Effect of fullerene coating on silicon thin film anodes for lithium rechargeable batteries
To improve the electrochemical performances of Si thin film anodes for lithium rechargeable batteries, fullerene thin films are prepared by plasma-assisted evaporation methods to be used as coating materials. Analyses via Raman and X-ray photoelectron spectroscopy indicate that amorphous polymeric f...
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| Published in | Journal of solid state electrochemistry Vol. 14; no. 1; pp. 51 - 56 |
|---|---|
| Main Authors | , , |
| Format | Journal Article |
| Language | English |
| Published |
Berlin/Heidelberg
Springer-Verlag
01.01.2010
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| Subjects | |
| Online Access | Get full text |
| ISSN | 1432-8488 1433-0768 |
| DOI | 10.1007/s10008-009-0787-4 |
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| Abstract | To improve the electrochemical performances of Si thin film anodes for lithium rechargeable batteries, fullerene thin films are prepared by plasma-assisted evaporation methods to be used as coating materials. Analyses via Raman and X-ray photoelectron spectroscopy indicate that amorphous polymeric films originated from fullerene are formed on the surface of the silicon thin film. The electrochemical performance of these fullerene-coated silicon thin film as an anode material for rechargeable lithium batteries has been investigated by cyclic voltammetry, charge/discharge tests, and electrochemical impedance spectroscopy. The fullerene-coated Si thin films demonstrated a high specific capacity of above 3,000 mAh g
−1
as well as good capacity retention for 40 cycles. In comparison with bare silicon anodes, the fullerene-coated silicon thin film showed superior and stable cycle performance which can be attributed to the fullerene coating layer which enhances the Li-ion kinetic property at the electrode/electrolyte interface. |
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| AbstractList | To improve the electrochemical performances of Si thin film anodes for lithium rechargeable batteries, fullerene thin films are prepared by plasma-assisted evaporation methods to be used as coating materials. Analyses via Raman and X-ray photoelectron spectroscopy indicate that amorphous polymeric films originated from fullerene are formed on the surface of the silicon thin film. The electrochemical performance of these fullerene-coated silicon thin film as an anode material for rechargeable lithium batteries has been investigated by cyclic voltammetry, charge/discharge tests, and electrochemical impedance spectroscopy. The fullerene-coated Si thin films demonstrated a high specific capacity of above 3,000 mAh g
−1
as well as good capacity retention for 40 cycles. In comparison with bare silicon anodes, the fullerene-coated silicon thin film showed superior and stable cycle performance which can be attributed to the fullerene coating layer which enhances the Li-ion kinetic property at the electrode/electrolyte interface. |
| Author | Lee, Joong Kee Chang, Wonyoung Arie, Arenst Andreas |
| Author_xml | – sequence: 1 givenname: Arenst Andreas surname: Arie fullname: Arie, Arenst Andreas organization: Advanced Energy Materials Processing Laboratory, Battery Research Center, Korea Institute of Science and Technology – sequence: 2 givenname: Wonyoung surname: Chang fullname: Chang, Wonyoung organization: Advanced Energy Materials Processing Laboratory, Battery Research Center, Korea Institute of Science and Technology – sequence: 3 givenname: Joong Kee surname: Lee fullname: Lee, Joong Kee email: leejk@kist.re.kr organization: Advanced Energy Materials Processing Laboratory, Battery Research Center, Korea Institute of Science and Technology |
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| Keywords | Lithium battery Fullerene Coating Silicon thin film Anodes |
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| Title | Effect of fullerene coating on silicon thin film anodes for lithium rechargeable batteries |
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