Bioresourced fillers for rubber composite sustainability: current development and future opportunities

Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black, produced by partial combustion or thermal decomposition of petroleum hydrocarbons, is by far the most dominant filler of rubber composites, followed...

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Published inGreen chemistry : an international journal and green chemistry resource : GC Vol. 23; no. 15; pp. 5337 - 5378
Main Authors Chang, Boon Peng, Gupta, Arvind, Muthuraj, Rajendran, Mekonnen, Tizazu H
Format Journal Article
LanguageEnglish
Published Cambridge Royal Society of Chemistry 02.08.2021
Subjects
biochar
biocomposites
Biomedical materials
Black carbon
Calcium carbonate
Carbon
Carbon black
Carbon footprint
Cellulose
Charcoal
Chemical properties
clay
Clay minerals
combustion
Composite materials
Environmental impact
Fillers
Footprint analysis
Fossil fuels
Green chemistry
lignin
manufacturing
Morphology
Nanocrystals
petroleum
Petroleum hydrocarbons
Physicochemical properties
Plants
Polysaccharides
Renewable resources
Rubber
Saccharides
Silica
Silicon dioxide
soot
Sustainability
Sustainable development
Sustainable materials
talc
Thermal decomposition
thermal degradation
Online AccessGet full text
ISSN1463-9262
1463-9270
1463-9270
DOI10.1039/d1gc01115d

