Aqueous charge injection: solvation bonding dynamics, molecular nonbond interactions, and extraordinary solute capabilities

Aqueous charge injection in forms of electrons, protons, lone pairs, ions, and molecular dipoles by solvation is ubiquitously important to our health and life. Pursuing fine-resolution detection and consistent insight into solvation dynamics and solute capabilities has become an increasingly active...

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Published inInternational reviews in physical chemistry Vol. 37; no. 3-4; pp. 363 - 558
Main Author Sun, Chang Q.
Format Journal Article
LanguageEnglish
Published Abingdon Taylor & Francis 02.10.2018
Taylor & Francis Ltd
Subjects
Acid
Alcohols
Aldehydes
anti-HB
base
Catalysis
Charge injection
diffusivity
Electrostatic shielding
Glycine
Hofmeister series
Hydration
hydrogen bond
Hydrogen bonds
Hydrogen peroxide
molecular interaction
phase transition
Phase transitions
phonon spectroscopy
polarization
Proteins
salt
solution viscosity
Solvation
Solvents
Stiffness
Sugar
super-HB
supersolidity
surface stress
Online AccessGet full text
ISSN0144-235X
1366-591X
DOI10.1080/0144235X.2018.1544446

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Abstract Aqueous charge injection in forms of electrons, protons, lone pairs, ions, and molecular dipoles by solvation is ubiquitously important to our health and life. Pursuing fine-resolution detection and consistent insight into solvation dynamics and solute capabilities has become an increasingly active subject. This treatise shows that charge injection by solvation mediates the O:H-O bonding network and properties of a solution through O:H formation, H↔H fragilization, O:⇔:O compression, electrostatic polarization, H 2 O dipolar shielding, solute-solute interaction, and undercoordinated H-O bond contraction. A combination of the hydrogen bond (O:H-O or HB with ':' being the electron lone pairs of oxygen) cooperativity notion and the differential phonon spectrometrics (DPS) has enabled quantitative information on the following: (i) the number fraction and phonon stiffness of HBs transiting from the mode of ordinary water to hydration; (ii) solute-solvent and solute-solute molecular nonbond interactions; and (iii) interdependence of skin stress, solution viscosity, molecular diffusivity, solvation thermodynamics, and critical pressures and temperatures for phase transitions. An examination of solvation dynamics has clarified the following: (i) the excessive protons create the H↔H or anti-HB point breaker to disrupt the acidic solution network and surface stress. (ii) The excessive lone pairs generate the O:⇔:O or super-HB point compressor to shorten the O:H nonbond but lengthen the H-O bond in H 2 O 2 and basic solutions; yet, bond-order-deficiency shortens and stiffens the H-O bond due H 2 O 2 and OH − solutes. (iii) Ions serve each as a charge center that aligns, clusters, stretches, and polarizes their neighboring HBs to form hydration shells. (iv) Solvation of alcohols, aldehydes, complex salts, carboxylic and formic acids, glycine, and sugars distorts the solute-solvent interface structures with the involvement of the anti-HB or the super-HB. Extending the knowledge and strategies to catalysis, solution-protein, drug-cell, liquid-solid, colloid-matrix interactions and molecular crystals would be even more fascinating and rewarding.
AbstractList Aqueous charge injection in forms of electrons, protons, lone pairs, ions, and molecular dipoles by solvation is ubiquitously important to our health and life. Pursuing fine-resolution detection and consistent insight into solvation dynamics and solute capabilities has become an increasingly active subject. This treatise shows that charge injection by solvation mediates the O:H-O bonding network and properties of a solution through O:H formation, H[left right arrow]H fragilization, O:[left right double arrow]:O compression, electrostatic polarization, H2O dipolar shielding, solute-solute interaction, and undercoordinated H-O bond contraction. A combination of the hydrogen bond (O:H-O or HB with ':' being the electron lone pairs of oxygen) cooperativity notion and the differential phonon spectrometrics (DPS) has enabled quantitative information on the following: (i) the number fraction and phonon stiffness of HBs transiting from the mode of ordinary water to hydration; (ii) solute-solvent and solute-solute