Heterogeneous Catalysis for CO2 Conversion into Chemicals and Fuels

Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO 2 can be converted into a wide range of valuable products, including CO, formic acid, methan...

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Published inTransactions of Tianjin University Vol. 28; no. 4; pp. 245 - 264
Main Authors Gao, Dunfeng, Li, Wanjun, Wang, Hanyu, Wang, Guoxiong, Cai, Rui
Format Journal Article
LanguageEnglish
Published Tianjin Tianjin University 01.08.2022
Springer Nature B.V
University of Chinese Academy of Sciences,Beijing 100049,China
State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China%State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China
Subjects
Acetic acid
Alkenes
Carbon dioxide
Catalytic converters
Conversion
Density functional theory
Engineering
Ethanol
Fine chemicals
Formic acid
Humanities and Social Sciences
Mechanical Engineering
multidisciplinary
Review
Science
Selectivity
electroreduction
CO
Fuels
hydrogenation
Chemicals
conversion
CO2 electroreduction
CO2 conversion
CO2 hydrogenation
Online AccessGet full text
ISSN1006-4982
1995-8196
DOI10.1007/s12209-022-00326-x

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Abstract Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO 2 can be converted into a wide range of valuable products, including CO, formic acid, methanol, methane, ethanol, acetic acid, propanol, light olefins, aromatics, and gasoline, as well as fine chemicals. In this mini-review, we summarize the recent progress in heterogeneous catalysis for CO 2 conversion into chemicals and fuels and highlight some representative studies of different conversion routes. The structure–performance correlations of typical catalytic materials used for the CO 2 conversion reactions have been revealed by combining advanced in situ/operando spectroscopy and microscopy characterizations and density functional theory calculations. Catalytic selectivity toward a single CO 2 reduction product/fraction should be further improved at an industrially relevant CO 2 conversion rate with considerable stability in the future. Graphical Abstract
AbstractList Catalytic conversion of CO2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO2 can be converted into a wide range of valuable products, including CO, formic acid, methanol, methane, ethanol, acetic acid, propanol, light olefi ns, aromatics, and gasoline, as well as fi ne chemicals. In this mini-review, we summarize the recent progress in heterogeneous catalysis for CO2 conversion into chemicals and fuels and highlight some representative studies of diff erent conversion routes. The structure–performance correlations of typical catalytic materials used for the CO2 conversion reactions have been revealed by combining advanced insitu/operando spectroscopy and microscopy characterizations and density functional theory cal-culations. Catalytic selectivity toward a single CO2 reduction product/fraction should be further improved at an industrially relevant CO2 conversion rate with considerable stability in the future.
Catalytic conversion of CO2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO2 can be converted into a wide range of valuable products, including CO, formic acid, methanol, methane, ethanol, acetic acid, propanol, light olefins, aromatics, and gasoline, as well as fine chemicals. In this mini-review, we summarize the recent progress in heterogeneous catalysis for CO2 conversion into chemicals and fuels and highlight some representative studies of different conversion routes. The structure–performance correlations of typical catalytic materials used for the CO2 conversion reactions have been revealed by combining advanced in situ/operando spectroscopy and microscopy characterizations and density functional theory calculations. Catalytic selectivity toward a single CO2 reduction product/fraction should be further improved at an industrially relevant CO2 conversion rate with considerable stability in the future.
Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO 2 can be converted into a wide range of valuable products, including CO, formic acid, methanol, methane, ethanol, acetic acid, propanol, light olefins, aromatics, and gasoline, as well as fine chemicals. In this mini-review, we summarize the recent progress in heterogeneous catalysis for CO 2 conversion into chemicals and fuels and highlight some representative studies of different conversion routes. The structure–performance correlations of typical catalytic materials used for the CO 2 conversion reactions have been revealed by combining advanced in situ/operando spectroscopy and microscopy characterizations and density functional theory calculations. Catalytic selectivity toward a single CO 2 reduction product/fraction should be further improved at an industrially relevant CO 2 conversion rate with considerable stability in the future. Graphical Abstract
Author Li, Wanjun
Wang, Guoxiong
Wang, Hanyu
Cai, Rui
Gao, Dunfeng
AuthorAffiliation State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China%State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China;University of Chinese Academy of Sciences,Beijing 100049,China
AuthorAffiliation_xml – name: State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China%State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China;University of Chinese Academy of Sciences,Beijing 100049,China
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Tue Jul 01 02:15:56 EDT 2025
Thu Apr 24 23:00:00 EDT 2025
Fri Feb 21 02:45:02 EST 2025
IsDoiOpenAccess true
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Issue 4
Keywords electroreduction
CO
Fuels
hydrogenation
Chemicals
conversion
CO2 electroreduction
CO2 conversion
CO2 hydrogenation
Language English
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PublicationSubtitle Advanced Energy Chemistry and Materials
PublicationTitle Transactions of Tianjin University
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PublicationTitle_FL Transactions of Tianjin University
PublicationYear 2022
Publisher Tianjin University
Springer Nature B.V
University of Chinese Academy of Sciences,Beijing 100049,China
State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China%State Key Laboratory of Catalysis,Dalian National Laboratory for Clean Energy,Dalian Institute of Chemical Physics,Chinese Academy of Sciences,Dalian 116023, China
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– name: University of Chinese Academy of Sciences,Beijing 100049,China
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Snippet Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis,...
Catalytic conversion of CO2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis,...
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SubjectTerms Acetic acid
Alkenes
Carbon dioxide
Catalytic converters
Conversion
Density functional theory
Engineering
Ethanol
Fine chemicals
Formic acid
Humanities and Social Sciences
Mechanical Engineering
multidisciplinary
Review
Science
Selectivity
Title Heterogeneous Catalysis for CO2 Conversion into Chemicals and Fuels
URI https://link.springer.com/article/10.1007/s12209-022-00326-x
https://www.proquest.com/docview/2707399614
https://d.wanfangdata.com.cn/periodical/tianjdxxb-e202204003
Volume 28
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