Establishment of Kinetic Model for Catalytic Pyrolysis of Daqing Atmospheric Residue
An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in the catalytic pyrolysis process of Daqing atmospheric residue. The model contains 21 kinetic parameters and one for catalyst deactivation. A series of experiments were carded out in a riser reactor over...
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| Published in | Chinese journal of chemical engineering Vol. 17; no. 1; pp. 78 - 82 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2009
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(09)60036-7 |
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| Abstract | An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in the catalytic pyrolysis process of Daqing atmospheric residue. The model contains 21 kinetic parameters and one for catalyst deactivation. A series of experiments were carded out in a riser reactor over catalyst named LTB-2. The ki- netic parameters were estimated by using sub-model method, and apparent activation energies were calculated according to the Arrhenius equation： The predicted yields coincided well with the experimental values. It shows that the kinetic parameters estimated by using the sub-model method were reliable. |
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| AbstractList | An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in thecatalytic pyrolysis process of Daqing atmospheric residue. The model contains 21 kinetic parameters and one for catalyst deactivation. A series of experiments were carried out in a riser reactor over catalyst named LTB-2. The kinetic parameters were estimated by using sub-model method, and apparent activation energies were calculated according to the Arrhenius equation. The predicted yields coincided well with the experimental values. It shows thatthe kinetic parameters estimated by using the sub-model method were reliable. An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in the catalytic pyrolysis process of Daqing atmospheric residue. The model contains 21 kinetic parameters and one for catalyst deactivation. A series of experiments were carded out in a riser reactor over catalyst named LTB-2. The ki- netic parameters were estimated by using sub-model method, and apparent activation energies were calculated according to the Arrhenius equation： The predicted yields coincided well with the experimental values. It shows that the kinetic parameters estimated by using the sub-model method were reliable. |
| Author | 刘熠斌 陈小博 赵辉 杨朝合 |
| AuthorAffiliation | State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Dongying 257061, China |
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| CitedBy_id | crossref_primary_10_1039_C6CY01886F crossref_primary_10_1016_j_cjche_2020_01_017 crossref_primary_10_1016_j_fuel_2017_09_099 crossref_primary_10_1016_j_jaap_2019_01_009 crossref_primary_10_1016_j_fuel_2013_02_020 crossref_primary_10_1016_j_fuproc_2011_10_023 crossref_primary_10_1021_ef200545m |
| Cites_doi | 10.1016/j.catcom.2006.10.036 10.1021/ef000097a 10.1021/ie00087a003 10.1002/aic.690160316 10.1002/aic.690220412 10.1021/ie00011a013 10.1021/ie00024a007 10.1016/S1004-9541(07)60085-8 10.1021/ie00090a004 10.1021/ie50424a010 10.1021/i260025a018 10.1021/ie030433l 10.1016/j.apcata.2005.11.010 10.1021/ie00090a005 10.1016/S0920-5861(99)00073-5 |
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| Snippet | An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in the catalytic pyrolysis process of Daqing atmospheric... An 8-lump kinetic model was proposed to predict the yields of propylene, ethylene and gasoline in thecatalytic pyrolysis process of Daqing atmospheric residue.... |
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| SubjectTerms | Atmospherics Catalysts catalytic pyrolysis Chemical engineering Ethylene kinetic model Mathematical models parameter estimation Pyrolysis Reaction kinetics Residues sub-model 催化裂解反应 动力学模型 参数估计 |
| Title | Establishment of Kinetic Model for Catalytic Pyrolysis of Daqing Atmospheric Residue |
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