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Abstract Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black, produced by partial combustion or thermal decomposition of petroleum hydrocarbons, is by far the most dominant filler of rubber composites, followed by mineral fillers ( e.g. silica, talc, clay, calcium carbonate, etc .). However, the manufacture of carbon black has a considerable carbon footprint. Similarly, mineral fillers also do not come without challenges, including poor compatibility with rubber matrices and high density. Consequently, the need for sustainable and green fillers with a low or even zero carbon footprint has dramatically increased. In recent years, plant-derived sustainable materials, such as cellulose nanocrystals, natural fibers, lignin, biochar, polysaccharides, etc ., have been extensively investigated as substitute or complementary fillers of rubbers. In this work, we critically reviewed recent developments in the innovation and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure-processing-property relationships in rubber composites. A wide range of biofillers with an array of structure, morphology, and physico-chemical properties and their various attributes in different rubbers are intensively reviewed and discussed. Effective preparation strategies and surface modification platforms on the different biofillers to develop high-performance sustainable rubber biocomposites were critically reviewed. Finally, future perspectives for biofillers in rubber composite applications and challenges are discussed. This article reviewed the recent progress in the development and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure-processing-property relationship of rubber composites.
AbstractList Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black, produced by partial combustion or thermal decomposition of petroleum hydrocarbons, is by far the most dominant filler of rubber composites, followed by mineral fillers ( e.g. silica, talc, clay, calcium carbonate, etc .). However, the manufacture of carbon black has a considerable carbon footprint. Similarly, mineral fillers also do not come without challenges, including poor compatibility with rubber matrices and high density. Consequently, the need for sustainable and green fillers with a low or even zero carbon footprint has dramatically increased. In recent years, plant-derived sustainable materials, such as cellulose nanocrystals, natural fibers, lignin, biochar, polysaccharides, etc ., have been extensively investigated as substitute or complementary fillers of rubbers. In this work, we critically reviewed recent developments in the innovation and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure-processing-property relationships in rubber composites. A wide range of biofillers with an array of structure, morphology, and physico-chemical properties and their various attributes in different rubbers are intensively reviewed and discussed. Effective preparation strategies and surface modification platforms on the different biofillers to develop high-performance sustainable rubber biocomposites were critically reviewed. Finally, future perspectives for biofillers in rubber composite applications and challenges are discussed. This article reviewed the recent progress in the development and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure-processing-property relationship of rubber composites.
Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black, produced by partial combustion or thermal decomposition of petroleum hydrocarbons, is by far the most dominant filler of rubber composites, followed by mineral fillers (e.g. silica, talc, clay, calcium carbonate, etc.). However, the manufacture of carbon black has a considerable carbon footprint. Similarly, mineral fillers also do not come without challenges, including poor compatibility with rubber matrices and high density. Consequently, the need for sustainable and green fillers with a low or even zero carbon footprint has dramatically increased. In recent years, plant-derived sustainable materials, such as cellulose nanocrystals, natural fibers, lignin, biochar, polysaccharides, etc., have been extensively investigated as substitute or complementary fillers of rubbers. In this work, we critically reviewed recent developments in the innovation and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure–processing–property relationships in rubber composites. A wide range of biofillers with an array of structure, morphology, and physico-chemical properties and their various attributes in different rubbers are intensively reviewed and discussed. Effective preparation strategies and surface modification platforms on the different biofillers to develop high-performance sustainable rubber biocomposites were critically reviewed. Finally, future perspectives for biofillers in rubber composite applications and challenges are discussed.
Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black, produced by partial combustion or thermal decomposition of petroleum hydrocarbons, is by far the most dominant filler of rubber composites, followed by mineral fillers ( e.g. silica, talc, clay, calcium carbonate, etc .). However, the manufacture of carbon black has a considerable carbon footprint. Similarly, mineral fillers also do not come without challenges, including poor compatibility with rubber matrices and high density. Consequently, the need for sustainable and green fillers with a low or even zero carbon footprint has dramatically increased. In recent years, plant-derived sustainable materials, such as cellulose nanocrystals, natural fibers, lignin, biochar, polysaccharides, etc ., have been extensively investigated as substitute or complementary fillers of rubbers. In this work, we critically reviewed recent developments in the innovation and utilization of sustainable biofillers for rubber composite applications, emphasizing the effect of the filler on the structure–processing–property relationships in rubber composites. A wide range of biofillers with an array of structure, morphology, and physico-chemical properties and their various attributes in different rubbers are intensively reviewed and discussed. Effective preparation strategies and surface modification platforms on the different biofillers to develop high-performance sustainable rubber biocomposites were critically reviewed. Finally, future perspectives for biofillers in rubber composite applications and challenges are discussed.
Author Muthuraj, Rajendran
Mekonnen, Tizazu H
Gupta, Arvind
Chang, Boon Peng
AuthorAffiliation Department of Chemical Engineering
Waterloo Institute for Nanotechnology
University of Waterloo
Worn Again Technologies Ltd
Institute of Polymer Research
AuthorAffiliation_xml – name: Department of Chemical Engineering
– name: Worn Again Technologies Ltd
– name: Institute of Polymer Research
– name: Waterloo Institute for Nanotechnology
– name: University of Waterloo
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  givenname: Boon Peng
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  givenname: Tizazu H
  surname: Mekonnen
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Notes Dr. Rajendran Muthuraj is currently a Polymer Scientist with Worn Again Technologies Ltd, UK. From 2015-2018, he was a post-doctoral researcher at the University of Bolton, UK, IMT Mines Ales, France, and the University of South Brittany, France. He received his Ph.D. in polymer engineering from the University of Guelph, Canada in 2015. His research interests focus on sustainable polymeric material development for various applications including packaging. He has published several peer-reviewed journal articles and book chapters. He has also received the Innovation of the Year Award from the University of Guelph, Canada for innovating a high-performance and 100% compostable bio-composite.
Dr. Tizazu H. Mekonnen is an Assistant Professor of Chemical Engineering at the University of Waterloo. Prior to his faculty position, he worked as a Polymer Engineering and Nanomaterial Scientist at E.I. DuPont. In his current role, he runs a Sustainable Polymers lab and trains graduate students and postdoctoral fellows in the next-generation sustainable polymer systems. His group actively researches on renewable polymer design, sustainable nanomaterials, polymer modifications, and processing-structure-property correlations of polymers for material applications (thin films, coatings, rubber products, engineering composites, and adhesives). He has also developed a strong collaboration with the polymer, rubber/elastomer, composites, agroforestry, and confectionery and food industries.
Dr. Arvind Gupta received his Ph.D. from IIT-Guwahati, India (2018). He is currently a Postdoctoral Fellow at the University of Waterloo, Canada. His research focuses on the development of new formulations based on conventional plastics and renewable bioplastics and biobased polymers for commercial applications. Preparation of Shape memory polyurethane, polymer synthesis, and
Dr. Boon Peng Chang received his Ph.D. from the University of Science Malaysia (2014) under the supervision of Prof. Hazizan Md Akil. He has worked as a postdoctoral fellow in the Bioproducts Discovery and Development Centre, University of Guelph, Canada, under the supervision of Prof. Amar Mohanty and Prof. Manjusri Misra. He is currently a research associate in the Department of Chemical Engineering, University of Waterloo, Canada, under the supervision of Prof. Tizazu Mekonnen. His main research focuses on the production and characterization of environmentally friendly polymer blends and biocomposites from renewable resources; and thermochemical conversion of agro-wastes into value-added products.
in situ
polymerization are key areas of his research work. To date, he has published 20 research papers on his research topics in peer-reviewed international journals. Also, he has filed 4 patents (2 granted) and written several book chapters to his credit.
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Snippet Ending the fossil fuel era towards a sustainable future will require high-performing renewable materials with a low environmental impact. Carbon black,...
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SubjectTerms biochar
biocomposites
Biomedical materials
Black carbon
Calcium carbonate
Carbon
Carbon black
Carbon footprint
Cellulose
Charcoal
Chemical properties
clay
Clay minerals
combustion
Composite materials
Environmental impact
Fillers
Footprint analysis
Fossil fuels
Green chemistry
lignin
manufacturing
Morphology
Nanocrystals
petroleum
Petroleum hydrocarbons
Physicochemical properties
Plants
Polysaccharides
Renewable resources
Rubber
Saccharides
Silica
Silicon dioxide
soot
Sustainability
Sustainable development
Sustainable materials
talc
Thermal decomposition
thermal degradation
Title Bioresourced fillers for rubber composite sustainability: current development and future opportunities
URI https://www.proquest.com/docview/2557217247
https://www.proquest.com/docview/2636421606
Volume 23
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