of Chemistry, Shiraz University of Technology, Shiraz 71555-313, Iran 11-3270/TQ heavy n-alkanes, density, Tao-Mason equation of state, Ihm-Song-Mason equation of state ObjectType-Article-2 SourceType-Scholarly Journals-1 ObjectType-Feature-1 content type line 23 ObjectType-Article-1 ObjectType-Feature-2 |
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| References | Prauznitz, Lichtentaler, Azevedo (bib20) 1999 Vargaftik (bib27) 1983 Carnahan, Starling (bib7) 1969; 51 Pitzer, Curl (bib22) 1957; 79 Karimi, Yousefi, Papari (bib15) 2011; 44 Macdonald (bib2) 1969; 41 Dymond, Malhorta (bib5) 1988; 9 Ghatee, Boushehri (bib26) 1996; 17 Longuet-Higgins, Widom (bib1) 1964; 8 Song, Mason (bib9) 1990; 42 Cho (bib4) 1990; 67 Sandler (bib19) 1989 Karimi, Yousefi, Papari (bib16) 2011; 19 Barker, Henderson (bib6) 1967; 47 Levelt Sengers, Deiters, Klask, Swidersky, Schneider (bib18) 1993; 14 Ihm, Song, Mason (bib11) 1991; 94 Song, Mason (bib10) 1992; 75 Tsonopolous (bib24) 1975; 21 Berry, Rice, Ross (bib3) 1980 Yousefi, Moghadasi, Papari, Campo (bib14) 2009; 48 Tao, Mason (bib13) 1994; 100 Tsonopolous (bib25) 1978; 24 Hankinson, Thomson (bib29) 1979; 25 Ihm, Song, Mason (bib12) 1992; 75 Tsonopolous (bib23) 1974; 20 Song, Mason (bib8) 1989; 91 Eslami (bib28) 2000; 169 Tao, Mason (bib21) 1992; 13 Yousefi, Karimi (bib17) 2012; 18 Macdonald (10.1016/S1004-9541(13)60548-0_bib2) 1969; 41 Hankinson (10.1016/S1004-9541(13)60548-0_bib29) 1979; 25 Tsonopolous (10.1016/S1004-9541(13)60548-0_bib23) 1974; 20 Song (10.1016/S1004-9541(13)60548-0_bib9) 1990; 42 Tao (10.1016/S1004-9541(13)60548-0_bib21) 1992; 13 Berry (10.1016/S1004-9541(13)60548-0_bib3) 1980 Yousefi (10.1016/S1004-9541(13)60548-0_bib14) 2009; 48 Eslami (10.1016/S1004-9541(13)60548-0_bib28) 2000; 169 Longuet-Higgins (10.1016/S1004-9541(13)60548-0_bib1) 1964; 8 Vargaftik (10.1016/S1004-9541(13)60548-0_bib27) 1983 Carnahan (10.1016/S1004-9541(13)60548-0_bib7) 1969; 51 Pitzer (10.1016/S1004-9541(13)60548-0_bib22) 1957; 79 Karimi (10.1016/S1004-9541(13)60548-0_bib15) 2011; 44 Tsonopolous (10.1016/S1004-9541(13)60548-0_bib24) 1975; 21 Dymond (10.1016/S1004-9541(13)60548-0_bib5) 1988; 9 Sandler (10.1016/S1004-9541(13)60548-0_bib19) 1989 Tao (10.1016/S1004-9541(13)60548-0_bib13) 1994; 100 Tsonopolous (10.1016/S1004-9541(13)60548-0_bib25) 1978; 24 Song (10.1016/S1004-9541(13)60548-0_bib8) 1989; 91 Yousefi (10.1016/S1004-9541(13)60548-0_bib17) 2012; 18 Ihm (10.1016/S1004-9541(13)60548-0_bib11) 1991; 94 Karimi (10.1016/S1004-9541(13)60548-0_bib16) 2011; 19 Cho (10.1016/S1004-9541(13)60548-0_bib4) 1990; 67 Barker (10.1016/S1004-9541(13)60548-0_bib6) 1967; 47 Ihm (10.1016/S1004-9541(13)60548-0_bib12) 1992; 75 Ghatee (10.1016/S1004-9541(13)60548-0_bib26) 1996; 17 Song (10.1016/S1004-9541(13)60548-0_bib10) 1992; 75 Levelt Sengers (10.1016/S1004-9541(13)60548-0_bib18) 1993; 14 Prauznitz (10.1016/S1004-9541(13)60548-0_bib20) 1999 |
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| Snippet | In our previous paper we extended the Tao and Mason equation of state （TM EOS） to refrigerant fluids, using the speed of sound data. This is a continuation... In our previous paper we extended the Tao and Mason equation of state (TM EOS) to refrigerant fluids, using the speed of sound data. This is a continuation for... |
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| SubjectTerms | Density Deviation EOS Equations of state Freezing point heavy n-alkanes Ihm-Song-Mason equation of state Liquids Mathematical analysis PVT特性 Refrigerants Tao-Mason equation of state Virial coefficients 摄动理论 梅森公式 液体密度 状态方程 第二维里系数 长链正构烷烃 |
| Title | Extension of Tao-Mason Equation of State to Heavy n-Alkanes |
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