Dynamic supramolecular polymers built from cucurbit[n]urils and viologens
This review article focuses on supramolecular assemblies involving cucurbit[n]uril‐based containers and viologen guests as key building elements. Cucurbit[n]urils (CB[n], n = 5–8,10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4′‐bipyridinium salts, known as...
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| Published in | Polymer international Vol. 68; no. 4; pp. 572 - 588 |
|---|---|
| Main Authors | , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Chichester, UK
John Wiley & Sons, Ltd
01.04.2019
Wiley Subscription Services, Inc Wiley |
| Subjects | |
| Online Access | Get full text |
| ISSN | 0959-8103 1097-0126 |
| DOI | 10.1002/pi.5709 |
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| Abstract | This review article focuses on supramolecular assemblies involving cucurbit[n]uril‐based containers and viologen guests as key building elements. Cucurbit[n]urils (CB[n], n = 5–8,10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4′‐bipyridinium salts, known as viologens, either as discrete 1:1 inclusion compounds with CB[7] or as ternary inclusion compounds involving two hosts or two guests (2:1 with CB[7] and 1:2 or 1:1:1 with CB[8]). This property is currently being actively exploited to design and prepare self‐assembled dynamic stimuli‐responsive supramolecular polymers including gels, vesicles, films and organized arrays of polymeric microspheres or nanoparticles. This review highlights the main benefits of such polymers and gives an overview of the achievements and progress made in this field over the past decades. © 2018 Society of Chemical Industry
The scope of this review is to highlight the strategies which have been implemented to promote the formation of self‐assembled supramolecular polymers from cucurbit[n]uril (CB[n]) hosts and viologen guests, used as key building elements. The first part provides an overview of the polymeric systems reported in the literature involving these two components. The second part is dedicated to the applications of these specific host–guest processes in ‘soft material’ science. |
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| AbstractList | This review article focuses on supramolecular assemblies involving cucurbit[n]uril‐based containers and viologen guests as key building elements. Cucurbit[n]urils (CB[n], n = 5–8,10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4′‐bipyridinium salts, known as viologens, either as discrete 1:1 inclusion compounds with CB[7] or as ternary inclusion compounds involving two hosts or two guests (2:1 with CB[7] and 1:2 or 1:1:1 with CB[8]). This property is currently being actively exploited to design and prepare self‐assembled dynamic stimuli‐responsive supramolecular polymers including gels, vesicles, films and organized arrays of polymeric microspheres or nanoparticles. This review highlights the main benefits of such polymers and gives an overview of the achievements and progress made in this field over the past decades. © 2018 Society of Chemical Industry This review article focuses on supramolecular assemblies involving cucurbit[n]uril-based containers and viologen guests as key building elements. Cucurbit[n]urils (CB[n], n=5-10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4'-bipyridinium salts, known as viologens, either as discrete 1:1 inclusion compounds with CB[7] or as ternary inclusion compounds involving two hosts or two guests (2:1) with CB[7], and (1:2 or 1:1:1) with CB[8]. This property is currently being actively exploited to design and prepare self-assembled dynamic stimuli-responsive supramolecular polymers including gels, vesicles, films and organized arrays of polymeric microspheres or nanoparticles. This reviews highlights the main benefits of such polymers and gives an overview of the achievements and progresses made in this field over the past decades . This review article focuses on supramolecular assemblies involving cucurbit[n]uril‐based containers and viologen guests as key building elements. Cucurbit[n]urils (CB[n], n = 5–8,10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4′‐bipyridinium salts, known as viologens, either as discrete 1:1 inclusion compounds with CB[7] or as ternary inclusion compounds involving two hosts or two guests (2:1 with CB[7] and 1:2 or 1:1:1 with CB[8]). This property is currently being actively exploited to design and prepare self‐assembled dynamic stimuli‐responsive supramolecular polymers including gels, vesicles, films and organized arrays of polymeric