The Dependence of the Dissociation Rate of Methane-SDS Hydrate below Ice Point on Its Manners of Forming and Processing
The dissociation rates of methane hydrates formed with and without the presence of sodium dodecyl sulfate （methane-SDS hydrates）, were measured under atmospheric pressure and temperatures below ice point to investigate the influence of the hydrate production conditions and manners upon its dissociat...
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| Published in | Chinese journal of chemical engineering Vol. 17; no. 1; pp. 128 - 135 |
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| Main Author | |
| Format | Journal Article |
| Language | English |
| Published |
Elsevier B.V
01.02.2009
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1004-9541 2210-321X |
| DOI | 10.1016/S1004-9541(09)60043-4 |
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| Abstract | The dissociation rates of methane hydrates formed with and without the presence of sodium dodecyl sulfate （methane-SDS hydrates）, were measured under atmospheric pressure and temperatures below ice point to investigate the influence of the hydrate production conditions and manners upon its dissociation kinetic behavior. The experimental results demonstrated that the dissociation rate of methane hydrate below ice point is strongly dependent on the manners of hydrate formation and processing. The dissociation rate of hydrate formed quiescently was lower than that of hydrate formed with stirring; the dissociation rate of hydrate formed at lower pressure was higher than that of hydrate formed at higher oressure; the comoaction of hydrate after its formation lowered its stability, i.e., increased＇its dissociation rate.The stability of hydrate could beincreased by prolonging the time period for which hydrate was held at formation temperature and pressure before it was cooled down, or by prolonging the time period for which hydrate was held at dissociation temperature and formation pressure before it was depressurized to atmospheric pressure. It was found that the dissociation rate of methane hydrate varied with the temperature （ranging from 245.2 to 272.2 K） anomalously as reported on the dissociation of methane hydrate without the presence of surfactant as kinetic promoter. The dissociation rate at 268 K was found to be the lowest when the manners and conditions at which hydrates were formed and processed were fixed. |
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| AbstractList | The dissociation rates of methane hydrates formed with and without the presence of sodium dodecylsulfate (methane-SDS hydrates), were measured under atmospheric pressure and temperatures below ice point toinvestigate the influence of the hydrate production conditions and manners upon its dissociation kinetic behavior. The experimental results demonstrated that the dissociation rate of methane hydrate below ice point is strongly dependent on the manners of hydrate formation and processing. The dissociation rate of hydrate formed quiescentlywas lower than that of hydrate formed with stirring; the dissociation rate of hydrate formed at lower pressure was higher than that of hydrate formed at higher pressure; the compaction of hydrate after its formation lowered its stability, i.e., increased its dissociation rate. The stability of hydrate could be increased by prolonging the time periodfor which hydrate was held at formation temperature and pressure before it was cooled down, or by prolonging thetime period for which hydrate was held at dissociation temperature and formation pressure before it was depressurized to atmospheric pressure. It was found that the dissociation rate of methane hydrate varied with the temperature(ranging from 245.2 to 272.2 K) anomalously as reported on the dissociation of methane hydrate without the presence of surfactant as kinetic promoter. The dissociation rate at 268 K was found to be the lowest when the manners and conditions at which hydrates were formed and processed were fixed. The dissociation rates of methane hydrates formed with and without the presence of sodium dodecyl sulfate （methane-SDS hydrates）, were measured under atmospheric pressure and temperatures below ice point to investigate the influence of the hydrate production conditions and manners upon its dissociation kinetic behavior. The experimental results demonstrated that the dissociation rate of methane hydrate below ice point is strongly dependent on the manners of hydrate formation and processing. The dissociation