Intercluster aurophilicity-driven aggregation lighting circularly polarized luminescence of chiral gold clusters

Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU 4 PL 4 /Au 4 PD 4 and ( Au 4 L 4 ) n /( Au 4 D 4 ) n with atomic precision. In Au 4 PL 4 /Au 4 PD 4 , the discrete chiral Au 4 -based aggregation-induced emission (AIE) luminogens are separated by bulky substitutes. The c...

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Published in	Nano research Vol. 13; no. 12; pp. 3248 - 3252
Main Authors	Han, Zhen, Zhao, Xueli, Peng, Peng, Li, Si, Zhang, Chong, Cao, Man, Li, Kai, Wang, Zhao-Yang, Zang, Shuang-Quan
Format	Journal Article
Language	English
Published	Beijing Tsinghua University Press 01.12.2020
Subjects	Agglomeration Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Chemistry and Materials Science Circular polarization Clean energy Condensed Matter Physics Crystallization Emissions Gold Ligands Light emitting diodes Luminescence Materials Science Metal clusters Nanotechnology Organic light emitting diodes Photoluminescence Photons Quantum dots Research Article Single crystals gold cluster aggregation-induced emission atomic precision circularly polarized luminescence intercluster aurophilicity
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ISSN	1998-0124 1998-0000
DOI	10.1007/s12274-020-2997-0

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Abstract	Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU 4 PL 4 /Au 4 PD 4 and ( Au 4 L 4 ) n /( Au 4 D 4 ) n with atomic precision. In Au 4 PL 4 /Au 4 PD 4 , the discrete chiral Au 4 -based aggregation-induced emission (AIE) luminogens are separated by bulky substitutes. The corresponding aggregates are cyan-emitting with a photoluminescence quantum yield (PLQY) of 14.4%. Upon decreasing the size of the substituents, these chiral Au 4 clusters are strung together by inter-cluster Au-Au interactions, which cause a low-energy green emission from the aggregated ( Au 4 L 4 ) n /(Au 4 D 4 ) n with a much higher PLQY of 41.4% and more intense circularly polarised photoluminescence (CPL) with a dissymmetry factor \| g PL \| of 7.0 × 10 − 3 . Using ( Au 4 L 4 ) n / (Au 4 D 4 ) n , circularly polarised organic light-emitting diodes (CP-OLEDs) were for the first time fabricated with \| g EL \| = \| g PL \|. These findings signify that inter-cluster metallophilic interactions are a new and important type of driving force for AIE and crystallization-induced emission (CIE), suggesting great potential of CPL-active metal clusters in CP-OLEDs.
AbstractList	Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU4PL4/Au4PD4 and (Au4L4)n/(Au4D4)n with atomic precision. In Au4PL4/Au4PD4, the discrete chiral Au4-based aggregation-induced emission (AIE) luminogens are separated by bulky substitutes. The corresponding aggregates are cyan-emitting with a photoluminescence quantum yield (PLQY) of 14.4%. Upon decreasing the size of the substituents, these chiral Au4 clusters are strung together by inter-cluster Au-Au interactions, which cause a low-energy green emission from the aggregated (Au4L4)n/(Au4D4)n with a much higher PLQY of 41.4% and more intense circularly polarised photoluminescence (CPL) with a dissymmetry factor \|gPL\| of 7.0 × 10−3. Using (Au4L4)n/(Au4D4)n, circularly polarised organic light-emitting diodes (CP-OLEDs) were for the first time fabricated with \|gEL\| = \|gPL\|. These findings signify that inter-cluster metallophilic interactions are a new and important type of driving force for AIE and crystallization-induced emission (CIE), suggesting great potential of CPL-active metal clusters in CP-OLEDs. Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU 4 PL 4 /Au 4 PD 4 and ( Au 4 L 4 ) n /( Au 4 D 4 ) n with atomic precision. In Au 4 PL 4 /Au 4 PD 4 , the discrete chiral Au 4 -based aggregation-induced emission (AIE) luminogens are separated by bulky substitutes. The corresponding aggregates are cyan-emitting with a photoluminescence quantum yield (PLQY) of 14.4%. Upon decreasing the size of the substituents, these chiral Au 4 clusters are strung together by inter-cluster Au-Au interactions, which cause a low-energy green emission from the aggregated ( Au 4 L 4 ) n /(Au 4 D 4 ) n with a much higher PLQY of 41.4% and more intense circularly polarised photoluminescence (CPL) with a dissymmetry factor \| g PL \| of 7.0 × 10 − 3 . Using ( Au 4 L 4 ) n / (Au 4 D 4 ) n , circularly polarised organic light-emitting diodes (CP-OLEDs) were for the first time fabricated with \| g EL \| = \| g PL \|. These findings signify that inter-cluster metallophilic interactions are a new and important type of driving force for AIE and crystallization-induced emission (CIE), suggesting great potential of CPL-active metal clusters in CP-OLEDs.
Author	Li, Kai Zang, Shuang-Quan Han, Zhen Peng, Peng Cao, Man Wang, Zhao-Yang Li, Si Zhao, Xueli Zhang, Chong
Author_xml	– sequence: 1 givenname: Zhen surname: Han fullname: Han, Zhen organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 2 givenname: Xueli surname: Zhao fullname: Zhao, Xueli organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 3 givenname: Peng surname: Peng fullname: Peng, Peng organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 4 givenname: Si surname: Li fullname: Li, Si organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 5 givenname: Chong surname: Zhang fullname: Zhang, Chong organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 6 givenname: Man surname: Cao fullname: Cao, Man organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 7 givenname: Kai surname: Li fullname: Li, Kai organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 8 givenname: Zhao-Yang surname: Wang fullname: Wang, Zhao-Yang email: wangzy@zzu.edu.cn organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University – sequence: 9 givenname: Shuang-Quan surname: Zang fullname: Zang, Shuang-Quan email: zangsqzg@zzu.edu.cn organization: Green Catalysis Center, and College of Chemistry, Zhengzhou University
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Snippet	Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU 4 PL 4 /Au 4 PD 4 and ( Au 4 L 4 ) n /( Au 4 D 4 ) n with atomic precision. In... Herein, we prepared two novel pairs of enantiomeric gold cluster complexes, AU4PL4/Au4PD4 and (Au4L4)n/(Au4D4)n with atomic precision. In Au4PL4/Au4PD4, the...
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SubjectTerms	Agglomeration Atomic/Molecular Structure and Spectra Biomedicine Biotechnology Chemistry and Materials Science Circular polarization Clean energy Condensed Matter Physics Crystallization Emissions Gold Ligands Light emitting diodes Luminescence Materials Science Metal clusters Nanotechnology Organic light emitting diodes Photoluminescence Photons Quantum dots Research Article Single crystals
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Title	Intercluster aurophilicity-driven aggregation lighting circularly polarized luminescence of chiral gold clusters
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