molecular nonbond interactions; and (iii) interdependence of skin stress, solution viscosity, molecular diffusivity, solvation thermodynamics, and critical pressures and temperatures for phase transitions. An examination of solvation dynamics has clarified the following: (i) the excessive protons create the H[left right arrow]H or anti-HB point breaker to disrupt the acidic solution network and surface stress. (ii) The excessive lone pairs generate the O:[left right double arrow]:O or super-HB point compressor to shorten the O:H nonbond but lengthen the H-O bond in H2O2 and basic solutions; yet, bond-order-deficiency shortens and stiffens the H-O bond due H2O2 and OH- solutes. (iii) Ions serve each as a charge center that aligns, clusters, stretches, and polarizes their neighboring HBs to form hydration shells. (iv) Solvation of alcohols, aldehydes, complex salts, carboxylic and formic acids, glycine, and sugars distorts the solute-solvent interface structures with the involvement of the anti-HB or the super-HB. Extending the knowledge and strategies to catalysis, solution-protein, drug-cell, liquid-solid, colloid-matrix interactions and molecular crystals would be even more fascinating and rewarding.
Aqueous charge injection in forms of electrons, protons, lone pairs, ions, and molecular dipoles by solvation is ubiquitously important to our health and life. Pursuing fine-resolution detection and consistent insight into solvation dynamics and solute capabilities has become an increasingly active subject. This treatise shows that charge injection by solvation mediates the O:H-O bonding network and properties of a solution through O:H formation, H↔H fragilization, O:⇔:O compression, electrostatic polarization, H 2 O dipolar shielding, solute-solute interaction, and undercoordinated H-O bond contraction. A combination of the hydrogen bond (O:H-O or HB with ':' being the electron lone pairs of oxygen) cooperativity notion and the differential phonon spectrometrics (DPS) has enabled quantitative information on the following: (i) the number fraction and phonon stiffness of HBs transiting from the mode of ordinary water to hydration; (ii) solute-solvent and solute-solute molecular nonbond interactions; and (iii) interdependence of skin stress, solution viscosity, molecular diffusivity, solvation thermodynamics, and critical pressures and temperatures for phase transitions. An examination of solvation dynamics has clarified the following: (i) the excessive protons create the H↔H or anti-HB point breaker to disrupt the acidic solution network and surface stress. (ii) The excessive lone pairs generate the O:⇔:O or super-HB point compressor to shorten the O:H nonbond but lengthen the H-O bond in H 2 O 2 and basic solutions; yet, bond-order-deficiency shortens and stiffens the H-O bond due H 2 O 2 and OH − solutes. (iii) Ions serve each as a charge center that aligns, clusters, stretches, and polarizes their neighboring HBs to form hydration shells. (iv) Solvation of alcohols, aldehydes, complex salts, carboxylic and formic acids, glycine, and sugars distorts the solute-solvent interface structures with the involvement of the anti-HB or the super-HB. Extending the knowledge and strategies to catalysis, solution-protein, drug-cell, liquid-solid, colloid-matrix interactions and molecular crystals would be even more fascinating and rewarding.
Author Sun, Chang Q.
Author_xml – sequence: 1
  givenname: Chang Q.
  surname: Sun
  fullname: Sun, Chang Q.
  email: ecqsun@ntu.edu.sg
  organization: NOVITAS, EEE, Nanyang Technological University
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Snippet Aqueous charge injection in forms of electrons, protons, lone pairs, ions, and molecular dipoles by solvation is ubiquitously important to our health and life....
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SubjectTerms Acid
Alcohols
Aldehydes
anti-HB
base
Catalysis
Charge injection
diffusivity
Electrostatic shielding
Glycine
Hofmeister series
Hydration
hydrogen bond
Hydrogen bonds
Hydrogen peroxide
molecular interaction
phase transition
Phase transitions
phonon spectroscopy
polarization
Proteins
salt
solution viscosity
Solvation
Solvents
Stiffness
Sugar
super-HB
supersolidity
surface stress
Title Aqueous charge injection: solvation bonding dynamics, molecular nonbond interactions, and extraordinary solute capabilities
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