rate of hydrate formed quiescently was lower than that of hydrate formed with stirring; the dissociation rate of hydrate formed at lower pressure was higher than that of hydrate formed at higher oressure; the comoaction of hydrate after its formation lowered its stability, i.e., increased＇its dissociation rate.The stability of hydrate could beincreased by prolonging the time period for which hydrate was held at formation temperature and pressure before it was cooled down, or by prolonging the time period for which hydrate was held at dissociation temperature and formation pressure before it was depressurized to atmospheric pressure. It was found that the dissociation rate of methane hydrate varied with the temperature （ranging from 245.2 to 272.2 K） anomalously as reported on the dissociation of methane hydrate without the presence of surfactant as kinetic promoter. The dissociation rate at 268 K was found to be the lowest when the manners and conditions at which hydrates were formed and processed were fixed. The dissociation rates of methane hydrates formed with and without the presence of sodium dodecylsulfate (methane-SDS hydrates), were measured under atmospheric pressure and temperatures below ice point toinvestigate the influence of the hydrate production conditions and manners upon its dissociation kinetic behavior. The experimental results demonstrated that the dissociation rate of methane hydrate below ice point is strongly dependent on the manners of hydrate formation and processing. The dissociation rate of hydrate formed quiescentlywas lower than that of hydrate formed with stirring; the dissociation rate of hydrate formed at lower pressure was higher than that of hydrate formed at higher pressure; the compaction of hydrate after its formation lowered its stability, i.e., increased its dissociation rate. The stability of hydrate could be increased by prolonging the time periodfor which hydrate was held at formation temperature and pressure before it was cooled down, or by prolonging thetime period for which hydrate was held at dissociation temperature and formation pressure before it was depressurized to atmospheric pressure. It was found that the dissociation rate of methane hydrate varied with the temperature(ranging from 245.2 to 272.2 K) anomalously as reported on the dissociation of methane hydrate without the presence of surfactant as kinetic promoter. The dissociation rate at 268 K was found to be the lowest when the manners and conditions at which hydrates were formed and processed were fixed. |
| Author | 王秀林 陈光进 孙长宇 杨兰英 马庆兰 陈俊 刘鹏 唐绪龙 赵焕伟 陈卫东 |
| AuthorAffiliation | State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing 102249, China Development Engineering Institute, China Oilfield Service Limited, Beijing 101149, China |
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| CitedBy_id | crossref_primary_10_1016_j_cjche_2020_02_003 crossref_primary_10_1002_ceat_201200089 crossref_primary_10_1016_j_jtice_2018_10_007 crossref_primary_10_1021_acs_energyfuels_5b00837 crossref_primary_10_1016_j_fuel_2011_10_029 crossref_primary_10_1016_j_fuel_2024_133194 crossref_primary_10_1016_j_cjche_2024_04_022 crossref_primary_10_1016_j_apenergy_2021_117750 crossref_primary_10_1021_je301153t crossref_primary_10_1016_j_geoen_2023_212412 |
| Cites_doi | 10.1139/p03-018 10.1016/0016-7037(86)90110-9 10.1021/es001148l 10.1016/S0378-3812(01)00460-5 10.1002/aic.690481030 10.1021/jp011435r 10.1039/f19888403731 10.1021/ie50296a010 10.1021/jp012189m 10.1016/j.ces.2004.09.003 10.1002/aic.11005 10.1016/j.ces.2005.05.014 10.1063/1.1748079 10.1029/93RG00268 10.1016/0165-232X(92)90014-L 10.1021/jp003061s 10.1021/jp0526851 10.1016/j.ces.2004.07.010 10.1016/S0009-2509(00)00072-5 |
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| Snippet | The dissociation rates of methane hydrates formed with and without the presence of sodium dodecyl sulfate （methane-SDS hydrates）, were measured under... The dissociation rates of methane hydrates formed with and without the presence of sodium dodecylsulfate (methane-SDS hydrates), were measured under... |
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| SubjectTerms | Atmospheric pressure Barometric pressure Chemical engineering dissociation hydrate Hydrates kinetics Methane hydrates SDS Sodium Stability storage surfactant Surfactants 分解速率 生成方式 甲烷水合物 表面活性剂 |
| Title | The Dependence of the Dissociation Rate of Methane-SDS Hydrate below Ice Point on Its Manners of Forming and Processing |
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