Nanosized Rh grown on single-walled carbon nanohorns for efficient methanol oxidation reaction
Reasonable design and controllable synthesis of non-Pt catalysts with high methanol oxidation activity are regarded as a valid way to promote the large-scale commercial applications of direct methanol fuel cells (DMFCs). Herein, we develop a convenient and cost-effective approach to the successful f...
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| Published in | Rare metals Vol. 41; no. 6; pp. 2108 - 2117 |
|---|---|
| Main Authors | , , , , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Beijing
Nonferrous Metals Society of China
01.06.2022
Springer Nature B.V |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1001-0521 1867-7185 |
| DOI | 10.1007/s12598-021-01882-2 |
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| Abstract | Reasonable design and controllable synthesis of non-Pt catalysts with high methanol oxidation activity are regarded as a valid way to promote the large-scale commercial applications of direct methanol fuel cells (DMFCs). Herein, we develop a convenient and cost-effective approach to the successful fabrication of nanosized Rh grown on single-walled carbon nanohorns (Rh/SWCNH) as anode catalysts for DMFCs. The unique architectural configuration endows the as-obtained hybrids with a series of intriguing structural merits, including large specific surface areas, abundant opened holes, optimized electronic structures, homogeneous Rh dispersion, and good electrical conductivity. As a consequence, the resulting Rh/SWCNH catalysts exhibit exceptional electrocatalytic properties in terms of a large electrochemically active surface area of 102.5 m
2
·g
−1
, a high mass activity of 784.0 mA·mg
−1
, as well as reliable long-term durability towards the methanol oxidation reaction in alkaline media, thereby holding great potential as alternatives for commercial Pt/carbon black and Pd/carbon black catalysts.
Graphic abstract |
|---|---|
| AbstractList | Reasonable design and controllable synthesis of non-Pt catalysts with high methanol oxidation activity are regarded as a valid way to promote the large-scale commercial applications of direct methanol fuel cells (DMFCs). Herein, we develop a convenient and cost-effective approach to the successful fabrication of nanosized Rh grown on single-walled carbon nanohorns (Rh/SWCNH) as anode catalysts for DMFCs. The unique architectural configuration endows the as-obtained hybrids with a series of intriguing structural merits, including large specific surface areas, abundant opened holes, optimized electronic structures, homogeneous Rh dispersion, and good electrical conductivity. As a consequence, the resulting Rh/SWCNH catalysts exhibit exceptional electrocatalytic properties in terms of a large electrochemically active surface area of 102.5 m2·g−1, a high mass activity of 784.0 mA·mg−1, as well as reliable long-term durability towards the methanol oxidation reaction in alkaline media, thereby holding great potential as alternatives for commercial Pt/carbon black and Pd/carbon black catalysts.Graphic abstract Reasonable design and controllable synthesis of non-Pt catalysts with high methanol oxidation activity are regarded as a valid way to promote the large-scale commercial applications of direct methanol fuel cells (DMFCs). Herein, we develop a convenient and cost-effective approach to the successful fabrication of nanosized Rh grown on single-walled carbon nanohorns (Rh/SWCNH) as anode catalysts for DMFCs. The unique architectural configuration endows the as-obtained hybrids with a series of intriguing structural merits, including large specific surface areas, abundant opened holes, optimized electronic structures, homogeneous Rh dispersion, and good electrical conductivity. As a consequence, the resulting Rh/SWCNH catalysts exhibit exceptional electrocatalytic properties in terms of a large electrochemically active surface area of 102.5 m 2 ·g −1 , a high mass activity of 784.0 mA·mg −1 , as well as reliable long-term durability towards the methanol oxidation reaction in alkaline media, thereby holding great potential as alternatives for commercial Pt/carbon black and Pd/carbon black catalysts. Graphic abstract |
| Author | He, Hai-Yan Guo, Xiang-Jie Li, Ya-Nan Zhang, Qi Yang, Lu Chen, Yang Huang, Hua-Jie Xu, Xing-Tao |
| Author_xml | – sequence: 1 givenname: Xiang-Jie surname: Guo fullname: Guo, Xiang-Jie organization: College of Mechanics and Materials, Hohai University – sequence: 2 givenname: Qi surname: Zhang fullname: Zhang, Qi organization: College of Mechanics and Materials, Hohai University – sequence: 3 givenname: Ya-Nan surname: Li fullname: Li, Ya-Nan organization: College of Mechanics and Materials, Hohai University – sequence: 4 givenname: Yang surname: Chen fullname: Chen, Yang organization: College of Mechanics and Materials, Hohai University – sequence: 5 givenname: Lu surname: Yang fullname: Yang, Lu organization: College of Mechanics and Materials, Hohai University – sequence: 6 givenname: Hai-Yan surname: He fullname: He, Hai-Yan organization: College of Mechanics and Materials, Hohai University – sequence: 7 givenname: Xing-Tao surname: Xu fullname: Xu, Xing-Tao organization: International Center for Materials Nanoarchitectonics (WPI-MANA), National Institute for Materials Science – sequence: 8 givenname: Hua-Jie orcidid: 0000-0001-5685-4994 surname: Huang fullname: Huang, Hua-Jie email: huanghuajie@hhu.edu.cn organization: College of Mechanics and Materials, Hohai University |
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| Keywords | Rhodium Carbon nanohorns Electrocatalysts Methanol oxidation Fuel cells |
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| SubjectTerms | Biomaterials Carbon Carbon black Catalysts Chemical synthesis Chemistry and Materials Science Electrical resistivity Energy Fuel cells Materials Engineering Materials Science Metallic Materials Methanol Nanoscale Science and Technology Original Article Oxidation Palladium Physical Chemistry Rhodium Surface area |
| Title | Nanosized Rh grown on single-walled carbon nanohorns for efficient methanol oxidation reaction |
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