microspheres or nanoparticles. This review highlights the main benefits of such polymers and gives an overview of the achievements and progress made in this field over the past decades. © 2018 Society of Chemical Industry The scope of this review is to highlight the strategies which have been implemented to promote the formation of self‐assembled supramolecular polymers from cucurbit[n]uril (CB[n]) hosts and viologen guests, used as key building elements. The first part provides an overview of the polymeric systems reported in the literature involving these two components. The second part is dedicated to the applications of these specific host–guest processes in ‘soft material’ science. This review article focuses on supramolecular assemblies involving cucurbit[ n ]uril‐based containers and viologen guests as key building elements. Cucurbit[ n ]urils (CB[ n ], n = 5–8,10) are fascinating hosts forming a wide range of inclusion complexes (caviplexes) with 4,4′‐bipyridinium salts, known as viologens, either as discrete 1:1 inclusion compounds with CB[7] or as ternary inclusion compounds involving two hosts or two guests (2:1 with CB[7] and 1:2 or 1:1:1 with CB[8]). This property is currently being actively exploited to design and prepare self‐assembled dynamic stimuli‐responsive supramolecular polymers including gels, vesicles, films and organized arrays of polymeric microspheres or nanoparticles. This review highlights the main benefits of such polymers and gives an overview of the achievements and progress made in this field over the past decades. © 2018 Society of Chemical Industry |
| Author | Guy, Laure Demets, Grégoire Jean‐François Ramos, Ana Paula Bucher, Christophe Correia, Henrique Dias Chowdhury, Shagor |
| Author_xml | – sequence: 1 givenname: Henrique Dias surname: Correia fullname: Correia, Henrique Dias organization: Departamento de Química, Faculdade de Filosofia Ciências e Letras de Ribeirão Preto, Universidade de São Paulo, Av. Bandeirantes 3900, CEP 14040‐901 – sequence: 2 givenname: Shagor surname: Chowdhury fullname: Chowdhury, Shagor organization: Univ Lyon, Ens de Lyon, CNRS UMR 5182, Université Claude Bernard Lyon 1, Laboratoire de Chimie – sequence: 3 givenname: Ana Paula surname: Ramos fullname: Ramos, Ana Paula organization: Departamento de Química, Faculdade de Filosofia Ciências e Letras de Ribeirão Preto, Universidade de São Paulo, Av. Bandeirantes 3900, CEP 14040‐901 – sequence: 4 givenname: Laure surname: Guy fullname: Guy, Laure organization: Univ Lyon, Ens de Lyon, CNRS UMR 5182, Université Claude Bernard Lyon 1, Laboratoire de Chimie – sequence: 5 givenname: Grégoire Jean‐François surname: Demets fullname: Demets, Grégoire Jean‐François email: greg@usp.br organization: Departamento de Química, Faculdade de Filosofia Ciências e Letras de Ribeirão Preto, Universidade de São Paulo, Av. Bandeirantes 3900, CEP 14040‐901 – sequence: 6 givenname: Christophe orcidid: 0000-0003-1803-6733 surname: Bucher fullname: Bucher, Christophe email: christophe.bucher@ens-lyon.fr organization: Univ Lyon, Ens de Lyon, CNRS UMR 5182, Université Claude Bernard Lyon 1, Laboratoire de Chimie |
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| Copyright | 2018 Society of Chemical Industry Copyright © 2019 Society of Chemical Industry Distributed under a Creative Commons Attribution 4.0 International License |
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| Keywords | self-assembly films nanoparticles gels Viologens cucurbit[n]urils polymers |
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| Snippet | This review article focuses on supramolecular assemblies involving cucurbit[n]uril‐based containers and viologen guests as key building elements.... This review article focuses on supramolecular assemblies involving cucurbit[ n ]uril‐based containers and viologen guests as key building elements. Cucurbit[ n... This review article focuses on supramolecular assemblies involving cucurbit[n]uril-based containers and viologen guests as key building elements.... |
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| SubjectTerms | Chemical Sciences Containers cucurbit[n]urils Gels Inclusion complexes Microspheres Nanoparticles Organic chemistry Polymers Salts self‐assembly Supramolecular polymers viologens |
| Title | Dynamic supramolecular polymers built from cucurbit[n]urils and viologens |
| URI | https://onlinelibrary.wiley.com/doi/abs/10.1002%2Fpi.5709 https://www.proquest.com/docview/2190357302 https://hal.science/hal-01927354 |
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