Preparation of mechanically enhanced supramolecular carbon nanotube (CNT) film using a water-soluble π–π bonding linker
Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the π -electron-rich phenyl, naphthalenyl, and pyrenyl end-functionalized polyethylene oxides (PEOs) as supramolecular linkers, followed by vacuum filtration. Among them, the supramolecular CNT film...
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| Published in | Carbon Letters Vol. 29; no. 5; pp. 461 - 469 |
|---|---|
| Main Authors | , , , , |
| Format | Journal Article |
| Language | English |
| Published |
Singapore
Springer Singapore
01.10.2019
Springer Nature B.V 한국탄소학회 |
| Subjects | |
| Online Access | Get full text |
| ISSN | 1976-4251 2233-4998 |
| DOI | 10.1007/s42823-019-00048-6 |
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| Abstract | Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the
π
-electron-rich phenyl, naphthalenyl, and pyrenyl end-functionalized polyethylene oxides (PEOs) as supramolecular linkers, followed by vacuum filtration. Among them, the supramolecular CNT film produced by the pyrenyl end-functionalized PEO (PEO-Py) exhibited the highest mechanical strength, which was ~ 1.5–2 times higher than that of the CNT films produced using the typical dispersant, Triton X-100, although the functionality of PEO-Py was lower than that prepared using other linkers, and the content of PEO-Py in the CNT films was lower than that obtained using Triton X-100. Fluorescence and UV–Vis spectroscopy demonstrated that the improved mechanical properties of the supramolecular CNT film result from the formation of
π
–
π
interactions between the CNT and the pyrene moieties of the PEO-Py linker. Finally, the supramolecular CNT film exhibited a 40–50 dB electromagnetic shielding efficiency through hybridization with silver nanowires. |
|---|---|
| AbstractList | Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the
π
-electron-rich phenyl, naphthalenyl, and pyrenyl end-functionalized polyethylene oxides (PEOs) as supramolecular linkers, followed by vacuum filtration. Among them, the supramolecular CNT film produced by the pyrenyl end-functionalized PEO (PEO-Py) exhibited the highest mechanical strength, which was ~ 1.5–2 times higher than that of the CNT films produced using the typical dispersant, Triton X-100, although the functionality of PEO-Py was lower than that prepared using other linkers, and the content of PEO-Py in the CNT films was lower than that obtained using Triton X-100. Fluorescence and UV–Vis spectroscopy demonstrated that the improved mechanical properties of the supramolecular CNT film result from the formation of
π
–
π
interactions between the CNT and the pyrene moieties of the PEO-Py linker. Finally, the supramolecular CNT film exhibited a 40–50 dB electromagnetic shielding efficiency through hybridization with silver nanowires. Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the π-electron-rich phenyl, naphthalenyl, and pyrenyl end-functionalized polyethylene oxides (PEOs) as supramolecular linkers, followed by vacuum filtration. Among them, the supramolecular CNT film produced by the pyrenyl end-functionalized PEO (PEO-Py) exhibited the highest mechanical strength, which was ~ 1.5–2 times higher than that of the CNT films produced using the typical dispersant, Triton X-100, although the functionality of PEO-Py was lower than that prepared using other linkers, and the content of PEO-Py in the CNT films was lower than that obtained using Triton X-100. Fluorescence and UV–Vis spectroscopy demonstrated that the improved mechanical properties of the supramolecular CNT film result from the formation of π–π interactions between the CNT and the pyrene moieties of the PEO-Py linker. Finally, the supramolecular CNT film exhibited a 40–50 dB electromagnetic shielding efficiency through hybridization with silver nanowires. KCI Citation Count: 1 Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the π-electron-rich phenyl, naphthalenyl, and pyrenyl end-functionalized polyethylene oxides (PEOs) as supramolecular linkers, followed by vacuum filtration. Among them, the supramolecular CNT film produced by the pyrenyl end-functionalized PEO (PEO-Py) exhibited the highest mechanical strength, which was ~ 1.5–2 times higher than that of the CNT films produced using the typical dispersant, Triton X-100, although the functionality of PEO-Py was lower than that prepared using other linkers, and the content of PEO-Py in the CNT films was lower than that obtained using Triton X-100. Fluorescence and UV–Vis spectroscopy demonstrated that the improved mechanical properties of the supramolecular CNT film result from the formation of π–π interactions between the CNT and the pyrene moieties of the PEO-Py linker. Finally, the supramolecular CNT film exhibited a 40–50 dB electromagnetic shielding efficiency through hybridization with silver nanowires. |
| Author | Jeong, Hyein Kim, Kun Won Yoo, Moonseong Chung, Jae Woo Lee, Jun-Woo |
| Author_xml | – sequence: 1 givenname: Jun-Woo surname: Lee fullname: Lee, Jun-Woo organization: Department of Information Communication, Materials and Chemistry Convergence Technology, Soongsil University – sequence: 2 givenname: Moonseong surname: Yoo fullname: Yoo, Moonseong organization: Department of Information Communication, Materials and Chemistry Convergence Technology, Soongsil University – sequence: 3 givenname: Kun Won surname: Kim fullname: Kim, Kun Won organization: Department of Information Communication, Materials and Chemistry Convergence Technology, Soongsil University – sequence: 4 givenname: Hyein surname: Jeong fullname: Jeong, Hyein organization: Department of Information Communication, Materials and Chemistry Convergence Technology, Soongsil University – sequence: 5 givenname: Jae Woo surname: Chung fullname: Chung, Jae Woo email: jwchung@ssu.ac.kr organization: Department of Information Communication, Materials and Chemistry Convergence Technology, Soongsil University, Department of Organic Materials and Fiber Engineering, Soongsil University |
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| Snippet | Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the
π
-electron-rich phenyl, naphthalenyl, and pyrenyl... Mechanically enhanced supramolecular carbon nanotube (CNT) films were prepared in water by employing the π-electron-rich phenyl, naphthalenyl, and pyrenyl... |
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| SubjectTerms | Carbon Carbon nanotubes Characterization and Evaluation of Materials Chemistry and Materials Science Dispersants Electromagnetic shielding Electrons Hybridization Hydrocarbons Materials Engineering Materials Science Mechanical properties Molecular weight Nanotechnology Nanowires NMR Nuclear magnetic resonance Original Article Pi-electrons Polyethylene Polyethylene oxide Silver Spectroscopy Spectrum analysis Surfactants Toxicity Vacuum filtration 자연과학일반 |
| Title | Preparation of mechanically enhanced supramolecular carbon nanotube (CNT) film using a water-soluble π–π bonding linker |
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